Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers

Perovskite quantum dots (QDs) have showed excellent optoelectronic properties to extend the application range of novel solid-state lighting, such as perovskite QD based LEDs (QD-LEDs). However, the traditional device structure of perovskite QD-LEDs employed PEDOT:PSS as a hole inject layer (HIL), wh...

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Main Authors: Pao-Hsun Huang, Sih-An Chen, Li-Wei Chao, Jia-Xun Xie, Ching-Yu Liao, Zong-Liang Tseng, Sheng-Hui Chen
Format: Article
Language:English
Published: MDPI AG 2023-09-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/16/17/6060
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author Pao-Hsun Huang
Sih-An Chen
Li-Wei Chao
Jia-Xun Xie
Ching-Yu Liao
Zong-Liang Tseng
Sheng-Hui Chen
author_facet Pao-Hsun Huang
Sih-An Chen
Li-Wei Chao
Jia-Xun Xie
Ching-Yu Liao
Zong-Liang Tseng
Sheng-Hui Chen
author_sort Pao-Hsun Huang
collection DOAJ
description Perovskite quantum dots (QDs) have showed excellent optoelectronic properties to extend the application range of novel solid-state lighting, such as perovskite QD based LEDs (QD-LEDs). However, the traditional device structure of perovskite QD-LEDs employed PEDOT:PSS as a hole inject layer (HIL), which impairs stability due to acidic surface characteristics. This study proposes the sputtered NiO films as an HIL to replace acidic PEDOT:PSS. The NiO films with significantly different characteristics were prepared by controlling the sputtering parameters to investigate the devices’ performance of NiO-based CsPbBr<sub>3</sub> QD-LEDs. The optimized device showed an excellent performance with maxima luminescence of 20,118 cd/m<sup>2</sup> and an external quantum efficiency (EQE) up to 3.63%.
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spelling doaj.art-8c6ddd68b1d8439ba8b7cf75e5a403e02023-11-19T08:29:42ZengMDPI AGMaterials1996-19442023-09-011617606010.3390/ma16176060Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection LayersPao-Hsun Huang0Sih-An Chen1Li-Wei Chao2Jia-Xun Xie3Ching-Yu Liao4Zong-Liang Tseng5Sheng-Hui Chen6School of Ocean Information Engineering, Jimei University, Jimei District, Xiamen 361021, ChinaOrganic Electronics Research Center, Ming Chi University of Technology, No. 84, Gungjuan Rd., New Taipei City 24301, TaiwanOrganic Electronics Research Center, Ming Chi University of Technology, No. 84, Gungjuan Rd., New Taipei City 24301, TaiwanOrganic Electronics Research Center, Ming Chi University of Technology, No. 84, Gungjuan Rd., New Taipei City 24301, TaiwanOrganic Electronics Research Center, Ming Chi University of Technology, No. 84, Gungjuan Rd., New Taipei City 24301, TaiwanOrganic Electronics Research Center, Ming Chi University of Technology, No. 84, Gungjuan Rd., New Taipei City 24301, TaiwanDepartment of Optics and Photonics, National Central University, Taoyuan 320317, TaiwanPerovskite quantum dots (QDs) have showed excellent optoelectronic properties to extend the application range of novel solid-state lighting, such as perovskite QD based LEDs (QD-LEDs). However, the traditional device structure of perovskite QD-LEDs employed PEDOT:PSS as a hole inject layer (HIL), which impairs stability due to acidic surface characteristics. This study proposes the sputtered NiO films as an HIL to replace acidic PEDOT:PSS. The NiO films with significantly different characteristics were prepared by controlling the sputtering parameters to investigate the devices’ performance of NiO-based CsPbBr<sub>3</sub> QD-LEDs. The optimized device showed an excellent performance with maxima luminescence of 20,118 cd/m<sup>2</sup> and an external quantum efficiency (EQE) up to 3.63%.https://www.mdpi.com/1996-1944/16/17/6060CsPbBr<sub>3</sub> quantum dotlight-emitting diodeNiOsputter
spellingShingle Pao-Hsun Huang
Sih-An Chen
Li-Wei Chao
Jia-Xun Xie
Ching-Yu Liao
Zong-Liang Tseng
Sheng-Hui Chen
Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
Materials
CsPbBr<sub>3</sub> quantum dot
light-emitting diode
NiO
sputter
title Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
title_full Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
title_fullStr Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
title_full_unstemmed Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
title_short Efficient CsPbBr<sub>3</sub> Quantum-Dot Light-Emitting Diodes Using Sputtered NiO Films as Hole Injection Layers
title_sort efficient cspbbr sub 3 sub quantum dot light emitting diodes using sputtered nio films as hole injection layers
topic CsPbBr<sub>3</sub> quantum dot
light-emitting diode
NiO
sputter
url https://www.mdpi.com/1996-1944/16/17/6060
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