Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL

The development of efficient and reliable sensors operating at room temperature is essential to advance the application of terahertz (THz) science and technology. Pyroelectric THz detectors are among the best candidates, taking into account their variety, outstanding performance, ease of fabrication...

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Main Authors: Anatoly R. Melnikov, Evgeny V. Kalneus, Yaroslav V. Getmanov, Darya A. Shevchenko, Vasily V. Gerasimov, Oleg A. Anisimov, Matvey V. Fedin, Sergey L. Veber
Format: Article
Language:English
Published: MDPI AG 2023-10-01
Series:Polymers
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Online Access:https://www.mdpi.com/2073-4360/15/20/4124
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author Anatoly R. Melnikov
Evgeny V. Kalneus
Yaroslav V. Getmanov
Darya A. Shevchenko
Vasily V. Gerasimov
Oleg A. Anisimov
Matvey V. Fedin
Sergey L. Veber
author_facet Anatoly R. Melnikov
Evgeny V. Kalneus
Yaroslav V. Getmanov
Darya A. Shevchenko
Vasily V. Gerasimov
Oleg A. Anisimov
Matvey V. Fedin
Sergey L. Veber
author_sort Anatoly R. Melnikov
collection DOAJ
description The development of efficient and reliable sensors operating at room temperature is essential to advance the application of terahertz (THz) science and technology. Pyroelectric THz detectors are among the best candidates, taking into account their variety, outstanding performance, ease of fabrication, and robustness. In this work, we compare the performance of six different detectors, based on either LaTiO<sub>3</sub> crystal or different polymeric films, using monochromatic radiation of the Novosibirsk Free Electron Laser facility (NovoFEL) in the frequency range of 0.9–2.0 THz. The main characteristics, including noise equivalent power and frequency response, were determined for all of them. Possible reasons for the differences in the obtained characteristics are discussed on the basis of the main physicochemical characteristics and optical properties of the sensitive area. At least three detectors showed sufficient sensitivity to monitor the shape and duration of the THz macropulses utilizing only a small fraction of the THz radiation from the primary beam. This capability is crucial for accurate characterization of THz radiation during the main experiment at various specialized endstations at synchrotrons and free electron lasers. As an example of such characterization, the typical stability of the average NovoFEL radiation power at the beamline of the electron paramagnetic resonance endstation was investigated.
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spelling doaj.art-899ce8c1b2164b81817e96bb7d0788e42023-11-19T17:51:33ZengMDPI AGPolymers2073-43602023-10-011520412410.3390/polym15204124Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFELAnatoly R. Melnikov0Evgeny V. Kalneus1Yaroslav V. Getmanov2Darya A. Shevchenko3Vasily V. Gerasimov4Oleg A. Anisimov5Matvey V. Fedin6Sergey L. Veber7International Tomography Center, Siberian Branch of the Russian Academy of Sciences, 3a, Institutskaya Str., 630090 Novosibirsk, RussiaNovosibirsk State University, 1, Pirogova Str., 630090 Novosibirsk, RussiaNovosibirsk State University, 1, Pirogova Str., 630090 Novosibirsk, RussiaBudker Institute of Nuclear Physics, Siberian Branch of the Russian Academy of Sciences, 11, Acad. Lavrentieva Ave., 630090 Novosibirsk, RussiaNovosibirsk State University, 1, Pirogova Str., 630090 Novosibirsk, RussiaVoevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Sciences, 3, Institutskaya Str., 630090 Novosibirsk, RussiaInternational Tomography Center, Siberian Branch of the Russian Academy of Sciences, 3a, Institutskaya Str., 630090 Novosibirsk, RussiaInternational Tomography Center, Siberian Branch of the Russian Academy of Sciences, 3a, Institutskaya Str., 630090 Novosibirsk, RussiaThe development of efficient and reliable sensors operating at room temperature is essential to advance the application of terahertz (THz) science and technology. Pyroelectric THz detectors are among the best candidates, taking into account their variety, outstanding performance, ease of fabrication, and robustness. In this work, we compare the performance of six different detectors, based on either LaTiO<sub>3</sub> crystal or different polymeric films, using monochromatic radiation of the Novosibirsk Free Electron Laser facility (NovoFEL) in the frequency range of 0.9–2.0 THz. The main characteristics, including noise equivalent power and frequency response, were determined for all of them. Possible reasons for the differences in the obtained characteristics are discussed on the basis of the main physicochemical characteristics and optical properties of the sensitive area. At least three detectors showed sufficient sensitivity to monitor the shape and duration of the THz macropulses utilizing only a small fraction of the THz radiation from the primary beam. This capability is crucial for accurate characterization of THz radiation during the main experiment at various specialized endstations at synchrotrons and free electron lasers. As an example of such characterization, the typical stability of the average NovoFEL radiation power at the beamline of the electron paramagnetic resonance endstation was investigated.https://www.mdpi.com/2073-4360/15/20/4124THz radiationpyroelectric detectorpolyvinylidene difluoridelithium tantalitetetra-aminodiphenylnoise equivalent power
spellingShingle Anatoly R. Melnikov
Evgeny V. Kalneus
Yaroslav V. Getmanov
Darya A. Shevchenko
Vasily V. Gerasimov
Oleg A. Anisimov
Matvey V. Fedin
Sergey L. Veber
Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
Polymers
THz radiation
pyroelectric detector
polyvinylidene difluoride
lithium tantalite
tetra-aminodiphenyl
noise equivalent power
title Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
title_full Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
title_fullStr Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
title_full_unstemmed Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
title_short Comparative Study of Single Crystal and Polymeric Pyroelectric Detectors in the 0.9–2.0 THz Range Using Monochromatic Laser Radiation of the NovoFEL
title_sort comparative study of single crystal and polymeric pyroelectric detectors in the 0 9 2 0 thz range using monochromatic laser radiation of the novofel
topic THz radiation
pyroelectric detector
polyvinylidene difluoride
lithium tantalite
tetra-aminodiphenyl
noise equivalent power
url https://www.mdpi.com/2073-4360/15/20/4124
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