Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak

Organic milk has a high risk of food fraud as it can easily be adulterated with non-organic milk. This study aimed to identify metabolite markers for assessing the authenticity of organic milk from Jersey and Yak. In the untargeted strategy, ultra-high performance liquid chromatography-Q Exactive HF...

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Main Authors: Min Kang, Hongxia Wang, Chuxin Chen, Ran Suo, Jianfeng Sun, Quanhong Yue, Yaqiong Liu
Format: Article
Language:English
Published: Elsevier 2023-10-01
Series:Food Chemistry: X
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2590157523002298
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author Min Kang
Hongxia Wang
Chuxin Chen
Ran Suo
Jianfeng Sun
Quanhong Yue
Yaqiong Liu
author_facet Min Kang
Hongxia Wang
Chuxin Chen
Ran Suo
Jianfeng Sun
Quanhong Yue
Yaqiong Liu
author_sort Min Kang
collection DOAJ
description Organic milk has a high risk of food fraud as it can easily be adulterated with non-organic milk. This study aimed to identify metabolite markers for assessing the authenticity of organic milk from Jersey and Yak. In the untargeted strategy, ultra-high performance liquid chromatography-Q Exactive HF-X mass spectrometer coupled with chemometrics analysis was used to screen and identify tentative markers of organic milk from Jersey and Yak. In the targeted strategy, a quick and easy method of ultra-performance liquid chromatography–tandem mass spectrometry (UPLC-MS/MS) was developed to quantify three markers. The peptide of Thr-Ala-Val and D-biotin were determined to be metabolite markers for distinguishing organic and non-organic Jersey milk, whereas trimethylamine N-oxide was determined to be a metabolite marker for distinguishing organic and non-organic Yak milk. These findings provide critical information to facilitate assessments of organic milk authenticity.
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spelling doaj.art-90311cb421e84857b2d2979da35a30cf2023-09-23T05:12:16ZengElsevierFood Chemistry: X2590-15752023-10-0119100786Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and YakMin Kang0Hongxia Wang1Chuxin Chen2Ran Suo3Jianfeng Sun4Quanhong Yue5Yaqiong Liu6College of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCollege of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCollege of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCorresponding authors.; College of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCorresponding authors.; College of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCollege of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaCollege of Food Science and Technology, Hebei Agricultural University, 289th Lingyusi Street, Lianchi District, Baoding 071000, ChinaOrganic milk has a high risk of food fraud as it can easily be adulterated with non-organic milk. This study aimed to identify metabolite markers for assessing the authenticity of organic milk from Jersey and Yak. In the untargeted strategy, ultra-high performance liquid chromatography-Q Exactive HF-X mass spectrometer coupled with chemometrics analysis was used to screen and identify tentative markers of organic milk from Jersey and Yak. In the targeted strategy, a quick and easy method of ultra-performance liquid chromatography–tandem mass spectrometry (UPLC-MS/MS) was developed to quantify three markers. The peptide of Thr-Ala-Val and D-biotin were determined to be metabolite markers for distinguishing organic and non-organic Jersey milk, whereas trimethylamine N-oxide was determined to be a metabolite marker for distinguishing organic and non-organic Yak milk. These findings provide critical information to facilitate assessments of organic milk authenticity.http://www.sciencedirect.com/science/article/pii/S2590157523002298AuthenticityJersey milkMetabolomicYak milk
spellingShingle Min Kang
Hongxia Wang
Chuxin Chen
Ran Suo
Jianfeng Sun
Quanhong Yue
Yaqiong Liu
Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
Food Chemistry: X
Authenticity
Jersey milk
Metabolomic
Yak milk
title Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
title_full Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
title_fullStr Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
title_full_unstemmed Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
title_short Analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from Jersey and Yak
title_sort analytical strategies based on untargeted and targeted metabolomics for the accurate authentication of organic milk from jersey and yak
topic Authenticity
Jersey milk
Metabolomic
Yak milk
url http://www.sciencedirect.com/science/article/pii/S2590157523002298
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