Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan

The impact of Brown Carbon (BrC) to aerosol light absorption has been paid more attention recently and there are a large number of studies showing that the influence of BrC on radiative forcing should not be ignored. BrC also acts as an important component of haze pollution which is occurring freque...

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Main Authors: Yuyao Zhang, Yingying Ma, Wei Gong
Format: Article
Language:English
Published: Taylor & Francis Group 2017-10-01
Series:Geo-spatial Information Science
Subjects:
Online Access:http://dx.doi.org/10.1080/10095020.2017.1394660
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author Yuyao Zhang
Yingying Ma
Wei Gong
author_facet Yuyao Zhang
Yingying Ma
Wei Gong
author_sort Yuyao Zhang
collection DOAJ
description The impact of Brown Carbon (BrC) to aerosol light absorption has been paid more attention recently and there are a large number of studies showing that the influence of BrC on radiative forcing should not be ignored. BrC also acts as an important component of haze pollution which is occurring frequently in Wuhan, China. Therefore, it is essential to estimate their optical properties, composition, and mass concentration. Considering most haze pollution happens during the coldest time, we retrieved BrC columnar content during winter in Wuhan for the first time. Our method bases on the fact that BrC showed the strong spectral dependence on UV-light absorption. Using this method, we found that BrC makes up the small proportions of total aerosol volume (less than 10%). In the winter of 2011, we retrieved the daily-averaged columnar-integrated mass concentration of BrC on clear day is 4.353 mg/m2 while that of haze day is 12.750 mg/m2. According to the sensitivity study, we found that the results highly relied on the assumed aerosol refractive index. To reduce the uncertainty of this approach, we need to gain a better understanding of the temporal variability of the radiation absorbing components of these aerosols in the future.
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spelling doaj.art-99bb4a68f5ec4183b762cf57d3c3a5802022-12-22T03:06:51ZengTaylor & Francis GroupGeo-spatial Information Science1009-50201993-51532017-10-0120431932410.1080/10095020.2017.13946601394660Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of WuhanYuyao Zhang0Yingying Ma1Wei Gong2Wuhan UniversityWuhan UniversityWuhan UniversityThe impact of Brown Carbon (BrC) to aerosol light absorption has been paid more attention recently and there are a large number of studies showing that the influence of BrC on radiative forcing should not be ignored. BrC also acts as an important component of haze pollution which is occurring frequently in Wuhan, China. Therefore, it is essential to estimate their optical properties, composition, and mass concentration. Considering most haze pollution happens during the coldest time, we retrieved BrC columnar content during winter in Wuhan for the first time. Our method bases on the fact that BrC showed the strong spectral dependence on UV-light absorption. Using this method, we found that BrC makes up the small proportions of total aerosol volume (less than 10%). In the winter of 2011, we retrieved the daily-averaged columnar-integrated mass concentration of BrC on clear day is 4.353 mg/m2 while that of haze day is 12.750 mg/m2. According to the sensitivity study, we found that the results highly relied on the assumed aerosol refractive index. To reduce the uncertainty of this approach, we need to gain a better understanding of the temporal variability of the radiation absorbing components of these aerosols in the future.http://dx.doi.org/10.1080/10095020.2017.1394660Brown Carbon (BrC)Black Carbon (BC)aerosol complex refractive index
spellingShingle Yuyao Zhang
Yingying Ma
Wei Gong
Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
Geo-spatial Information Science
Brown Carbon (BrC)
Black Carbon (BC)
aerosol complex refractive index
title Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
title_full Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
title_fullStr Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
title_full_unstemmed Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
title_short Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan
title_sort retrieval of brown carbon based on the aerosol complex refractive indices in the winter of wuhan
topic Brown Carbon (BrC)
Black Carbon (BC)
aerosol complex refractive index
url http://dx.doi.org/10.1080/10095020.2017.1394660
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AT yingyingma retrievalofbrowncarbonbasedontheaerosolcomplexrefractiveindicesinthewinterofwuhan
AT weigong retrievalofbrowncarbonbasedontheaerosolcomplexrefractiveindicesinthewinterofwuhan