Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction
Amorphous metal catalysts often exhibit appealing catalytic properties, however, accurate control synthesis of amorphous nano-metal catalysts is a challenge. Here, the authors report a feasible strategy to prepare the amorphous Cu catalysts by supercritical CO2 treatment followed by electroreduction...
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2023-02-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-023-36721-8 |
| _version_ | 1797864294297108480 |
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| author | Chunjun Chen Xupeng Yan Yahui Wu Xiudong Zhang Shoujie Liu Fanyu Zhang Xiaofu Sun Qinggong Zhu Lirong Zheng Jing Zhang Xueqing Xing Zhonghua Wu Buxing Han |
| author_facet | Chunjun Chen Xupeng Yan Yahui Wu Xiudong Zhang Shoujie Liu Fanyu Zhang Xiaofu Sun Qinggong Zhu Lirong Zheng Jing Zhang Xueqing Xing Zhonghua Wu Buxing Han |
| author_sort | Chunjun Chen |
| collection | DOAJ |
| description | Amorphous metal catalysts often exhibit appealing catalytic properties, however, accurate control synthesis of amorphous nano-metal catalysts is a challenge. Here, the authors report a feasible strategy to prepare the amorphous Cu catalysts by supercritical CO2 treatment followed by electroreduction. The resulted catalyst shows high selectivity towards multi-carbon products for CO2 electroreduction. |
| first_indexed | 2024-04-09T22:49:32Z |
| format | Article |
| id | doaj.art-91245bccd1334167913511a85ed7ce39 |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-09T22:49:32Z |
| publishDate | 2023-02-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-91245bccd1334167913511a85ed7ce392023-03-22T11:40:51ZengNature PortfolioNature Communications2041-17232023-02-0114111010.1038/s41467-023-36721-8Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreductionChunjun Chen0Xupeng Yan1Yahui Wu2Xiudong Zhang3Shoujie Liu4Fanyu Zhang5Xiaofu Sun6Qinggong Zhu7Lirong Zheng8Jing Zhang9Xueqing Xing10Zhonghua Wu11Buxing Han12Beijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesChemistry and Chemical Engineering of Guangdong LaboratoryBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesInstitute of High Energy Physics, Chinese Academy of SciencesInstitute of High Energy Physics, Chinese Academy of SciencesInstitute of High Energy Physics, Chinese Academy of SciencesInstitute of High Energy Physics, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid and Interface and Thermodynamics, Institute of Chemistry, Chinese Academy of SciencesAmorphous metal catalysts often exhibit appealing catalytic properties, however, accurate control synthesis of amorphous nano-metal catalysts is a challenge. Here, the authors report a feasible strategy to prepare the amorphous Cu catalysts by supercritical CO2 treatment followed by electroreduction. The resulted catalyst shows high selectivity towards multi-carbon products for CO2 electroreduction.https://doi.org/10.1038/s41467-023-36721-8 |
| spellingShingle | Chunjun Chen Xupeng Yan Yahui Wu Xiudong Zhang Shoujie Liu Fanyu Zhang Xiaofu Sun Qinggong Zhu Lirong Zheng Jing Zhang Xueqing Xing Zhonghua Wu Buxing Han Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction Nature Communications |
| title | Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction |
| title_full | Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction |
| title_fullStr | Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction |
| title_full_unstemmed | Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction |
| title_short | Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction |
| title_sort | oxidation of metallic cu by supercritical co2 and control synthesis of amorphous nano metal catalysts for co2 electroreduction |
| url | https://doi.org/10.1038/s41467-023-36721-8 |
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