Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution
Abstract Waste-water pollution by radioactive elements such as uranium has emerged as a major issue that might seriously harm human health. Graphene oxide, graphene oxide nanoribbons, and sodium alginate nanocomposite aerogels (GO/GONRs/SA) were combined to create a novel nanocomposite using a modif...
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Nature Portfolio
2024-01-01
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Series: | Scientific Reports |
Online Access: | https://doi.org/10.1038/s41598-024-52043-1 |
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author | Ali A. Jabbar Dhia H. Hussain Kamal H. Latif Salim Albukhaty Adel Kareem Jasim Ghassan M. Sulaiman Mosleh M. Abomughaid |
author_facet | Ali A. Jabbar Dhia H. Hussain Kamal H. Latif Salim Albukhaty Adel Kareem Jasim Ghassan M. Sulaiman Mosleh M. Abomughaid |
author_sort | Ali A. Jabbar |
collection | DOAJ |
description | Abstract Waste-water pollution by radioactive elements such as uranium has emerged as a major issue that might seriously harm human health. Graphene oxide, graphene oxide nanoribbons, and sodium alginate nanocomposite aerogels (GO/GONRs/SA) were combined to create a novel nanocomposite using a modified Hummer's process and freeze-drying as an efficient adsorbent. Batch studies were conducted to determine the adsorption of uranium (VI) by aerogel. Aerogels composed of (GO/GONRs/SA) were used as an effective adsorbent for the removal of U (VI) from aqueous solution. Fourier transform infrared (FT-IR) spectroscopy, X-ray diffraction (XRD), scanning electron microscopy (SEM), and transmission electron microscopy (TEM) were used to describe the structure, morphologies, and characteristics of (GO/GONRs/SA) aerogels. The initial concentration of uranium (VI) and other environmental factors on U (VI) adsorption were investigated, period of contact, pH, and temperature. A pseudo-second-order kinetic model can be employed to characterize the kinetics of U (VI) adsorption onto aerogels. The Langmuir model could be applied to understand the adsorption isotherm, and the maximum adsorption capacity was 929.16 mg/g. The adsorption reaction is endothermic and occurs spontaneously. |
first_indexed | 2024-03-07T15:06:21Z |
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id | doaj.art-989dab92a31148e39378dea6bbd425fb |
institution | Directory Open Access Journal |
issn | 2045-2322 |
language | English |
last_indexed | 2024-03-07T15:06:21Z |
publishDate | 2024-01-01 |
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spelling | doaj.art-989dab92a31148e39378dea6bbd425fb2024-03-05T18:54:11ZengNature PortfolioScientific Reports2045-23222024-01-011411910.1038/s41598-024-52043-1Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solutionAli A. Jabbar0Dhia H. Hussain1Kamal H. Latif2Salim Albukhaty3Adel Kareem Jasim4Ghassan M. Sulaiman5Mosleh M. Abomughaid6College of Science/Chemistry Department, Mustansiriyah UniversityCollege of Science/Chemistry Department, Mustansiriyah UniversityCollege of Science/Chemistry Department, Mustansiriyah UniversityDepartment of Chemistry, College of Science, University of MisanDepartment of Chemistry, College of Science, University of MisanDivision of Biotechnology, Department of Applied Sciences, University of TechnologyDepartment of Medical Laboratory Sciences, College of Applied Medical Sciences, University of BishaAbstract Waste-water pollution by radioactive elements such as uranium has emerged as a major issue that might seriously harm human health. Graphene oxide, graphene oxide nanoribbons, and sodium alginate nanocomposite aerogels (GO/GONRs/SA) were combined to create a novel nanocomposite using a modified Hummer's process and freeze-drying as an efficient adsorbent. Batch studies were conducted to determine the adsorption of uranium (VI) by aerogel. Aerogels composed of (GO/GONRs/SA) were used as an effective adsorbent for the removal of U (VI) from aqueous solution. Fourier transform infrared (FT-IR) spectroscopy, X-ray diffraction (XRD), scanning electron microscopy (SEM), and transmission electron microscopy (TEM) were used to describe the structure, morphologies, and characteristics of (GO/GONRs/SA) aerogels. The initial concentration of uranium (VI) and other environmental factors on U (VI) adsorption were investigated, period of contact, pH, and temperature. A pseudo-second-order kinetic model can be employed to characterize the kinetics of U (VI) adsorption onto aerogels. The Langmuir model could be applied to understand the adsorption isotherm, and the maximum adsorption capacity was 929.16 mg/g. The adsorption reaction is endothermic and occurs spontaneously.https://doi.org/10.1038/s41598-024-52043-1 |
spellingShingle | Ali A. Jabbar Dhia H. Hussain Kamal H. Latif Salim Albukhaty Adel Kareem Jasim Ghassan M. Sulaiman Mosleh M. Abomughaid Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution Scientific Reports |
title | Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution |
title_full | Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution |
title_fullStr | Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution |
title_full_unstemmed | Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution |
title_short | Extremely efficient aerogels of graphene oxide/graphene oxide nanoribbons/sodium alginate for uranium removal from wastewater solution |
title_sort | extremely efficient aerogels of graphene oxide graphene oxide nanoribbons sodium alginate for uranium removal from wastewater solution |
url | https://doi.org/10.1038/s41598-024-52043-1 |
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