Formation of an Electron-Phonon Bifluid in Bulk Antimony

The flow of charge and entropy in solids usually depends on collisions decaying quasiparticle momentum. Hydrodynamic corrections can emerge, however, if most collisions among quasiparticles conserve momentum and the mean-free path approaches the sample dimensions. Here, through a study of electrical...

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Main Authors: Alexandre Jaoui, Adrien Gourgout, Gabriel Seyfarth, Alaska Subedi, Thomas Lorenz, Benoît Fauqué, Kamran Behnia
Format: Article
Language:English
Published: American Physical Society 2022-08-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.12.031023
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author Alexandre Jaoui
Adrien Gourgout
Gabriel Seyfarth
Alaska Subedi
Thomas Lorenz
Benoît Fauqué
Kamran Behnia
author_facet Alexandre Jaoui
Adrien Gourgout
Gabriel Seyfarth
Alaska Subedi
Thomas Lorenz
Benoît Fauqué
Kamran Behnia
author_sort Alexandre Jaoui
collection DOAJ
description The flow of charge and entropy in solids usually depends on collisions decaying quasiparticle momentum. Hydrodynamic corrections can emerge, however, if most collisions among quasiparticles conserve momentum and the mean-free path approaches the sample dimensions. Here, through a study of electrical and thermal transport in antimony (Sb) crystals of various sizes, we document the emergence of a two-component fluid of electrons and phonons. Lattice thermal conductivity is dominated by electron scattering down to 0.1 K and displays prominent quantum oscillations. The Dingle mobility does not vary despite an order-of-magnitude change in transport mobility. The Bloch-Grüneisen behavior of electrical resistivity is suddenly aborted below 15 K and replaced by a quadratic temperature dependence. At the Kelvin temperature range, the phonon scattering time and the electron-electron scattering time display a similar amplitude and temperature dependence. Taken together, the results draw a consistent picture of a bifluid where frequent momentum-conserving collisions between electrons and phonons dominate the transport properties.
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spelling doaj.art-897c0bfdf0b0426da5be673840e7335e2022-12-22T04:00:25ZengAmerican Physical SocietyPhysical Review X2160-33082022-08-0112303102310.1103/PhysRevX.12.031023Formation of an Electron-Phonon Bifluid in Bulk AntimonyAlexandre JaouiAdrien GourgoutGabriel SeyfarthAlaska SubediThomas LorenzBenoît FauquéKamran BehniaThe flow of charge and entropy in solids usually depends on collisions decaying quasiparticle momentum. Hydrodynamic corrections can emerge, however, if most collisions among quasiparticles conserve momentum and the mean-free path approaches the sample dimensions. Here, through a study of electrical and thermal transport in antimony (Sb) crystals of various sizes, we document the emergence of a two-component fluid of electrons and phonons. Lattice thermal conductivity is dominated by electron scattering down to 0.1 K and displays prominent quantum oscillations. The Dingle mobility does not vary despite an order-of-magnitude change in transport mobility. The Bloch-Grüneisen behavior of electrical resistivity is suddenly aborted below 15 K and replaced by a quadratic temperature dependence. At the Kelvin temperature range, the phonon scattering time and the electron-electron scattering time display a similar amplitude and temperature dependence. Taken together, the results draw a consistent picture of a bifluid where frequent momentum-conserving collisions between electrons and phonons dominate the transport properties.http://doi.org/10.1103/PhysRevX.12.031023
spellingShingle Alexandre Jaoui
Adrien Gourgout
Gabriel Seyfarth
Alaska Subedi
Thomas Lorenz
Benoît Fauqué
Kamran Behnia
Formation of an Electron-Phonon Bifluid in Bulk Antimony
Physical Review X
title Formation of an Electron-Phonon Bifluid in Bulk Antimony
title_full Formation of an Electron-Phonon Bifluid in Bulk Antimony
title_fullStr Formation of an Electron-Phonon Bifluid in Bulk Antimony
title_full_unstemmed Formation of an Electron-Phonon Bifluid in Bulk Antimony
title_short Formation of an Electron-Phonon Bifluid in Bulk Antimony
title_sort formation of an electron phonon bifluid in bulk antimony
url http://doi.org/10.1103/PhysRevX.12.031023
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