Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures

Piezoelectric composites with 3-3 connectivity gathered attraction due to their potential application as an acoustic transducer in medical imaging, non-destructive testing, etc. In this contribution, piezoelectric composites were fabricated with a material extrusion-based additive manufacturing proc...

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Main Authors: Tutu Sebastian, Miriam Bach, Andreas Geiger, Tony Lusiola, Lucjan Kozielski, Frank Clemens
Format: Article
Language:English
Published: MDPI AG 2021-10-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/14/20/5927
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author Tutu Sebastian
Miriam Bach
Andreas Geiger
Tony Lusiola
Lucjan Kozielski
Frank Clemens
author_facet Tutu Sebastian
Miriam Bach
Andreas Geiger
Tony Lusiola
Lucjan Kozielski
Frank Clemens
author_sort Tutu Sebastian
collection DOAJ
description Piezoelectric composites with 3-3 connectivity gathered attraction due to their potential application as an acoustic transducer in medical imaging, non-destructive testing, etc. In this contribution, piezoelectric composites were fabricated with a material extrusion-based additive manufacturing process (MEX), also well-known under the names fused deposition modeling (FDM), fused filament fabrication (FFF) or fused deposition ceramics (FDC). Thermoplastic filaments were used to achieve open and offset printed piezoelectric scaffold structures. Both scaffold structures were printed, debinded and sintered successfully using commercial PZT and BaTiO<sub>3</sub> powder. For the first time, it could be demonstrated, that using the MEX processing method, closed pore ferroelectric structure can be achieved without pore-former additive. After ceramic processing, the PZT scaffold structures were impregnated with epoxy resin to convert them into composites with 3-3 connectivity. A series of composites with varying ceramic content were achieved by changing the infill parameter during the 3D printing process systematically, and their electromechanical properties were investigated using the electromechanical aix PES device. Also, the Figure of merit (FOM) of these composites was calculated to assess the potential of this material as a candidate for transducer applications. A maximum for the FOM at 25 vol.% of PZT could be observed in this study.
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spelling doaj.art-8d8e7e324a7a4657a960f2ef3b6382a62023-11-22T18:56:07ZengMDPI AGMaterials1996-19442021-10-011420592710.3390/ma14205927Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold StructuresTutu Sebastian0Miriam Bach1Andreas Geiger2Tony Lusiola3Lucjan Kozielski4Frank Clemens5Laboratory for High Performance Ceramics, Empa, Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, SwitzerlandLaboratory for High Performance Ceramics, Empa, Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, SwitzerlandLaboratory for High Performance Ceramics, Empa, Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, SwitzerlandLaboratory for High Performance Ceramics, Empa, Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, SwitzerlandFaculty of Science and Technology, University of Silesia, 1A 75 Pułku Piechoty St., 41-500 Chorzów, PolandLaboratory for High Performance Ceramics, Empa, Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, SwitzerlandPiezoelectric composites with 3-3 connectivity gathered attraction due to their potential application as an acoustic transducer in medical imaging, non-destructive testing, etc. In this contribution, piezoelectric composites were fabricated with a material extrusion-based additive manufacturing process (MEX), also well-known under the names fused deposition modeling (FDM), fused filament fabrication (FFF) or fused deposition ceramics (FDC). Thermoplastic filaments were used to achieve open and offset printed piezoelectric scaffold structures. Both scaffold structures were printed, debinded and sintered successfully using commercial PZT and BaTiO<sub>3</sub> powder. For the first time, it could be demonstrated, that using the MEX processing method, closed pore ferroelectric structure can be achieved without pore-former additive. After ceramic processing, the PZT scaffold structures were impregnated with epoxy resin to convert them into composites with 3-3 connectivity. A series of composites with varying ceramic content were achieved by changing the infill parameter during the 3D printing process systematically, and their electromechanical properties were investigated using the electromechanical aix PES device. Also, the Figure of merit (FOM) of these composites was calculated to assess the potential of this material as a candidate for transducer applications. A maximum for the FOM at 25 vol.% of PZT could be observed in this study.https://www.mdpi.com/1996-1944/14/20/5927material extrusion-based additive manufacturing (MEX)fused deposition modeling (FDM)fused filament fabrication (FFF)thermoplastic processingPZTBaTiO<sub>3</sub>
spellingShingle Tutu Sebastian
Miriam Bach
Andreas Geiger
Tony Lusiola
Lucjan Kozielski
Frank Clemens
Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
Materials
material extrusion-based additive manufacturing (MEX)
fused deposition modeling (FDM)
fused filament fabrication (FFF)
thermoplastic processing
PZT
BaTiO<sub>3</sub>
title Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
title_full Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
title_fullStr Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
title_full_unstemmed Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
title_short Investigation of Electromechanical Properties on 3-D Printed Piezoelectric Composite Scaffold Structures
title_sort investigation of electromechanical properties on 3 d printed piezoelectric composite scaffold structures
topic material extrusion-based additive manufacturing (MEX)
fused deposition modeling (FDM)
fused filament fabrication (FFF)
thermoplastic processing
PZT
BaTiO<sub>3</sub>
url https://www.mdpi.com/1996-1944/14/20/5927
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