Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics
In this work, two series of BaTiO3-based ceramics, Ba1-xSrxTiO3 (x = 0, 0.2, 0.4, 0.6, 0.8) and BaTi1-xTaxO3 (x = 0.03, 0.06, 0.075, 0.09, 0.1), were synthesized by using standard solid-state reaction method at 1350 °C, and then sintered at 1400 °C for 10 h in air. Frequency-dependent dielectric and...
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University of Novi Sad
2023-09-01
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Series: | Processing and Application of Ceramics |
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Online Access: | https://doiserbia.nb.rs/img/doi/1820-6131/2023/1820-61312303286W.pdf |
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author | Wang Depeng Niu Ruifeng Cui Liqi Wang Weitian |
author_facet | Wang Depeng Niu Ruifeng Cui Liqi Wang Weitian |
author_sort | Wang Depeng |
collection | DOAJ |
description | In this work, two series of BaTiO3-based ceramics, Ba1-xSrxTiO3 (x = 0, 0.2, 0.4, 0.6, 0.8) and BaTi1-xTaxO3 (x = 0.03, 0.06, 0.075, 0.09, 0.1), were synthesized by using standard solid-state reaction method at 1350 °C, and then sintered at 1400 °C for 10 h in air. Frequency-dependent dielectric and impedance properties were investigated at low temperature range of 100-300K. The changes in dielectric properties of the Ba1-xSrxTiO3 ceramics are believed to originate from the phase transition due to the different A-site Sr2+ doping concentration. The local electron-pinned defect-dipole effect is responsible for the enhancement of dielectric constant observed in the B-site Ta5+ doped BaTi1-xTaxO3 ceramics. The complex impedance analysis was used to discern the temperature and frequency dependence of grains and grain boundaries responses. The results suggest that A- and B-site doped BaTiO3 ceramics can be applied for different dielectric devices at low temperatures. |
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issn | 1820-6131 2406-1034 |
language | English |
last_indexed | 2024-03-11T13:44:21Z |
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spelling | doaj.art-8f54879383a74f73b460d7d5e8f061732023-11-02T10:55:25ZengUniversity of Novi SadProcessing and Application of Ceramics1820-61312406-10342023-09-0117328629410.2298/PAC2303286WLow-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramicsWang Depeng0Niu Ruifeng1Cui Liqi 2Wang Weitian3School of Physics and Electronic Information, Yantai University, Yantai, P.R. ChinaSchool of Physics and Electronic Information, Yantai University, Yantai, P.R. ChinaSchool of Physics and Electronic Information, Yantai University, Yantai, P.R. ChinaSchool of Physics and Electronic Information, Yantai University, Yantai, P.R. ChinaIn this work, two series of BaTiO3-based ceramics, Ba1-xSrxTiO3 (x = 0, 0.2, 0.4, 0.6, 0.8) and BaTi1-xTaxO3 (x = 0.03, 0.06, 0.075, 0.09, 0.1), were synthesized by using standard solid-state reaction method at 1350 °C, and then sintered at 1400 °C for 10 h in air. Frequency-dependent dielectric and impedance properties were investigated at low temperature range of 100-300K. The changes in dielectric properties of the Ba1-xSrxTiO3 ceramics are believed to originate from the phase transition due to the different A-site Sr2+ doping concentration. The local electron-pinned defect-dipole effect is responsible for the enhancement of dielectric constant observed in the B-site Ta5+ doped BaTi1-xTaxO3 ceramics. The complex impedance analysis was used to discern the temperature and frequency dependence of grains and grain boundaries responses. The results suggest that A- and B-site doped BaTiO3 ceramics can be applied for different dielectric devices at low temperatures.https://doiserbia.nb.rs/img/doi/1820-6131/2023/1820-61312303286W.pdfperovskitesdopingdielectric propertiesimpedance analysis |
spellingShingle | Wang Depeng Niu Ruifeng Cui Liqi Wang Weitian Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics Processing and Application of Ceramics perovskites doping dielectric properties impedance analysis |
title | Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics |
title_full | Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics |
title_fullStr | Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics |
title_full_unstemmed | Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics |
title_short | Low-temperature dielectric and impedance properties of Ba1-xSrxTiO3 and BaTi1-xTaxO3 ceramics |
title_sort | low temperature dielectric and impedance properties of ba1 xsrxtio3 and bati1 xtaxo3 ceramics |
topic | perovskites doping dielectric properties impedance analysis |
url | https://doiserbia.nb.rs/img/doi/1820-6131/2023/1820-61312303286W.pdf |
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