Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal
Graphite carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is a visible light responsive semiconductor material with the advantages of high stability, low cost, high adjustability of structure and property. With the continuous development of green and non-secondary pollution phot...
| Main Authors: | , , , , |
|---|---|
| Format: | Article |
| Language: | zho |
| Published: |
Journal of Materials Engineering
2021-04-01
|
| Series: | Cailiao gongcheng |
| Subjects: | |
| Online Access: | http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2020.000285 |
| _version_ | 1828082236189048832 |
|---|---|
| author | GE Yu-jie WU Jiao HE Zhi-qiang WANG Guo-hua LIU Jin-xiang |
| author_facet | GE Yu-jie WU Jiao HE Zhi-qiang WANG Guo-hua LIU Jin-xiang |
| author_sort | GE Yu-jie |
| collection | DOAJ |
| description | Graphite carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is a visible light responsive semiconductor material with the advantages of high stability, low cost, high adjustability of structure and property. With the continuous development of green and non-secondary pollution photocatalytic technology, g-C<sub>3</sub>N<sub>4</sub>has gradually become a research hotspot in the field of environment and energy science. Nevertheless, the bare g-C<sub>3</sub>N<sub>4</sub> exhibits relatively low photocatalytic efficiency, which is due to the rapid recombination of photogenerated charge carriers and low visible light utilization efficiency. Among many modification methods, heterogeneous coupling is considered to be an effective method to improve the photocatalytic performance of g-C<sub>3</sub>N<sub>4</sub>. In recent years, with different inorganic semiconductors, precious metals, and carbon materials, heterogeneously coupled with g-C<sub>3</sub>N<sub>4</sub>, the researchers promoted the transfer efficiency of photoelectrons in the photocatalytic system, broadened the absorption range of visible light of g-C<sub>3</sub>N<sub>4</sub>-based photocatalysts, and enhanced the catalytic stability and structure regulation of g-C<sub>3</sub>N<sub>4</sub>. The catalytic mechanism of heterogeneous photocatalysts and construction of heterogeneous photocatalytic system based on g-C<sub>3</sub>N<sub>4</sub> were summarized, the research progress of g-C<sub>3</sub>N<sub>4</sub>-based heterojunction in degradation of environmental pollutants was discussed. Finally, the prospect of designing excellent g-C<sub>3</sub>N<sub>4</sub>-based photocatalyst and their applications in photocatalytic degradation of dyes,organic pollutants and reduction of toxic heavy metals with excellent performance and its prospect in the field of environmental pollutant removal were prospected. |
| first_indexed | 2024-04-11T03:47:46Z |
| format | Article |
| id | doaj.art-95d816a8c2f3478e91201d7b87a05f6f |
| institution | Directory Open Access Journal |
| issn | 1001-4381 1001-4381 |
| language | zho |
| last_indexed | 2024-04-11T03:47:46Z |
| publishDate | 2021-04-01 |
| publisher | Journal of Materials Engineering |
| record_format | Article |
| series | Cailiao gongcheng |
| spelling | doaj.art-95d816a8c2f3478e91201d7b87a05f6f2023-01-02T02:21:53ZzhoJournal of Materials EngineeringCailiao gongcheng1001-43811001-43812021-04-01494233310.11868/j.issn.1001-4381.2020.00028520210403Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removalGE Yu-jie0WU Jiao1HE Zhi-qiang2WANG Guo-hua3LIU Jin-xiang4School of Civil Engineering, University of South China, Hengyang 421001, Hunan, ChinaSchool of Civil Engineering, University of South China, Hengyang 421001, Hunan, ChinaSchool of Civil Engineering, University of South China, Hengyang 421001, Hunan, ChinaSchool of Civil Engineering, University of South China, Hengyang 421001, Hunan, ChinaSchool of Civil Engineering, University of South China, Hengyang 421001, Hunan, ChinaGraphite carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is a visible light responsive semiconductor material with the advantages of high stability, low cost, high adjustability of structure and property. With the continuous development of green and non-secondary pollution photocatalytic technology, g-C<sub>3</sub>N<sub>4</sub>has gradually become a research hotspot in the field of environment and energy science. Nevertheless, the bare g-C<sub>3</sub>N<sub>4</sub> exhibits relatively low photocatalytic efficiency, which is due to the rapid recombination of photogenerated charge carriers and low visible light utilization efficiency. Among many modification methods, heterogeneous coupling is considered to be an effective method to improve the photocatalytic performance of g-C<sub>3</sub>N<sub>4</sub>. In recent years, with different inorganic semiconductors, precious metals, and carbon materials, heterogeneously coupled with g-C<sub>3</sub>N<sub>4</sub>, the researchers promoted the transfer efficiency of photoelectrons in the photocatalytic system, broadened the absorption range of visible light of g-C<sub>3</sub>N<sub>4</sub>-based photocatalysts, and enhanced the catalytic stability and structure regulation of g-C<sub>3</sub>N<sub>4</sub>. The catalytic mechanism of heterogeneous photocatalysts and construction of heterogeneous photocatalytic system based on g-C<sub>3</sub>N<sub>4</sub> were summarized, the research progress of g-C<sub>3</sub>N<sub>4</sub>-based heterojunction in degradation of environmental pollutants was discussed. Finally, the prospect of designing excellent g-C<sub>3</sub>N<sub>4</sub>-based photocatalyst and their applications in photocatalytic degradation of dyes,organic pollutants and reduction of toxic heavy metals with excellent performance and its prospect in the field of environmental pollutant removal were prospected.http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2020.000285graphite carbon nitrideheterogeneous couplingphotocatalysisenvironmental pollutant |
| spellingShingle | GE Yu-jie WU Jiao HE Zhi-qiang WANG Guo-hua LIU Jin-xiang Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal Cailiao gongcheng graphite carbon nitride heterogeneous coupling photocatalysis environmental pollutant |
| title | Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal |
| title_full | Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal |
| title_fullStr | Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal |
| title_full_unstemmed | Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal |
| title_short | Research progress in preparation and application of g-C<sub>3</sub>N<sub>4</sub>-based heterogeneous photocatalyst for environmental pollutant removal |
| title_sort | research progress in preparation and application of g c sub 3 sub n sub 4 sub based heterogeneous photocatalyst for environmental pollutant removal |
| topic | graphite carbon nitride heterogeneous coupling photocatalysis environmental pollutant |
| url | http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2020.000285 |
| work_keys_str_mv | AT geyujie researchprogressinpreparationandapplicationofgcsub3subnsub4subbasedheterogeneousphotocatalystforenvironmentalpollutantremoval AT wujiao researchprogressinpreparationandapplicationofgcsub3subnsub4subbasedheterogeneousphotocatalystforenvironmentalpollutantremoval AT hezhiqiang researchprogressinpreparationandapplicationofgcsub3subnsub4subbasedheterogeneousphotocatalystforenvironmentalpollutantremoval AT wangguohua researchprogressinpreparationandapplicationofgcsub3subnsub4subbasedheterogeneousphotocatalystforenvironmentalpollutantremoval AT liujinxiang researchprogressinpreparationandapplicationofgcsub3subnsub4subbasedheterogeneousphotocatalystforenvironmentalpollutantremoval |