Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures
We present a multimer coupling classic harmonic oscillator model to reveal the scattering and photoluminescence (PL) properties of metallic nanoparticle chains. Taking particle number from 1 to 6 as examples, we compare the calculated spectra with the experimental ones from other researchers’ work,...
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Format: | Article |
Language: | English |
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Elsevier
2022-07-01
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Series: | Results in Physics |
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Online Access: | http://www.sciencedirect.com/science/article/pii/S2211379722003655 |
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author | Yuqing Cheng Yi Wang Mengtao Sun |
author_facet | Yuqing Cheng Yi Wang Mengtao Sun |
author_sort | Yuqing Cheng |
collection | DOAJ |
description | We present a multimer coupling classic harmonic oscillator model to reveal the scattering and photoluminescence (PL) properties of metallic nanoparticle chains. Taking particle number from 1 to 6 as examples, we compare the calculated spectra with the experimental ones from other researchers’ work, and they agree well with each other. Furthermore, scattering and PL properties are analyzed carefully varying with particle number n, coupling strength g, and effective free electron number N. Results indicates larger red-shift and smaller full width at half maximum (FWHM) of the scattering spectra with larger n or/and larger g. Particularly, the limitation of the red-shift is obtained in the limit of n→∞. Meanwhile, the splitting of PL modes increases as g increases, and the amplitudes are dependent on the excitation wavelength. This classic model is simple and shows a unified treatment for understanding the scattering and PL properties of multimer coupled systems. |
first_indexed | 2024-04-12T15:57:19Z |
format | Article |
id | doaj.art-8a308b6e4af84251a7e6228c35ac15f7 |
institution | Directory Open Access Journal |
issn | 2211-3797 |
language | English |
last_indexed | 2024-04-12T15:57:19Z |
publishDate | 2022-07-01 |
publisher | Elsevier |
record_format | Article |
series | Results in Physics |
spelling | doaj.art-8a308b6e4af84251a7e6228c35ac15f72022-12-22T03:26:20ZengElsevierResults in Physics2211-37972022-07-0138105668Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructuresYuqing Cheng0Yi Wang1Mengtao Sun2School of Mathematics and Physics, Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, ChinaSchool of Mathematics and Physics, Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, ChinaCorresponding author.; School of Mathematics and Physics, Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, ChinaWe present a multimer coupling classic harmonic oscillator model to reveal the scattering and photoluminescence (PL) properties of metallic nanoparticle chains. Taking particle number from 1 to 6 as examples, we compare the calculated spectra with the experimental ones from other researchers’ work, and they agree well with each other. Furthermore, scattering and PL properties are analyzed carefully varying with particle number n, coupling strength g, and effective free electron number N. Results indicates larger red-shift and smaller full width at half maximum (FWHM) of the scattering spectra with larger n or/and larger g. Particularly, the limitation of the red-shift is obtained in the limit of n→∞. Meanwhile, the splitting of PL modes increases as g increases, and the amplitudes are dependent on the excitation wavelength. This classic model is simple and shows a unified treatment for understanding the scattering and PL properties of multimer coupled systems.http://www.sciencedirect.com/science/article/pii/S2211379722003655Unified treatmentPhotoluminescenceScatteringCoupled metallic multi-nanostructure |
spellingShingle | Yuqing Cheng Yi Wang Mengtao Sun Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures Results in Physics Unified treatment Photoluminescence Scattering Coupled metallic multi-nanostructure |
title | Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures |
title_full | Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures |
title_fullStr | Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures |
title_full_unstemmed | Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures |
title_short | Unified treatment for photoluminescence and scattering of coupled metallic multi-nanostructures |
title_sort | unified treatment for photoluminescence and scattering of coupled metallic multi nanostructures |
topic | Unified treatment Photoluminescence Scattering Coupled metallic multi-nanostructure |
url | http://www.sciencedirect.com/science/article/pii/S2211379722003655 |
work_keys_str_mv | AT yuqingcheng unifiedtreatmentforphotoluminescenceandscatteringofcoupledmetallicmultinanostructures AT yiwang unifiedtreatmentforphotoluminescenceandscatteringofcoupledmetallicmultinanostructures AT mengtaosun unifiedtreatmentforphotoluminescenceandscatteringofcoupledmetallicmultinanostructures |