Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses

For both the B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO and B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass systems, <i>γ</i>-ray and neutron attenuation quali...

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Main Authors: Gandham Lakshminarayana, Youssef Elmahroug, Ashok Kumar, Huseyin Ozan Tekin, Najeh Rekik, Mengge Dong, Dong-Eun Lee, Jonghun Yoon, Taejoon Park
Format: Article
Language:English
Published: MDPI AG 2021-04-01
Series:Materials
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Online Access:https://www.mdpi.com/1996-1944/14/9/2265
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author Gandham Lakshminarayana
Youssef Elmahroug
Ashok Kumar
Huseyin Ozan Tekin
Najeh Rekik
Mengge Dong
Dong-Eun Lee
Jonghun Yoon
Taejoon Park
author_facet Gandham Lakshminarayana
Youssef Elmahroug
Ashok Kumar
Huseyin Ozan Tekin
Najeh Rekik
Mengge Dong
Dong-Eun Lee
Jonghun Yoon
Taejoon Park
author_sort Gandham Lakshminarayana
collection DOAJ
description For both the B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO and B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass systems, <i>γ</i>-ray and neutron attenuation qualities were evaluated. Utilizing the Phy-X/PSD program, within the 0.015–15 MeV energy range, linear attenuation coefficients (µ) and mass attenuation coefficients (μ/ρ) were calculated, and the attained μ/ρ quantities match well with respective simulation results computed by MCNPX, Geant4, and Penelope codes. Instead of B<sub>2</sub>O<sub>3</sub>/CaO or B<sub>2</sub>O<sub>3</sub>/SrO, the Bi<sub>2</sub>O<sub>3</sub> addition causes improved <i>γ</i>-ray shielding competence, i.e., rise in effective atomic number (<i>Z<sub>eff</sub></i>) and a fall in half-value layer (HVL), tenth-value layer (TVL), and mean free path (MFP). Exposure buildup factors (EBFs) and energy absorption buildup factors (EABFs) were derived using a geometric progression (G–P) fitting approach at 1–40 mfp penetration depths (PDs), within the 0.015–15 MeV range. Computed radiation protection efficiency (RPE) values confirm their excellent capacity for lower energy photons shielding. Comparably greater density (7.59 g/cm<sup>3</sup>), larger μ, μ/ρ, <i>Z<sub>eff</sub></i>, equivalent atomic number (<i>Z<sub>eq</sub></i>), and RPE, with the lowest HVL, TVL, MFP, EBFs, and EABFs derived for 30B<sub>2</sub>O<sub>3</sub>-60Bi<sub>2</sub>O<sub>3</sub>-10SrO (mol%) glass suggest it as an excellent <i>γ</i>-ray attenuator. Additionally, 30B<sub>2</sub>O<sub>3</sub>-60Bi<sub>2</sub>O<sub>3</sub>-10SrO (mol%) glass holds a commensurably bigger macroscopic removal cross-section for fast neutrons (<i>Σ<sub>R</sub></i>) (=0.1199 cm<sup>−1</sup>), obtained by applying Phy-X/PSD for fast neutrons shielding, owing to the presence of larger wt% of ‘Bi’ (80.6813 wt%) and moderate ‘B’ (2.0869 wt%) elements in it. 70B<sub>2</sub>O<sub>3</sub>-5Bi<sub>2</sub>O<sub>3</sub>-25CaO (mol%) sample (B: 17.5887 wt%, Bi: 24.2855 wt%, Ca: 11.6436 wt%, and O: 46.4821 wt%) shows high potentiality for thermal or slow neutrons and intermediate energy neutrons capture or absorption due to comprised high wt% of ‘B’ element in it.
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spelling doaj.art-8ea1442613e34b9fac1979d0182bcd522023-11-21T17:25:48ZengMDPI AGMaterials1996-19442021-04-01149226510.3390/ma14092265Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate GlassesGandham Lakshminarayana0Youssef Elmahroug1Ashok Kumar2Huseyin Ozan Tekin3Najeh Rekik4Mengge Dong5Dong-Eun Lee6Jonghun Yoon7Taejoon Park8Intelligent Construction Automation Center, Kyungpook National University, 80 Daehak-ro, Buk-gu, Daegu 41566, KoreaUnité de Recherche de Physique Nucléaire et des Hautes Energies, Faculté des Sciences de Tunis, Université de Tunis El Manar, Tunis 2092, TunisiaDepartment of Physics, University College, Benra-Dhuri, Punjab 148024, IndiaMedical Diagnostic Imaging Department, College of Health Sciences, University of Sharjah, Sharjah 27272, United Arab EmiratesPhysics Department, Faculty of Science, University of Ha’il, Ha’il 81451, Saudi ArabiaDepartment of Resource and Environment, Northeastern University, Shenyang 110819, ChinaSchool of Architecture, Civil, Environment and Energy, Kyungpook National University, 1370 Sangyeok-dong, Buk-gu, DaeGu 702-701, KoreaDepartment of Mechanical Engineering, Hanyang University, 55 Hanyangdaehak-ro, Ansan 15588, Gyeonggi-do, KoreaDepartment of Robotics Engineering, Hanyang University, 55 Hanyangdaehak-ro, Ansan 15588, Gyeonggi-do, KoreaFor both the B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO and B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass systems, <i>γ</i>-ray and neutron attenuation qualities were evaluated. Utilizing the Phy-X/PSD program, within the 0.015–15 MeV energy range, linear attenuation coefficients (µ) and mass attenuation coefficients (μ/ρ) were calculated, and the attained μ/ρ quantities match well with respective simulation results computed by MCNPX, Geant4, and Penelope codes. Instead of B<sub>2</sub>O<sub>3</sub>/CaO or B<sub>2</sub>O<sub>3</sub>/SrO, the Bi<sub>2</sub>O<sub>3</sub> addition causes improved <i>γ</i>-ray shielding competence, i.e., rise in effective atomic number (<i>Z<sub>eff</sub></i>) and a fall in half-value layer (HVL), tenth-value layer (TVL), and mean free path (MFP). Exposure buildup factors (EBFs) and energy absorption buildup factors (EABFs) were derived using a geometric progression (G–P) fitting approach at 1–40 mfp penetration depths (PDs), within the 0.015–15 MeV range. Computed radiation protection efficiency (RPE) values confirm their excellent capacity for lower energy photons shielding. Comparably greater density (7.59 g/cm<sup>3</sup>), larger μ, μ/ρ, <i>Z<sub>eff</sub></i>, equivalent atomic number (<i>Z<sub>eq</sub></i>), and RPE, with the lowest HVL, TVL, MFP, EBFs, and EABFs derived for 30B<sub>2</sub>O<sub>3</sub>-60Bi<sub>2</sub>O<sub>3</sub>-10SrO (mol%) glass suggest it as an excellent <i>γ</i>-ray attenuator. Additionally, 30B<sub>2</sub>O<sub>3</sub>-60Bi<sub>2</sub>O<sub>3</sub>-10SrO (mol%) glass holds a commensurably bigger macroscopic removal cross-section for fast neutrons (<i>Σ<sub>R</sub></i>) (=0.1199 cm<sup>−1</sup>), obtained by applying Phy-X/PSD for fast neutrons shielding, owing to the presence of larger wt% of ‘Bi’ (80.6813 wt%) and moderate ‘B’ (2.0869 wt%) elements in it. 70B<sub>2</sub>O<sub>3</sub>-5Bi<sub>2</sub>O<sub>3</sub>-25CaO (mol%) sample (B: 17.5887 wt%, Bi: 24.2855 wt%, Ca: 11.6436 wt%, and O: 46.4821 wt%) shows high potentiality for thermal or slow neutrons and intermediate energy neutrons capture or absorption due to comprised high wt% of ‘B’ element in it.https://www.mdpi.com/1996-1944/14/9/2265B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO glassB<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass<i>γ</i>- and neutron radiationPhy-X/PSD softwarePENELOPE coderadiation protection efficiency
spellingShingle Gandham Lakshminarayana
Youssef Elmahroug
Ashok Kumar
Huseyin Ozan Tekin
Najeh Rekik
Mengge Dong
Dong-Eun Lee
Jonghun Yoon
Taejoon Park
Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
Materials
B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO glass
B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass
<i>γ</i>- and neutron radiation
Phy-X/PSD software
PENELOPE code
radiation protection efficiency
title Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
title_full Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
title_fullStr Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
title_full_unstemmed Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
title_short Detailed Inspection of <i>γ</i>-ray, Fast and Thermal Neutrons Shielding Competence of Calcium Oxide or Strontium Oxide Comprising Bismuth Borate Glasses
title_sort detailed inspection of i γ i ray fast and thermal neutrons shielding competence of calcium oxide or strontium oxide comprising bismuth borate glasses
topic B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-CaO glass
B<sub>2</sub>O<sub>3</sub>-Bi<sub>2</sub>O<sub>3</sub>-SrO glass
<i>γ</i>- and neutron radiation
Phy-X/PSD software
PENELOPE code
radiation protection efficiency
url https://www.mdpi.com/1996-1944/14/9/2265
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