Freezing of few nanometers water droplets

Ice nucleation in confined geometries is a ubiquitous phenomenon, but difficult to characterize. Here the authors investigate experimentally the freezing of water nanodroplets surrounded by octane in nanopores down to 2 nm, and demonstrate that the soft curved oil-water interface suppresses heteroge...

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Main Authors: Alireza Hakimian, Mohammadjavad Mohebinia, Masoumeh Nazari, Ali Davoodabadi, Sina Nazifi, Zixu Huang, Jiming Bao, Hadi Ghasemi
Format: Article
Language:English
Published: Nature Portfolio 2021-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-27346-w
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author Alireza Hakimian
Mohammadjavad Mohebinia
Masoumeh Nazari
Ali Davoodabadi
Sina Nazifi
Zixu Huang
Jiming Bao
Hadi Ghasemi
author_facet Alireza Hakimian
Mohammadjavad Mohebinia
Masoumeh Nazari
Ali Davoodabadi
Sina Nazifi
Zixu Huang
Jiming Bao
Hadi Ghasemi
author_sort Alireza Hakimian
collection DOAJ
description Ice nucleation in confined geometries is a ubiquitous phenomenon, but difficult to characterize. Here the authors investigate experimentally the freezing of water nanodroplets surrounded by octane in nanopores down to 2 nm, and demonstrate that the soft curved oil-water interface suppresses heterogeneous ice nucleation, which occurs at a lower temperature than homogenous bulk nucleation.
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spelling doaj.art-93b3228db4fa47b8b73e22baf9b74b502022-12-21T20:39:23ZengNature PortfolioNature Communications2041-17232021-11-011211810.1038/s41467-021-27346-wFreezing of few nanometers water dropletsAlireza Hakimian0Mohammadjavad Mohebinia1Masoumeh Nazari2Ali Davoodabadi3Sina Nazifi4Zixu Huang5Jiming Bao6Hadi Ghasemi7Department of Mechanical Engineering, University of HoustonDepartment of Electrical and Computer Engineering, University of HoustonDepartment of Mechanical Engineering, University of HoustonDepartment of Mechanical Engineering, University of HoustonDepartment of Mechanical Engineering, University of HoustonDepartment of Mechanical Engineering, University of HoustonDepartment of Electrical and Computer Engineering, University of HoustonDepartment of Mechanical Engineering, University of HoustonIce nucleation in confined geometries is a ubiquitous phenomenon, but difficult to characterize. Here the authors investigate experimentally the freezing of water nanodroplets surrounded by octane in nanopores down to 2 nm, and demonstrate that the soft curved oil-water interface suppresses heterogeneous ice nucleation, which occurs at a lower temperature than homogenous bulk nucleation.https://doi.org/10.1038/s41467-021-27346-w
spellingShingle Alireza Hakimian
Mohammadjavad Mohebinia
Masoumeh Nazari
Ali Davoodabadi
Sina Nazifi
Zixu Huang
Jiming Bao
Hadi Ghasemi
Freezing of few nanometers water droplets
Nature Communications
title Freezing of few nanometers water droplets
title_full Freezing of few nanometers water droplets
title_fullStr Freezing of few nanometers water droplets
title_full_unstemmed Freezing of few nanometers water droplets
title_short Freezing of few nanometers water droplets
title_sort freezing of few nanometers water droplets
url https://doi.org/10.1038/s41467-021-27346-w
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AT alidavoodabadi freezingoffewnanometerswaterdroplets
AT sinanazifi freezingoffewnanometerswaterdroplets
AT zixuhuang freezingoffewnanometerswaterdroplets
AT jimingbao freezingoffewnanometerswaterdroplets
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