Systematic detection of local CH<sub>4</sub> anomalies by combining satellite measurements with high-resolution forecasts

<p>In this study, we present a novel monitoring methodology that combines satellite retrievals and forecasts to detect local <span class="inline-formula">CH<sub>4</sub></span> concentration anomalies worldwide. These anomalies are caused by rapidly changing an...

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Bibliographic Details
Main Authors: J. Barré, I. Aben, A. Agustí-Panareda, G. Balsamo, N. Bousserez, P. Dueben, R. Engelen, A. Inness, A. Lorente, J. McNorton, V.-H. Peuch, G. Radnoti, R. Ribas
Format: Article
Language:English
Published: Copernicus Publications 2021-04-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/21/5117/2021/acp-21-5117-2021.pdf
Description
Summary:<p>In this study, we present a novel monitoring methodology that combines satellite retrievals and forecasts to detect local <span class="inline-formula">CH<sub>4</sub></span> concentration anomalies worldwide. These anomalies are caused by rapidly changing anthropogenic emissions that significantly contribute to the <span class="inline-formula">CH<sub>4</sub></span> atmospheric budget and by biases in the satellite retrieval data. The method uses high-resolution (7 km <span class="inline-formula">×</span> 7 km) retrievals of total column <span class="inline-formula">CH<sub>4</sub></span> from the TROPOspheric Monitoring Instrument (TROPOMI) on board the Sentinel 5 Precursor satellite. Observations are combined with high-resolution <span class="inline-formula">CH<sub>4</sub></span> forecasts (<span class="inline-formula">∼</span> 9 <span class="inline-formula">km</span>) produced by the Copernicus Atmosphere Monitoring Service (CAMS) to provide departures (observations minus forecasts) at close to the satellite's native resolution at appropriate time. Investigating these departures is an effective way to link satellite measurements and emission inventory data in a quantitative manner. We perform filtering on the departures to remove the synoptic-scale and meso-alpha-scale biases in both forecasts and satellite observations. We then apply a simple classification scheme to the filtered departures to detect anomalies and plumes that are missing (e.g. pipeline or facility leaks), underreported or overreported (e.g. depleted drilling fields) in the CAMS emissions. The classification method also shows some limitations to detect emission anomalies only due to local satellite retrieval biases linked to albedo and scattering issues.</p>
ISSN:1680-7316
1680-7324