Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment

Due to multiple charge transport pathways, adjustable layer spacing, compositional flexibility, low manufacturing cost, and absorption of visible light, layered double hydroxides (LDHs) are a promising material for wastewater treatment. In this study, LDH films and Fe-doped LDH films with different...

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Main Authors: Zhongchuan Wang, Pengfei Fang, Parveen Kumar, Weiwei Wang, Bo Liu, Jiao Li
Format: Article
Language:English
Published: MDPI AG 2019-05-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/9/6/807
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author Zhongchuan Wang
Pengfei Fang
Parveen Kumar
Weiwei Wang
Bo Liu
Jiao Li
author_facet Zhongchuan Wang
Pengfei Fang
Parveen Kumar
Weiwei Wang
Bo Liu
Jiao Li
author_sort Zhongchuan Wang
collection DOAJ
description Due to multiple charge transport pathways, adjustable layer spacing, compositional flexibility, low manufacturing cost, and absorption of visible light, layered double hydroxides (LDHs) are a promising material for wastewater treatment. In this study, LDH films and Fe-doped LDH films with different metal ions (Ni, Al, Fe) on the surface of conductive cloth were successfully prepared and applied for the photocatalytic degradation of wastewater containing methyl orange and Ag ions under visible-light irradiation. The chemical state of Fe ions and the composition of LDHs on methyl orange photodegradation were investigated. The experimental results showed that LDH films exhibited high photocatalytic activity. The photocatalytic activity of LDH films on methyl orange improved in the mixed wastewater, and the Fe-doped NiAl−LDH films exhibited best visible-light photocatalytic performance. The analysis showed that Ag ions in the mixed wastewater were reduced by the LDH films and subsequently deposited on the surface of the LDH films. The Ag nanoparticles acted as electron traps and promoted the photocatalytic activity of the LDH films on methyl orange. Thus, we have demonstrated that prepared LDH films can be used in the treatment of mixed wastewater and have broad application prospects in environmental remediation and purification processes.
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spelling doaj.art-93965f2fe00144098bd1ff16649a68802022-12-21T23:59:13ZengMDPI AGNanomaterials2079-49912019-05-019680710.3390/nano9060807nano9060807Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater TreatmentZhongchuan Wang0Pengfei Fang1Parveen Kumar2Weiwei Wang3Bo Liu4Jiao Li5School of Material Science and Engineering, Shandong University of Technology, Zibo 255000, ChinaSchool of Material Science and Engineering, Shandong University of Technology, Zibo 255000, ChinaLaboratory of Functional Molecular and Materials, School of Physics and Optoelectronic Engineering, Shandong University of Technology, Zibo 255000, ChinaSchool of Material Science and Engineering, Shandong University of Technology, Zibo 255000, ChinaSchool of Material Science and Engineering, Shandong University of Technology, Zibo 255000, ChinaSchool of Material Science and Engineering, Shandong University of Technology, Zibo 255000, ChinaDue to multiple charge transport pathways, adjustable layer spacing, compositional flexibility, low manufacturing cost, and absorption of visible light, layered double hydroxides (LDHs) are a promising material for wastewater treatment. In this study, LDH films and Fe-doped LDH films with different metal ions (Ni, Al, Fe) on the surface of conductive cloth were successfully prepared and applied for the photocatalytic degradation of wastewater containing methyl orange and Ag ions under visible-light irradiation. The chemical state of Fe ions and the composition of LDHs on methyl orange photodegradation were investigated. The experimental results showed that LDH films exhibited high photocatalytic activity. The photocatalytic activity of LDH films on methyl orange improved in the mixed wastewater, and the Fe-doped NiAl−LDH films exhibited best visible-light photocatalytic performance. The analysis showed that Ag ions in the mixed wastewater were reduced by the LDH films and subsequently deposited on the surface of the LDH films. The Ag nanoparticles acted as electron traps and promoted the photocatalytic activity of the LDH films on methyl orange. Thus, we have demonstrated that prepared LDH films can be used in the treatment of mixed wastewater and have broad application prospects in environmental remediation and purification processes.https://www.mdpi.com/2079-4991/9/6/807LDHsfilmmixed wastewaterphotocatalytic activity
spellingShingle Zhongchuan Wang
Pengfei Fang
Parveen Kumar
Weiwei Wang
Bo Liu
Jiao Li
Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
Nanomaterials
LDHs
film
mixed wastewater
photocatalytic activity
title Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
title_full Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
title_fullStr Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
title_full_unstemmed Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
title_short Controlled Growth of LDH Films with Enhanced Photocatalytic Activity in a Mixed Wastewater Treatment
title_sort controlled growth of ldh films with enhanced photocatalytic activity in a mixed wastewater treatment
topic LDHs
film
mixed wastewater
photocatalytic activity
url https://www.mdpi.com/2079-4991/9/6/807
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AT parveenkumar controlledgrowthofldhfilmswithenhancedphotocatalyticactivityinamixedwastewatertreatment
AT weiweiwang controlledgrowthofldhfilmswithenhancedphotocatalyticactivityinamixedwastewatertreatment
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