Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)

We investigate the shape of monatomic high Cu islands on a Cu(111) surface by variable-temperature scanning tunneling microscopy between 110 K and 240 K. Low temperature dendrites evolve towards more compact shapes at increasing temperature; finally reaching the equilibrium shape of a hexagon with r...

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Main Authors: C Sprodowski, K Morgenstern
Format: Article
Language:English
Published: IOP Publishing 2020-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ab944b
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author C Sprodowski
K Morgenstern
author_facet C Sprodowski
K Morgenstern
author_sort C Sprodowski
collection DOAJ
description We investigate the shape of monatomic high Cu islands on a Cu(111) surface by variable-temperature scanning tunneling microscopy between 110 K and 240 K. Low temperature dendrites evolve towards more compact shapes at increasing temperature; finally reaching the equilibrium shape of a hexagon with rounded corners. Time-lapsed imaging at increasing temperature reveals the onset of shape change to be at ≈170 K, corresponding to the onset of edge and corner diffusion of atoms along the island’s borders. Despite a substantial variation for individual islands at each temperature, the mean fractal dimension increases monotonously between 170 K up to 240 K, from the smallest to the largest values feasible for islands grown on surfaces.
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spelling doaj.art-8d0f359b4f2d4d158f4c13c9ae79d81a2023-08-08T15:31:54ZengIOP PublishingNew Journal of Physics1367-26302020-01-0122606305510.1088/1367-2630/ab944bTemperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)C Sprodowski0K Morgenstern1Institut für Festkörperphysik, Leibniz Universität Hannover , Appelstr. 2, D-30167 Hannover, GermanyRuhr-Universität Bochum , Lehrstuhl für physikalische Chemie I, Universitätsstr. 150, D-44801 Bochum, GermanyWe investigate the shape of monatomic high Cu islands on a Cu(111) surface by variable-temperature scanning tunneling microscopy between 110 K and 240 K. Low temperature dendrites evolve towards more compact shapes at increasing temperature; finally reaching the equilibrium shape of a hexagon with rounded corners. Time-lapsed imaging at increasing temperature reveals the onset of shape change to be at ≈170 K, corresponding to the onset of edge and corner diffusion of atoms along the island’s borders. Despite a substantial variation for individual islands at each temperature, the mean fractal dimension increases monotonously between 170 K up to 240 K, from the smallest to the largest values feasible for islands grown on surfaces.https://doi.org/10.1088/1367-2630/ab944bfractal dimensiontime-lapsed STMshape evolution
spellingShingle C Sprodowski
K Morgenstern
Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
New Journal of Physics
fractal dimension
time-lapsed STM
shape evolution
title Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
title_full Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
title_fullStr Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
title_full_unstemmed Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
title_short Temperature-dependent change of the fractal dimension of Cu dendrites on Cu(111)
title_sort temperature dependent change of the fractal dimension of cu dendrites on cu 111
topic fractal dimension
time-lapsed STM
shape evolution
url https://doi.org/10.1088/1367-2630/ab944b
work_keys_str_mv AT csprodowski temperaturedependentchangeofthefractaldimensionofcudendritesoncu111
AT kmorgenstern temperaturedependentchangeofthefractaldimensionofcudendritesoncu111