Broadband nonlinear optical properties of red fluorescent carbon dots

Carbon dots (CDs) provide ideal platforms for applications in bioimaging, sensing, and photocatalysis. Herein, a new type of red fluorescent carbon dot (RCD) is successfully synthesized, and its broadband nonlinear optical (NLO) properties are systematically characterized. The nonlinear absorption c...

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Main Authors: Wenxuan Fan, Jun He, Hao Wei, Chen Zhang, Menglong Zhu, Defeng Xu, Si Xiao, Jiangling He, Zhihui Chen, Jianqiao Meng
Format: Article
Language:English
Published: Elsevier 2022-07-01
Series:Results in Physics
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2211379722003102
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author Wenxuan Fan
Jun He
Hao Wei
Chen Zhang
Menglong Zhu
Defeng Xu
Si Xiao
Jiangling He
Zhihui Chen
Jianqiao Meng
author_facet Wenxuan Fan
Jun He
Hao Wei
Chen Zhang
Menglong Zhu
Defeng Xu
Si Xiao
Jiangling He
Zhihui Chen
Jianqiao Meng
author_sort Wenxuan Fan
collection DOAJ
description Carbon dots (CDs) provide ideal platforms for applications in bioimaging, sensing, and photocatalysis. Herein, a new type of red fluorescent carbon dot (RCD) is successfully synthesized, and its broadband nonlinear optical (NLO) properties are systematically characterized. The nonlinear absorption coefficient (αNL) values of the RCDs at 580, 630, 650, 1064 nm are − 0.65, −3.09, −4.02, and 0.14 cm/GW, respectively. The nonlinear absorption transforms from saturable absorption to two-photon absorption in the near-infrared domain. We demonstrate the application of the RCDs for imaging Hela cells. Our results indicate that the synthesized RCDs with a broadband NLO response exhibit potential applications in saturable absorbers and deep-tissue imaging.
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spelling doaj.art-95a924d9e56e43cbb20def6a6c614d752022-12-22T00:39:48ZengElsevierResults in Physics2211-37972022-07-0138105591Broadband nonlinear optical properties of red fluorescent carbon dotsWenxuan Fan0Jun He1Hao Wei2Chen Zhang3Menglong Zhu4Defeng Xu5Si Xiao6Jiangling He7Zhihui Chen8Jianqiao Meng9Hunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaHunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaHunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaHunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaDepartment of Applied Physics, School of Microelectronics and Physics, Hunan University of Technology and Business, Changsha 410205, PR ChinaHunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaHunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR ChinaNational R&D Center for Se-rich Agricultural. Products Processing, Hubei Engineering Research Center for Deep Processing of Green Se-rich Agricultural Products, School of Modern, Industry for Selenium Science and Engineering, Wuhan Polytechnic University, Wuhan 430023, PR China; Corresponding authors.Hunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR China; Corresponding authors.Hunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, PR China; Corresponding authors.Carbon dots (CDs) provide ideal platforms for applications in bioimaging, sensing, and photocatalysis. Herein, a new type of red fluorescent carbon dot (RCD) is successfully synthesized, and its broadband nonlinear optical (NLO) properties are systematically characterized. The nonlinear absorption coefficient (αNL) values of the RCDs at 580, 630, 650, 1064 nm are − 0.65, −3.09, −4.02, and 0.14 cm/GW, respectively. The nonlinear absorption transforms from saturable absorption to two-photon absorption in the near-infrared domain. We demonstrate the application of the RCDs for imaging Hela cells. Our results indicate that the synthesized RCDs with a broadband NLO response exhibit potential applications in saturable absorbers and deep-tissue imaging.http://www.sciencedirect.com/science/article/pii/S2211379722003102Carbon dotsNonlinear opticsTwo-photon absorptionFluorescenceBiological imaging
spellingShingle Wenxuan Fan
Jun He
Hao Wei
Chen Zhang
Menglong Zhu
Defeng Xu
Si Xiao
Jiangling He
Zhihui Chen
Jianqiao Meng
Broadband nonlinear optical properties of red fluorescent carbon dots
Results in Physics
Carbon dots
Nonlinear optics
Two-photon absorption
Fluorescence
Biological imaging
title Broadband nonlinear optical properties of red fluorescent carbon dots
title_full Broadband nonlinear optical properties of red fluorescent carbon dots
title_fullStr Broadband nonlinear optical properties of red fluorescent carbon dots
title_full_unstemmed Broadband nonlinear optical properties of red fluorescent carbon dots
title_short Broadband nonlinear optical properties of red fluorescent carbon dots
title_sort broadband nonlinear optical properties of red fluorescent carbon dots
topic Carbon dots
Nonlinear optics
Two-photon absorption
Fluorescence
Biological imaging
url http://www.sciencedirect.com/science/article/pii/S2211379722003102
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