Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue
The discharge of dyes in the textile industry leads to several hazardous effects on the environment. One of the most effective methods on treating dye-contaminated wastewater is photocatalytic degradation. TiO2 has been widely used as a photocatalyst for wastewater treatment. Since the light absorpt...
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Format: | Article |
Language: | English |
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Taylor & Francis Group
2019-07-01
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Series: | Journal of Asian Ceramic Societies |
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Online Access: | http://dx.doi.org/10.1080/21870764.2019.1636929 |
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author | Syasya Nazifa Binti Saiful Amran Viona Wongso Nur Syakinah Abdul Halim Muhammad Khalid Husni Nonni Soraya Sambudi Muhammad Dzul Hakim Wirzal |
author_facet | Syasya Nazifa Binti Saiful Amran Viona Wongso Nur Syakinah Abdul Halim Muhammad Khalid Husni Nonni Soraya Sambudi Muhammad Dzul Hakim Wirzal |
author_sort | Syasya Nazifa Binti Saiful Amran |
collection | DOAJ |
description | The discharge of dyes in the textile industry leads to several hazardous effects on the environment. One of the most effective methods on treating dye-contaminated wastewater is photocatalytic degradation. TiO2 has been widely used as a photocatalyst for wastewater treatment. Since the light absorption of TiO2 is in the UV light range, however, doping of TiO2 with a non-metal or metal element is needed to improve its absorption in the visible light range. In this study, TiO2 photocatalyst was doped with carbon using sucrose as a carbon+e at ratios of 0.75:1 and 1:1. The surface area of TiO2 after doping with carbon improved to two times the TiO2 surface area. Additionally, the band gap energy of TiO2 was successfully reduced to 2.38 eV after doping with carbon. In order to avoid the secondary pollutant problems, the carbon-doped TiO2 was then immobilized with polyamide fibers at 1wt%, 2wt% and 3wt% to facilitate recollection of the photocatalyst. A photodegradation test was performed by degrading methylene blue under visible light irradiation using 70W halogen lamps with a total of 5 hours of time interval readings. The highest percentage degradation was recorded at 82.67% using immobilized 2wt% 1:1 carbon-doped TiO2 in polyamide fibers. |
first_indexed | 2024-12-14T11:43:53Z |
format | Article |
id | doaj.art-99ac99284c6f473f878405e6e3c2e8cf |
institution | Directory Open Access Journal |
issn | 2187-0764 |
language | English |
last_indexed | 2024-12-14T11:43:53Z |
publishDate | 2019-07-01 |
publisher | Taylor & Francis Group |
record_format | Article |
series | Journal of Asian Ceramic Societies |
spelling | doaj.art-99ac99284c6f473f878405e6e3c2e8cf2022-12-21T23:02:41ZengTaylor & Francis GroupJournal of Asian Ceramic Societies2187-07642019-07-017332133010.1080/21870764.2019.16369291636929Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blueSyasya Nazifa Binti Saiful Amran0Viona Wongso1Nur Syakinah Abdul Halim2Muhammad Khalid Husni3Nonni Soraya Sambudi4Muhammad Dzul Hakim Wirzal5Universiti Teknologi PETRONASUniversiti Teknologi PETRONASUniversiti Teknologi PETRONASUniversiti Teknologi PETRONASUniversiti Teknologi PETRONASUniversiti Teknologi PETRONASThe discharge of dyes in the textile industry leads to several hazardous effects on the environment. One of the most effective methods on treating dye-contaminated wastewater is photocatalytic degradation. TiO2 has been widely used as a photocatalyst for wastewater treatment. Since the light absorption of TiO2 is in the UV light range, however, doping of TiO2 with a non-metal or metal element is needed to improve its absorption in the visible light range. In this study, TiO2 photocatalyst was doped with carbon using sucrose as a carbon+e at ratios of 0.75:1 and 1:1. The surface area of TiO2 after doping with carbon improved to two times the TiO2 surface area. Additionally, the band gap energy of TiO2 was successfully reduced to 2.38 eV after doping with carbon. In order to avoid the secondary pollutant problems, the carbon-doped TiO2 was then immobilized with polyamide fibers at 1wt%, 2wt% and 3wt% to facilitate recollection of the photocatalyst. A photodegradation test was performed by degrading methylene blue under visible light irradiation using 70W halogen lamps with a total of 5 hours of time interval readings. The highest percentage degradation was recorded at 82.67% using immobilized 2wt% 1:1 carbon-doped TiO2 in polyamide fibers.http://dx.doi.org/10.1080/21870764.2019.1636929Titanium dioxidepolyamideelectrospinningcarbon-doped TiO2methylene blue |
spellingShingle | Syasya Nazifa Binti Saiful Amran Viona Wongso Nur Syakinah Abdul Halim Muhammad Khalid Husni Nonni Soraya Sambudi Muhammad Dzul Hakim Wirzal Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue Journal of Asian Ceramic Societies Titanium dioxide polyamide electrospinning carbon-doped TiO2 methylene blue |
title | Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue |
title_full | Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue |
title_fullStr | Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue |
title_full_unstemmed | Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue |
title_short | Immobilized carbon-doped TiO2 in polyamide fibers for the degradation of methylene blue |
title_sort | immobilized carbon doped tio2 in polyamide fibers for the degradation of methylene blue |
topic | Titanium dioxide polyamide electrospinning carbon-doped TiO2 methylene blue |
url | http://dx.doi.org/10.1080/21870764.2019.1636929 |
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