Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China

<p>Fine particulate matter (PM<span class="inline-formula"><sub>2.5</sub></span>) has altered the radiation balance on Earth and raised environmental and health risks for decades but has only been monitored widely since 2013 in China. Historical long-term PM&l...

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Main Authors: J. Zhong, X. Zhang, K. Gui, J. Liao, Y. Fei, L. Jiang, L. Guo, L. Liu, H. Che, Y. Wang, D. Wang, Z. Zhou
Format: Article
Language:English
Published: Copernicus Publications 2022-07-01
Series:Earth System Science Data
Online Access:https://essd.copernicus.org/articles/14/3197/2022/essd-14-3197-2022.pdf
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author J. Zhong
X. Zhang
X. Zhang
K. Gui
J. Liao
Y. Fei
L. Jiang
L. Guo
L. Liu
H. Che
Y. Wang
D. Wang
Z. Zhou
author_facet J. Zhong
X. Zhang
X. Zhang
K. Gui
J. Liao
Y. Fei
L. Jiang
L. Guo
L. Liu
H. Che
Y. Wang
D. Wang
Z. Zhou
author_sort J. Zhong
collection DOAJ
description <p>Fine particulate matter (PM<span class="inline-formula"><sub>2.5</sub></span>) has altered the radiation balance on Earth and raised environmental and health risks for decades but has only been monitored widely since 2013 in China. Historical long-term PM<span class="inline-formula"><sub>2.5</sub></span> records with high temporal resolution are essential but lacking for both research and environmental management. Here, we reconstruct a site-based PM<span class="inline-formula"><sub>2.5</sub></span> dataset at 6 h intervals from 1960 to 2020 that combines long-term visibility, conventional meteorological observations, emissions, and elevation. The PM<span class="inline-formula"><sub>2.5</sub></span> concentration at each site is estimated based on an advanced machine learning model, LightGBM, that takes advantage of spatial features from 20 surrounding meteorological stations. Our model's performance is comparable to or even better than those of previous studies in by-year cross validation (CV) (<span class="inline-formula"><i>R</i><sup>2</sup>=0.7</span>) and spatial CV (<span class="inline-formula"><i>R</i><sup>2</sup>=0.76</span>) and is more advantageous in long-term records and high temporal resolution. This model also reconstructs a 0.25<span class="inline-formula"><sup>∘</sup></span> <span class="inline-formula">×</span> 0.25<span class="inline-formula"><sup>∘</sup></span>, 6-hourly, gridded PM<span class="inline-formula"><sub>2.5</sub></span> dataset by incorporating spatial features. The results show PM<span class="inline-formula"><sub>2.5</sub></span> pollution worsens gradually or maintains before 2010 from an interdecadal scale but mitigates in the following decade. Although the turning points vary in different regions, PM<span class="inline-formula"><sub>2.5</sub></span> mass concentrations in key regions decreased significantly after 2013 due to clean air actions. In particular, the annual average value of PM<span class="inline-formula"><sub>2.5</sub></span> in 2020 is nearly the lowest since 1960. These two PM<span class="inline-formula"><sub>2.5</sub></span> datasets (publicly available at <a href="https://doi.org/10.5281/zenodo.6372847">https://doi.org/10.5281/zenodo.6372847</a>, Zhong et al., 2022) provide spatiotemporal variations at high resolution, which lay the foundation for research studies associated with air pollution, climate change, and atmospheric chemical reanalysis.</p>
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spelling doaj.art-908a4c35d89d49eb93b23b0195c27a002022-12-22T02:59:36ZengCopernicus PublicationsEarth System Science Data1866-35081866-35162022-07-01143197321110.5194/essd-14-3197-2022Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in ChinaJ. Zhong0X. Zhang1X. Zhang2K. Gui3J. Liao4Y. Fei5L. Jiang6L. Guo7L. Liu8H. Che9Y. Wang10D. Wang11Z. Zhou12State Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaCenter for Excellence in Regional Atmospheric Environment, IUE, Chinese Academy of Sciences, Xiamen 361021, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaNational Meteorological Information Center, Beijing 100081, ChinaNational Meteorological Information Center, Beijing 100081, ChinaEarth System Numerical Prediction Center, Beijing 100081, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaDepartment of Earth System Science, Tsinghua University, Beijing 100084, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaNational Meteorological Information Center, Beijing 100081, China<p>Fine particulate matter (PM<span class="inline-formula"><sub>2.5</sub></span>) has altered the radiation balance on Earth and raised environmental and health risks for decades but has only been monitored widely since 2013 in China. Historical long-term PM<span class="inline-formula"><sub>2.5</sub></span> records with high temporal resolution are essential but lacking for both research and environmental management. Here, we reconstruct a site-based PM<span class="inline-formula"><sub>2.5</sub></span> dataset at 6 h intervals from 1960 to 2020 that combines long-term visibility, conventional meteorological observations, emissions, and elevation. The PM<span class="inline-formula"><sub>2.5</sub></span> concentration at each site is estimated based on an advanced machine learning model, LightGBM, that takes advantage of spatial features from 20 surrounding meteorological stations. Our model's performance is comparable to or even better than those of previous studies in by-year cross validation (CV) (<span class="inline-formula"><i>R</i><sup>2</sup>=0.7</span>) and spatial CV (<span class="inline-formula"><i>R</i><sup>2</sup>=0.76</span>) and is more advantageous in long-term records and high temporal resolution. This model also reconstructs a 0.25<span class="inline-formula"><sup>∘</sup></span> <span class="inline-formula">×</span> 0.25<span class="inline-formula"><sup>∘</sup></span>, 6-hourly, gridded PM<span class="inline-formula"><sub>2.5</sub></span> dataset by incorporating spatial features. The results show PM<span class="inline-formula"><sub>2.5</sub></span> pollution worsens gradually or maintains before 2010 from an interdecadal scale but mitigates in the following decade. Although the turning points vary in different regions, PM<span class="inline-formula"><sub>2.5</sub></span> mass concentrations in key regions decreased significantly after 2013 due to clean air actions. In particular, the annual average value of PM<span class="inline-formula"><sub>2.5</sub></span> in 2020 is nearly the lowest since 1960. These two PM<span class="inline-formula"><sub>2.5</sub></span> datasets (publicly available at <a href="https://doi.org/10.5281/zenodo.6372847">https://doi.org/10.5281/zenodo.6372847</a>, Zhong et al., 2022) provide spatiotemporal variations at high resolution, which lay the foundation for research studies associated with air pollution, climate change, and atmospheric chemical reanalysis.</p>https://essd.copernicus.org/articles/14/3197/2022/essd-14-3197-2022.pdf
spellingShingle J. Zhong
X. Zhang
X. Zhang
K. Gui
J. Liao
Y. Fei
L. Jiang
L. Guo
L. Liu
H. Che
Y. Wang
D. Wang
Z. Zhou
Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
Earth System Science Data
title Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
title_full Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
title_fullStr Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
title_full_unstemmed Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
title_short Reconstructing 6-hourly PM<sub>2.5</sub> datasets from 1960 to 2020 in China
title_sort reconstructing 6 hourly pm sub 2 5 sub datasets from 1960 to 2020 in china
url https://essd.copernicus.org/articles/14/3197/2022/essd-14-3197-2022.pdf
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