Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}

Three-dimensional, commensurate long-range magnetic order in La_{2}CuO_{4} quickly evolves to quasi-two-dimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La_{2−x}Sr_{x}/Ba_{x}CuO_{4} family of superconductors. The onse...

Full description

Bibliographic Details
Main Authors: Qianli Ma, Kirrily C. Rule, Zachary W. Cronkwright, Mirela Dragomir, Gabrielle Mitchell, Evan M. Smith, Songxue Chi, Alexander I. Kolesnikov, Matthew B. Stone, Bruce D. Gaulin
Format: Article
Language:English
Published: American Physical Society 2021-05-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.3.023151
_version_ 1797211003346223104
author Qianli Ma
Kirrily C. Rule
Zachary W. Cronkwright
Mirela Dragomir
Gabrielle Mitchell
Evan M. Smith
Songxue Chi
Alexander I. Kolesnikov
Matthew B. Stone
Bruce D. Gaulin
author_facet Qianli Ma
Kirrily C. Rule
Zachary W. Cronkwright
Mirela Dragomir
Gabrielle Mitchell
Evan M. Smith
Songxue Chi
Alexander I. Kolesnikov
Matthew B. Stone
Bruce D. Gaulin
author_sort Qianli Ma
collection DOAJ
description Three-dimensional, commensurate long-range magnetic order in La_{2}CuO_{4} quickly evolves to quasi-two-dimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La_{2−x}Sr_{x}/Ba_{x}CuO_{4} family of superconductors. The onset of superconductivity in these systems is known to be coincident with a remarkable rotation of the incommensurate spin order from “diagonal stripes” below x = 0.05 to “parallel stripes” above. However, little is known about the spin correlations at optimal and high doping levels, around and beyond the proposed quantum critical point for the pseudogap phase, p^{*}. Here, we present elastic and inelastic neutron scattering measurements on single crystals of La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4} with x = 0.125, 0.19, 0.24, and 0.26 and show that two-dimensional, quasistatic, parallel spin stripes have an onset at temperatures such that the parallel spin stripe phase extends beyond p^{*} and envelops the entirety of superconducting ground states in this system. We also show that the elastic order parameter for parallel spin stripes at optimum doping, x = 0.19, displays an inflection point at superconducting T_{c}, while the low-energy dynamic spectral weight of parallel stripe fluctuations grows with decreasing temperature and saturates below T_{c}.
first_indexed 2024-04-24T10:19:35Z
format Article
id doaj.art-8a3ac1056ec74c3dbf58f5bb54210462
institution Directory Open Access Journal
issn 2643-1564
language English
last_indexed 2024-04-24T10:19:35Z
publishDate 2021-05-01
publisher American Physical Society
record_format Article
series Physical Review Research
spelling doaj.art-8a3ac1056ec74c3dbf58f5bb542104622024-04-12T17:10:12ZengAmerican Physical SocietyPhysical Review Research2643-15642021-05-013202315110.1103/PhysRevResearch.3.023151Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}Qianli MaKirrily C. RuleZachary W. CronkwrightMirela DragomirGabrielle MitchellEvan M. SmithSongxue ChiAlexander I. KolesnikovMatthew B. StoneBruce D. GaulinThree-dimensional, commensurate long-range magnetic order in La_{2}CuO_{4} quickly evolves to quasi-two-dimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La_{2−x}Sr_{x}/Ba_{x}CuO_{4} family of superconductors. The onset of superconductivity in these systems is known to be coincident with a remarkable rotation of the incommensurate spin order from “diagonal stripes” below x = 0.05 to “parallel stripes” above. However, little is known about the spin correlations at optimal and high doping levels, around and beyond the proposed quantum critical point for the pseudogap phase, p^{*}. Here, we present elastic and inelastic neutron scattering measurements on single crystals of La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4} with x = 0.125, 0.19, 0.24, and 0.26 and show that two-dimensional, quasistatic, parallel spin stripes have an onset at temperatures such that the parallel spin stripe phase extends beyond p^{*} and envelops the entirety of superconducting ground states in this system. We also show that the elastic order parameter for parallel spin stripes at optimum doping, x = 0.19, displays an inflection point at superconducting T_{c}, while the low-energy dynamic spectral weight of parallel stripe fluctuations grows with decreasing temperature and saturates below T_{c}.http://doi.org/10.1103/PhysRevResearch.3.023151
spellingShingle Qianli Ma
Kirrily C. Rule
Zachary W. Cronkwright
Mirela Dragomir
Gabrielle Mitchell
Evan M. Smith
Songxue Chi
Alexander I. Kolesnikov
Matthew B. Stone
Bruce D. Gaulin
Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
Physical Review Research
title Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
title_full Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
title_fullStr Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
title_full_unstemmed Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
title_short Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La_{1.6−x}Nd_{0.4}Sr_{x}CuO_{4}
title_sort parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in la 1 6 x nd 0 4 sr x cuo 4
url http://doi.org/10.1103/PhysRevResearch.3.023151
work_keys_str_mv AT qianlima parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT kirrilycrule parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT zacharywcronkwright parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT mireladragomir parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT gabriellemitchell parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT evanmsmith parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT songxuechi parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT alexanderikolesnikov parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT matthewbstone parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4
AT brucedgaulin parallelspinstripesandtheircoexistencewithsuperconductinggroundstatesatoptimalandhighdopinginla16xnd04srxcuo4