Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth

The 4H-SiC crystal is found to have great potential in terahertz generation via nonlinear optical frequency conversion due to its extremely high optical damage threshold, wide transparent range, etc. In this paper, optical rectification (OR) with tilted-pulse-front (TPF) setting based on the 4H-SiC...

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Main Authors: Fangjie Li, Kai Zhong, Yiwen Zhang, Tong Wu, Yuxin Liu, Hongzhan Qiao, Jining Li, Degang Xu, Jianquan Yao
Format: Article
Language:English
Published: Cambridge University Press 2023-01-01
Series:High Power Laser Science and Engineering
Subjects:
Online Access:https://www.cambridge.org/core/product/identifier/S209547192300052X/type/journal_article
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author Fangjie Li
Kai Zhong
Yiwen Zhang
Tong Wu
Yuxin Liu
Hongzhan Qiao
Jining Li
Degang Xu
Jianquan Yao
author_facet Fangjie Li
Kai Zhong
Yiwen Zhang
Tong Wu
Yuxin Liu
Hongzhan Qiao
Jining Li
Degang Xu
Jianquan Yao
author_sort Fangjie Li
collection DOAJ
description The 4H-SiC crystal is found to have great potential in terahertz generation via nonlinear optical frequency conversion due to its extremely high optical damage threshold, wide transparent range, etc. In this paper, optical rectification (OR) with tilted-pulse-front (TPF) setting based on the 4H-SiC crystal is proposed. The theory accounts for the optimization of incident pulse pre-chirping in the TPF OR process under high-intensity femtosecond laser pumping. Compared with the currently recognized LiNbO3-based TPF OR, which generates a single-cycle terahertz pulse within 3 THz, 4H-SiC demonstrates a significant advantage in producing ultra-widely tunable (up to over 14 THz, TPF angle 31°–38°) terahertz waves with high efficiency (~10–2) and strong field (~MV/cm). Besides, the spectrum characteristics, as well as the evolution from single- to multi-cycle terahertz pulses can be modulated flexibly by pre-chirping. The simulation results show that 4H-SiC enables terahertz frequency extending to an unprecedent range by OR, which has extremely important potential in strong-field terahertz applications.
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spelling doaj.art-92750c71372f47e4baa40bad48e922762023-10-02T12:03:40ZengCambridge University PressHigh Power Laser Science and Engineering2095-47192052-32892023-01-011110.1017/hpl.2023.52Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidthFangjie Li0https://orcid.org/0000-0001-7683-3461Kai Zhong1https://orcid.org/0000-0002-5320-8388Yiwen Zhang2Tong Wu3Yuxin Liu4https://orcid.org/0009-0004-8264-9141Hongzhan Qiao5Jining Li6Degang Xu7Jianquan Yao8School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Marine Science and Technology, Tianjin University, Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaSchool of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin, China Key Laboratory of Opto-electronic Information Technology, Ministry of Education (Tianjin University), Tianjin, ChinaThe 4H-SiC crystal is found to have great potential in terahertz generation via nonlinear optical frequency conversion due to its extremely high optical damage threshold, wide transparent range, etc. In this paper, optical rectification (OR) with tilted-pulse-front (TPF) setting based on the 4H-SiC crystal is proposed. The theory accounts for the optimization of incident pulse pre-chirping in the TPF OR process under high-intensity femtosecond laser pumping. Compared with the currently recognized LiNbO3-based TPF OR, which generates a single-cycle terahertz pulse within 3 THz, 4H-SiC demonstrates a significant advantage in producing ultra-widely tunable (up to over 14 THz, TPF angle 31°–38°) terahertz waves with high efficiency (~10–2) and strong field (~MV/cm). Besides, the spectrum characteristics, as well as the evolution from single- to multi-cycle terahertz pulses can be modulated flexibly by pre-chirping. The simulation results show that 4H-SiC enables terahertz frequency extending to an unprecedent range by OR, which has extremely important potential in strong-field terahertz applications.https://www.cambridge.org/core/product/identifier/S209547192300052X/type/journal_articleoptical rectificationsilicon carbideterahertz radiationtilted-pulse-front
spellingShingle Fangjie Li
Kai Zhong
Yiwen Zhang
Tong Wu
Yuxin Liu
Hongzhan Qiao
Jining Li
Degang Xu
Jianquan Yao
Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
High Power Laser Science and Engineering
optical rectification
silicon carbide
terahertz radiation
tilted-pulse-front
title Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
title_full Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
title_fullStr Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
title_full_unstemmed Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
title_short Optical rectification in 4H-SiC: paving the way to generate strong terahertz fields with ultra-wide bandwidth
title_sort optical rectification in 4h sic paving the way to generate strong terahertz fields with ultra wide bandwidth
topic optical rectification
silicon carbide
terahertz radiation
tilted-pulse-front
url https://www.cambridge.org/core/product/identifier/S209547192300052X/type/journal_article
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