Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids

The investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves ch...

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Main Authors: Robert E. Grisenti, Anton Kalinin, Claudia Goy, Alexander Schottelius
Format: Article
Language:English
Published: Taylor & Francis Group 2018-01-01
Series:Advances in Physics: X
Subjects:
Online Access:http://dx.doi.org/10.1080/23746149.2017.1418183
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author Robert E. Grisenti
Anton Kalinin
Claudia Goy
Alexander Schottelius
author_facet Robert E. Grisenti
Anton Kalinin
Claudia Goy
Alexander Schottelius
author_sort Robert E. Grisenti
collection DOAJ
description The investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves challenging. Here, we show that microscopic laminar jets in vacuum offer a powerful tool for novel studies of supercooled liquids on previously inaccessible time scales in a class of atomic and molecular model systems that have so far remained inaccessible because of the lack of adequate experimental approaches. The use of liquid jets represents a remarkable opportunity to significantly advance our knowledge of topics that are relevant to interdisciplinary fields such as atmospheric physics and material science.
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spelling doaj.art-92c4eaa30c2b4e38a2273cffc93fc0b62022-12-21T17:42:58ZengTaylor & Francis GroupAdvances in Physics: X2374-61492018-01-013110.1080/23746149.2017.14181831418183Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquidsRobert E. Grisenti0Anton Kalinin1Claudia Goy2Alexander Schottelius3Institut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätInstitut für Kernphysik, J. W. Goethe-UniversitätThe investigation of non-equilibrium phase transformations, such as crystallization, in supercooled liquids – below their melting point but still liquid – is of fundamental importance in condensed matter physics. However, accessing experimentally the details of such fast structural changes proves challenging. Here, we show that microscopic laminar jets in vacuum offer a powerful tool for novel studies of supercooled liquids on previously inaccessible time scales in a class of atomic and molecular model systems that have so far remained inaccessible because of the lack of adequate experimental approaches. The use of liquid jets represents a remarkable opportunity to significantly advance our knowledge of topics that are relevant to interdisciplinary fields such as atmospheric physics and material science.http://dx.doi.org/10.1080/23746149.2017.1418183Liquid jetssupercooled liquidscrystallizationRaman and X-ray scattering
spellingShingle Robert E. Grisenti
Anton Kalinin
Claudia Goy
Alexander Schottelius
Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
Advances in Physics: X
Liquid jets
supercooled liquids
crystallization
Raman and X-ray scattering
title Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
title_full Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
title_fullStr Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
title_full_unstemmed Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
title_short Evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
title_sort evaporating laminar microjets for studies of rapidly evolving structural transformations in supercooled liquids
topic Liquid jets
supercooled liquids
crystallization
Raman and X-ray scattering
url http://dx.doi.org/10.1080/23746149.2017.1418183
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AT antonkalinin evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids
AT claudiagoy evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids
AT alexanderschottelius evaporatinglaminarmicrojetsforstudiesofrapidlyevolvingstructuraltransformationsinsupercooledliquids