Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal

We have investigated the Mn-site substitution effect in Nd0.45Sr0.55MnO3 single crystal, which has an A-type layered antiferromagnetic (A-AFM) phase with the 3dx2−y2-type orbital-order. Substitution of Fe or Ga for Mn-site suppresses both the A-AFM order and competing ferromagnetic (FM) correlation,...

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Main Authors: Y. Izuchi, M. Akaki, D. Akahoshi, H. Kuwahara
Format: Article
Language:English
Published: AIP Publishing LLC 2014-02-01
Series:APL Materials
Online Access:http://dx.doi.org/10.1063/1.4866050
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author Y. Izuchi
M. Akaki
D. Akahoshi
H. Kuwahara
author_facet Y. Izuchi
M. Akaki
D. Akahoshi
H. Kuwahara
author_sort Y. Izuchi
collection DOAJ
description We have investigated the Mn-site substitution effect in Nd0.45Sr0.55MnO3 single crystal, which has an A-type layered antiferromagnetic (A-AFM) phase with the 3dx2−y2-type orbital-order. Substitution of Fe or Ga for Mn-site suppresses both the A-AFM order and competing ferromagnetic (FM) correlation, whereas Cr substitution suppresses only the A-AFM order but reactivates the underlying FM correlation via double-exchange mechanism along the AFM coupled c-direction. In Nd0.45Sr0.55Mn0.95Cr0.05O3, the A-AFM state with the orbital-order is changed into the orbital-disordered three-dimensional FM metallic state by applying magnetic field of μ0H = 12 T, which is much smaller than that of the parent compound Nd0.45Sr0.55MnO3.
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spelling doaj.art-92608306ad5f4f9394c79f40c15356dc2022-12-22T01:28:19ZengAIP Publishing LLCAPL Materials2166-532X2014-02-0122022106022106-710.1063/1.4866050008402APMReduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystalY. Izuchi0M. Akaki1D. Akahoshi2H. Kuwahara3Department of Physics, Sophia University, Tokyo 102-8554, JapanThe Institute for Solid State Physics, The University of Tokyo, Kashiwa 277-8581, JapanDepartment of Physics, Toho University, Funabashi 274-8510, JapanDepartment of Physics, Sophia University, Tokyo 102-8554, JapanWe have investigated the Mn-site substitution effect in Nd0.45Sr0.55MnO3 single crystal, which has an A-type layered antiferromagnetic (A-AFM) phase with the 3dx2−y2-type orbital-order. Substitution of Fe or Ga for Mn-site suppresses both the A-AFM order and competing ferromagnetic (FM) correlation, whereas Cr substitution suppresses only the A-AFM order but reactivates the underlying FM correlation via double-exchange mechanism along the AFM coupled c-direction. In Nd0.45Sr0.55Mn0.95Cr0.05O3, the A-AFM state with the orbital-order is changed into the orbital-disordered three-dimensional FM metallic state by applying magnetic field of μ0H = 12 T, which is much smaller than that of the parent compound Nd0.45Sr0.55MnO3.http://dx.doi.org/10.1063/1.4866050
spellingShingle Y. Izuchi
M. Akaki
D. Akahoshi
H. Kuwahara
Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
APL Materials
title Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
title_full Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
title_fullStr Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
title_full_unstemmed Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
title_short Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45Sr0.55MnO3 crystal
title_sort reduction of critical field for magnetic and orbital ordering phase transition in impurity substituted nd0 45sr0 55mno3 crystal
url http://dx.doi.org/10.1063/1.4866050
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AT makaki reductionofcriticalfieldformagneticandorbitalorderingphasetransitioninimpuritysubstitutednd045sr055mno3crystal
AT dakahoshi reductionofcriticalfieldformagneticandorbitalorderingphasetransitioninimpuritysubstitutednd045sr055mno3crystal
AT hkuwahara reductionofcriticalfieldformagneticandorbitalorderingphasetransitioninimpuritysubstitutednd045sr055mno3crystal