Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching

Random quasi-phase matching (RQPM) in polycrystalline materials has been considered as an important technique for nonlinear optical frequency conversion, especially in wideband laser generation involving femtosecond lasers. In this paper, optical rectification (OR) based on RQPM in ZnSe ceramics was...

Full description

Bibliographic Details
Main Authors: Sijia Wang, Kai Zhong, Hongzhan Qiao, Fangjie Li, Jining Li, Degang Xu, Jianquan Yao
Format: Article
Language:English
Published: MDPI AG 2022-08-01
Series:Crystals
Subjects:
Online Access:https://www.mdpi.com/2073-4352/12/9/1188
_version_ 1797489743019114496
author Sijia Wang
Kai Zhong
Hongzhan Qiao
Fangjie Li
Jining Li
Degang Xu
Jianquan Yao
author_facet Sijia Wang
Kai Zhong
Hongzhan Qiao
Fangjie Li
Jining Li
Degang Xu
Jianquan Yao
author_sort Sijia Wang
collection DOAJ
description Random quasi-phase matching (RQPM) in polycrystalline materials has been considered as an important technique for nonlinear optical frequency conversion, especially in wideband laser generation involving femtosecond lasers. In this paper, optical rectification (OR) based on RQPM in ZnSe ceramics was investigated for the first time, which could convert ultrashort optical pulses to broadband terahertz waves. A theoretical model of RQPM OR was built, with which the effects of material grain size, thickness, pump wavelength and pump pulse duration on terahertz generation, were simulated and discussed. It was found that RQPM OR in ZnSe is indeed effective in terahertz generation but insensitive to the material grain size and pump wavelength RQPM OR is even better than traditional single crystals such as ZnTe in bandwidth and robustness. The results can be a reference to optimize the RQPM OR nonlinear process, and hopefully, this work will promote the application of costless polycrystalline materials in the hot field of terahertz generation.
first_indexed 2024-03-10T00:21:01Z
format Article
id doaj.art-97610307829f42a3a7e82f239068ef51
institution Directory Open Access Journal
issn 2073-4352
language English
last_indexed 2024-03-10T00:21:01Z
publishDate 2022-08-01
publisher MDPI AG
record_format Article
series Crystals
spelling doaj.art-97610307829f42a3a7e82f239068ef512023-11-23T15:42:49ZengMDPI AGCrystals2073-43522022-08-01129118810.3390/cryst12091188Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase MatchingSijia Wang0Kai Zhong1Hongzhan Qiao2Fangjie Li3Jining Li4Degang Xu5Jianquan Yao6Key Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaKey Laboratory of Optoelectronics Information Technology (Ministry of Education), School of Precision Instruments and Optoelectronics Engineering, Tianjin University, Tianjin 300072, ChinaRandom quasi-phase matching (RQPM) in polycrystalline materials has been considered as an important technique for nonlinear optical frequency conversion, especially in wideband laser generation involving femtosecond lasers. In this paper, optical rectification (OR) based on RQPM in ZnSe ceramics was investigated for the first time, which could convert ultrashort optical pulses to broadband terahertz waves. A theoretical model of RQPM OR was built, with which the effects of material grain size, thickness, pump wavelength and pump pulse duration on terahertz generation, were simulated and discussed. It was found that RQPM OR in ZnSe is indeed effective in terahertz generation but insensitive to the material grain size and pump wavelength RQPM OR is even better than traditional single crystals such as ZnTe in bandwidth and robustness. The results can be a reference to optimize the RQPM OR nonlinear process, and hopefully, this work will promote the application of costless polycrystalline materials in the hot field of terahertz generation.https://www.mdpi.com/2073-4352/12/9/1188random quasi-phase matchingpolycrystalline materialoptical rectificationterahertz wavesZnSe
spellingShingle Sijia Wang
Kai Zhong
Hongzhan Qiao
Fangjie Li
Jining Li
Degang Xu
Jianquan Yao
Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
Crystals
random quasi-phase matching
polycrystalline material
optical rectification
terahertz waves
ZnSe
title Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
title_full Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
title_fullStr Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
title_full_unstemmed Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
title_short Study of Optical Rectification in Polycrystalline Materials Based on Random Quasi-Phase Matching
title_sort study of optical rectification in polycrystalline materials based on random quasi phase matching
topic random quasi-phase matching
polycrystalline material
optical rectification
terahertz waves
ZnSe
url https://www.mdpi.com/2073-4352/12/9/1188
work_keys_str_mv AT sijiawang studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT kaizhong studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT hongzhanqiao studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT fangjieli studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT jiningli studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT degangxu studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching
AT jianquanyao studyofopticalrectificationinpolycrystallinematerialsbasedonrandomquasiphasematching