Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces

Optomechanical manipulation of plasmonic nanoparticles is an area of current interest, both fundamental and applied. However, no experimental method is available to determine the forward-directed scattering force that dominates for incident light of a wavelength close to the plasmon resonance. Here,...

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Main Authors: C. Zensen, N. Villadsen, F. Winterer, S. R. Keiding, T. Lohmüller
Format: Article
Language:English
Published: AIP Publishing LLC 2016-05-01
Series:APL Photonics
Online Access:http://dx.doi.org/10.1063/1.4945351
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author C. Zensen
N. Villadsen
F. Winterer
S. R. Keiding
T. Lohmüller
author_facet C. Zensen
N. Villadsen
F. Winterer
S. R. Keiding
T. Lohmüller
author_sort C. Zensen
collection DOAJ
description Optomechanical manipulation of plasmonic nanoparticles is an area of current interest, both fundamental and applied. However, no experimental method is available to determine the forward-directed scattering force that dominates for incident light of a wavelength close to the plasmon resonance. Here, we demonstrate how the scattering force acting on a single gold nanoparticle in solution can be measured. An optically trapped 80 nm particle was repetitively pushed from the side with laser light resonant to the particle plasmon frequency. A lock-in analysis of the particle movement provides a measured value for the scattering force. We obtain a resolution of less than 3 femtonewtons which is an order of magnitude smaller than any measurement of switchable forces performed on nanoparticles in solution with single beam optical tweezers to date. We compared the results of the force measurement with Mie simulations of the optical scattering force on a gold nanoparticle and found good agreement between experiment and theory within a few fN.
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spelling doaj.art-94d313d4f878479a9c43fc9d24a661ee2022-12-22T03:24:24ZengAIP Publishing LLCAPL Photonics2378-09672016-05-0112026102026102-810.1063/1.4945351004601APPPushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forcesC. Zensen0N. Villadsen1F. Winterer2S. R. Keiding3T. Lohmüller4Photonics and Optoelectronics Group, Department of Physics and Center for Nanoscience (CeNS), Ludwig-Maximilians-Universität München, 80799 Munich, GermanyDepartment of Chemistry, Aarhus University, DK 8000 Aarhus C, DenmarkPhotonics and Optoelectronics Group, Department of Physics and Center for Nanoscience (CeNS), Ludwig-Maximilians-Universität München, 80799 Munich, GermanyDepartment of Chemistry, Aarhus University, DK 8000 Aarhus C, DenmarkPhotonics and Optoelectronics Group, Department of Physics and Center for Nanoscience (CeNS), Ludwig-Maximilians-Universität München, 80799 Munich, GermanyOptomechanical manipulation of plasmonic nanoparticles is an area of current interest, both fundamental and applied. However, no experimental method is available to determine the forward-directed scattering force that dominates for incident light of a wavelength close to the plasmon resonance. Here, we demonstrate how the scattering force acting on a single gold nanoparticle in solution can be measured. An optically trapped 80 nm particle was repetitively pushed from the side with laser light resonant to the particle plasmon frequency. A lock-in analysis of the particle movement provides a measured value for the scattering force. We obtain a resolution of less than 3 femtonewtons which is an order of magnitude smaller than any measurement of switchable forces performed on nanoparticles in solution with single beam optical tweezers to date. We compared the results of the force measurement with Mie simulations of the optical scattering force on a gold nanoparticle and found good agreement between experiment and theory within a few fN.http://dx.doi.org/10.1063/1.4945351
spellingShingle C. Zensen
N. Villadsen
F. Winterer
S. R. Keiding
T. Lohmüller
Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
APL Photonics
title Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
title_full Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
title_fullStr Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
title_full_unstemmed Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
title_short Pushing nanoparticles with light — A femtonewton resolved measurement of optical scattering forces
title_sort pushing nanoparticles with light a femtonewton resolved measurement of optical scattering forces
url http://dx.doi.org/10.1063/1.4945351
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