Intraseasonal variation of the northeast Asian anomalous anticyclone and its impacts on PM<sub>2.5</sub> pollution in the North China Plain in early winter

<p>The canonical view of the northeast Asian anomalous anticyclone (NAAA) is a crucial factor for determining poor air quality (i.e., higher particulate matter, PM<span class="inline-formula"><sub>2.5</sub></span> concentrations) in the North China Plain (NCP)...

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Bibliographic Details
Main Authors: X. An, W. Chen, P. Hu, S. Chen, L. Sheng
Format: Article
Language:English
Published: Copernicus Publications 2022-05-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/22/6507/2022/acp-22-6507-2022.pdf
Description
Summary:<p>The canonical view of the northeast Asian anomalous anticyclone (NAAA) is a crucial factor for determining poor air quality (i.e., higher particulate matter, PM<span class="inline-formula"><sub>2.5</sub></span> concentrations) in the North China Plain (NCP) on the interannual timescale. However, there is considerable intraseasonal variability in the NAAA in early winter (November–January), and the corresponding mechanism of its impacts on PM<span class="inline-formula"><sub>2.5</sub></span> pollution in the NCP is not well understood. Here, we find that the intraseasonal NAAA usually establishes quickly on day 3 prior to its peak day with a duration of 8 d, and its evolution is closely tied to the Rossby wave from upstream (i.e., the North Atlantic). Moreover, we find that the NAAA with a westward tilt might be mainly related to the wavenumbers 3–4. Further results reveal that against this background, the probability of regional PM<span class="inline-formula"><sub>2.5</sub></span> pollution for at least 3 d in the NCP is as high as 69 % (80 % at least 2 d) in the Nov–Jan (NDJ) period 2000–2021. In particular, air quality in the NCP tends to deteriorate on day 2 prior to the peak day and reaches a peak on the next day with a life cycle of 4 d. In the course of PM<span class="inline-formula"><sub>2.5</sub></span> pollution, a shallower atmospheric boundary layer and stronger surface southerly wind anomaly associated with the NAAA in the NCP appear 1 d earlier than poor air quality, which provides dynamic and thermal conditions for the accumulation of pollutants and finally occurrence of the PM<span class="inline-formula"><sub>2.5</sub></span> pollution on the following day. Furthermore, we show that the stagnant air leading to poor air quality is determined by the special structure of temperature in the vertical direction of the NAAA, while weak ventilation conditions might be related to a rapid build-up of the NAAA. The present results quantify the impact of the NAAA on PM<span class="inline-formula"><sub>2.5</sub></span> pollution in the NCP on the intraseasonal timescale.</p>
ISSN:1680-7316
1680-7324