Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond

We propose the generation of attosecond entangled biphotons in the extreme-ultraviolet regime by two-photon decay of a metastable atomic state as a source similar to spontaneous parametric down-conversion photons. The 1s2s ^{1}S_{0} metastable state in helium decays to the ground state by the emissi...

Full description

Bibliographic Details
Main Authors: Yimeng Wang, Siddhant Pandey, Chris H. Greene, Niranjan Shivaram
Format: Article
Language:English
Published: American Physical Society 2022-09-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.4.L032038
_version_ 1797210659836919808
author Yimeng Wang
Siddhant Pandey
Chris H. Greene
Niranjan Shivaram
author_facet Yimeng Wang
Siddhant Pandey
Chris H. Greene
Niranjan Shivaram
author_sort Yimeng Wang
collection DOAJ
description We propose the generation of attosecond entangled biphotons in the extreme-ultraviolet regime by two-photon decay of a metastable atomic state as a source similar to spontaneous parametric down-conversion photons. The 1s2s ^{1}S_{0} metastable state in helium decays to the ground state by the emission of two energy-time entangled photons with a photon bandwidth equal to the total energy spacing of 20.62 eV. This results in a pair correlation time in the attosecond regime making these entangled photons a highly suitable source for attosecond pump-probe experiments. The biphoton generation rate from a direct four-photon excitation of helium at 240 nm is calculated and used to assess some feasible schemes to generate these biphotons. Possible applications of entangled biphotons in attosecond timescale experiments, and a discussion of their potential to reach the zeptosecond regime are presented.
first_indexed 2024-04-24T10:14:07Z
format Article
id doaj.art-939c70b63a5b47fb91ba3ace2d390775
institution Directory Open Access Journal
issn 2643-1564
language English
last_indexed 2024-04-24T10:14:07Z
publishDate 2022-09-01
publisher American Physical Society
record_format Article
series Physical Review Research
spelling doaj.art-939c70b63a5b47fb91ba3ace2d3907752024-04-12T17:24:19ZengAmerican Physical SocietyPhysical Review Research2643-15642022-09-0143L03203810.1103/PhysRevResearch.4.L032038Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyondYimeng WangSiddhant PandeyChris H. GreeneNiranjan ShivaramWe propose the generation of attosecond entangled biphotons in the extreme-ultraviolet regime by two-photon decay of a metastable atomic state as a source similar to spontaneous parametric down-conversion photons. The 1s2s ^{1}S_{0} metastable state in helium decays to the ground state by the emission of two energy-time entangled photons with a photon bandwidth equal to the total energy spacing of 20.62 eV. This results in a pair correlation time in the attosecond regime making these entangled photons a highly suitable source for attosecond pump-probe experiments. The biphoton generation rate from a direct four-photon excitation of helium at 240 nm is calculated and used to assess some feasible schemes to generate these biphotons. Possible applications of entangled biphotons in attosecond timescale experiments, and a discussion of their potential to reach the zeptosecond regime are presented.http://doi.org/10.1103/PhysRevResearch.4.L032038
spellingShingle Yimeng Wang
Siddhant Pandey
Chris H. Greene
Niranjan Shivaram
Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
Physical Review Research
title Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
title_full Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
title_fullStr Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
title_full_unstemmed Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
title_short Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
title_sort attosecond entangled photons from two photon decay of metastable atoms a source for attosecond experiments and beyond
url http://doi.org/10.1103/PhysRevResearch.4.L032038
work_keys_str_mv AT yimengwang attosecondentangledphotonsfromtwophotondecayofmetastableatomsasourceforattosecondexperimentsandbeyond
AT siddhantpandey attosecondentangledphotonsfromtwophotondecayofmetastableatomsasourceforattosecondexperimentsandbeyond
AT chrishgreene attosecondentangledphotonsfromtwophotondecayofmetastableatomsasourceforattosecondexperimentsandbeyond
AT niranjanshivaram attosecondentangledphotonsfromtwophotondecayofmetastableatomsasourceforattosecondexperimentsandbeyond