Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
The investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves ch...
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Format: | Article |
Language: | English |
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Taylor & Francis Group
2018-01-01
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Series: | Advances in Physics: X |
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Online Access: | http://dx.doi.org/10.1080/23746149.2017.1418183 |
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author | Robert E. Grisenti Anton Kalinin Claudia Goy Alexander Schottelius |
author_facet | Robert E. Grisenti Anton Kalinin Claudia Goy Alexander Schottelius |
author_sort | Robert E. Grisenti |
collection | DOAJ |
description | The investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves challenging. Here, we show that microscopic laminar jets in vacuum offer a powerful tool for novel studies of supercooled liquids on previously inaccessible time scales in a class of atomic and molecular model systems that have so far remained inaccessible because of the lack of adequate experimental approaches. The use of liquid jets represents a remarkable opportunity to significantly advance our knowledge of topics that are relevant to interdisciplinary fields such as atmospheric physics and material science. |
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format | Article |
id | doaj.art-92c4eaa30c2b4e38a2273cffc93fc0b6 |
institution | Directory Open Access Journal |
issn | 2374-6149 |
language | English |
last_indexed | 2024-12-23T14:50:30Z |
publishDate | 2018-01-01 |
publisher | Taylor & Francis Group |
record_format | Article |
series | Advances in Physics: X |
spelling | doaj.art-92c4eaa30c2b4e38a2273cffc93fc0b62022-12-21T17:42:58ZengTaylor & Francis GroupAdvances in Physics: X2374-61492018-01-013110.1080/23746149.2017.14181831418183Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquidsRobert E. Grisenti0Anton Kalinin1Claudia Goy2Alexander Schottelius3Institut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätThe investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves challenging. Here, we show that microscopic laminar jets in vacuum offer a powerful tool for novel studies of supercooled liquids on previously inaccessible time scales in a class of atomic and molecular model systems that have so far remained inaccessible because of the lack of adequate experimental approaches. The use of liquid jets represents a remarkable opportunity to significantly advance our knowledge of topics that are relevant to interdisciplinary fields such as atmospheric physics and material science.http://dx.doi.org/10.1080/23746149.2017.1418183Liquid jetssupercooled liquidscrystallizationRaman and X-ray scattering |
spellingShingle | Robert E. Grisenti Anton Kalinin Claudia Goy Alexander Schottelius Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids Advances in Physics: X Liquid jets supercooled liquids crystallization Raman and X-ray scattering |
title | Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
title_full | Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
title_fullStr | Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
title_full_unstemmed | Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
title_short | Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
title_sort | evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids |
topic | Liquid jets supercooled liquids crystallization Raman and X-ray scattering |
url | http://dx.doi.org/10.1080/23746149.2017.1418183 |
work_keys_str_mv | AT robertegrisenti evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids AT antonkalinin evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids AT claudiagoy evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids AT alexanderschottelius evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids |