A systematic study of the dynamics of chain formation in electrorheological fluids

We report a systematic study of the dynamics of chain formation in electrorheological fluids using Brownian dynamics simulations. The parameters of the system such as applied electric field, polarizability, dipole moment, friction coefficient, and number density are expressed in reduced units and ch...

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Main Authors: Dávid Fertig, Dezső Boda, István Szalai
Format: Article
Language:English
Published: AIP Publishing LLC 2021-02-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/5.0037985
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author Dávid Fertig
Dezső Boda
István Szalai
author_facet Dávid Fertig
Dezső Boda
István Szalai
author_sort Dávid Fertig
collection DOAJ
description We report a systematic study of the dynamics of chain formation in electrorheological fluids using Brownian dynamics simulations. The parameters of the system such as applied electric field, polarizability, dipole moment, friction coefficient, and number density are expressed in reduced units and changed in a wide range in order to map the system’s behavior as a function of them. We define time constants obtained from bi-exponential fits to time dependence of various physical quantities such as dipolar energy, diffusion constant, and average chain length. The smaller time constant is associated with the formation of shorter chains (pairs, triplets, and so on), while the larger time constant is associated with the formation of longer chains in the regime of those that overarch the simulation cell. We use the approximation that the dipole moments are induced by the applied electric field only, as usual in the literature. However, we report preliminary results for the case when particle–particle polarization is also possible.
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spelling doaj.art-95d9b8e5eb7246578f1be2d1104b7ba02022-12-21T20:22:29ZengAIP Publishing LLCAIP Advances2158-32262021-02-01112025243025243-1510.1063/5.0037985A systematic study of the dynamics of chain formation in electrorheological fluidsDávid Fertig0Dezső Boda1István Szalai2Center for Natural Sciences, University of Pannonia, Egyetem u. 10, Veszprém 8200, HungaryCenter for Natural Sciences, University of Pannonia, Egyetem u. 10, Veszprém 8200, HungaryResearch Centre for Engineering Sciences, University of Pannonia, Egyetem u. 10, Veszprém 8200, HungaryWe report a systematic study of the dynamics of chain formation in electrorheological fluids using Brownian dynamics simulations. The parameters of the system such as applied electric field, polarizability, dipole moment, friction coefficient, and number density are expressed in reduced units and changed in a wide range in order to map the system’s behavior as a function of them. We define time constants obtained from bi-exponential fits to time dependence of various physical quantities such as dipolar energy, diffusion constant, and average chain length. The smaller time constant is associated with the formation of shorter chains (pairs, triplets, and so on), while the larger time constant is associated with the formation of longer chains in the regime of those that overarch the simulation cell. We use the approximation that the dipole moments are induced by the applied electric field only, as usual in the literature. However, we report preliminary results for the case when particle–particle polarization is also possible.http://dx.doi.org/10.1063/5.0037985
spellingShingle Dávid Fertig
Dezső Boda
István Szalai
A systematic study of the dynamics of chain formation in electrorheological fluids
AIP Advances
title A systematic study of the dynamics of chain formation in electrorheological fluids
title_full A systematic study of the dynamics of chain formation in electrorheological fluids
title_fullStr A systematic study of the dynamics of chain formation in electrorheological fluids
title_full_unstemmed A systematic study of the dynamics of chain formation in electrorheological fluids
title_short A systematic study of the dynamics of chain formation in electrorheological fluids
title_sort systematic study of the dynamics of chain formation in electrorheological fluids
url http://dx.doi.org/10.1063/5.0037985
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