Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects

Materials such as silicon, copper, gold, and aluminum exhibit strong absorption and scattering characterization under short-pulsed laser irradiation. Due to the photoelastic effect and thermoelastic relaxation, the focal area may induce a local modulation in the refractive index, which can be detect...

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Main Authors: Zhiying Xia, Bin Ni, Ruijie Hou, Yang Zhang, Lianping Hou, Jamie Jiangmin Hou, John H. Marsh, Xuefeng Liu, Jichuan Xiong
Format: Article
Language:English
Published: MDPI AG 2022-06-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/12/12/6256
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author Zhiying Xia
Bin Ni
Ruijie Hou
Yang Zhang
Lianping Hou
Jamie Jiangmin Hou
John H. Marsh
Xuefeng Liu
Jichuan Xiong
author_facet Zhiying Xia
Bin Ni
Ruijie Hou
Yang Zhang
Lianping Hou
Jamie Jiangmin Hou
John H. Marsh
Xuefeng Liu
Jichuan Xiong
author_sort Zhiying Xia
collection DOAJ
description Materials such as silicon, copper, gold, and aluminum exhibit strong absorption and scattering characterization under short-pulsed laser irradiation. Due to the photoelastic effect and thermoelastic relaxation, the focal area may induce a local modulation in the refractive index, which can be detected with the intensity reflection coefficient perturbation. Normally, the thermal effect causes a weak refractive index change and is negligible, compared with the pressure-induced effect in most photoacoustic analytical systems. In this study, we present a theoretical model with the whole process of absorbed energy conversion analysis for the refractive index perturbation induced by both thermal effect and photoacoustic pressure. In this model, data analysis was carried out on the transformation of the energy absorbed by the sample into heat and stress. To prove the feasibility of this model, numerical simulation was performed for the photothermal and photoacoustic effects under different incident intensities using the finite element method. Experiment results on silicon and carbon fiber verified that the refractive index change induced by the photothermal effect can be detected and be incorporated with pressure-induced refractive index change. The simulation results showed very good agreement with the results of the experiments. The main aim of this study was to further understand the absorption and conversion process of short-pulsed light energy and the resulting photothermal and photoacoustic effects.
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spelling doaj.art-9a040b232353481da21a7761b69d26422023-11-23T15:30:30ZengMDPI AGApplied Sciences2076-34172022-06-011212625610.3390/app12126256Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal EffectsZhiying Xia0Bin Ni1Ruijie Hou2Yang Zhang3Lianping Hou4Jamie Jiangmin Hou5John H. Marsh6Xuefeng Liu7Jichuan Xiong8School of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaSchool of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaSchool of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaSchool of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaJames Watt School of Engineering, University of Glasgow, Glasgow G12 8QQ, UKThe Royal College of Surgeons of Edinburgh, Nicolson Street, Edinburgh EH8 9DW, UKJames Watt School of Engineering, University of Glasgow, Glasgow G12 8QQ, UKSchool of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaSchool of Electronic and Optical Engineering, Nanjing University of Science and Technology, Nanjing 210094, ChinaMaterials such as silicon, copper, gold, and aluminum exhibit strong absorption and scattering characterization under short-pulsed laser irradiation. Due to the photoelastic effect and thermoelastic relaxation, the focal area may induce a local modulation in the refractive index, which can be detected with the intensity reflection coefficient perturbation. Normally, the thermal effect causes a weak refractive index change and is negligible, compared with the pressure-induced effect in most photoacoustic analytical systems. In this study, we present a theoretical model with the whole process of absorbed energy conversion analysis for the refractive index perturbation induced by both thermal effect and photoacoustic pressure. In this model, data analysis was carried out on the transformation of the energy absorbed by the sample into heat and stress. To prove the feasibility of this model, numerical simulation was performed for the photothermal and photoacoustic effects under different incident intensities using the finite element method. Experiment results on silicon and carbon fiber verified that the refractive index change induced by the photothermal effect can be detected and be incorporated with pressure-induced refractive index change. The simulation results showed very good agreement with the results of the experiments. The main aim of this study was to further understand the absorption and conversion process of short-pulsed light energy and the resulting photothermal and photoacoustic effects.https://www.mdpi.com/2076-3417/12/12/6256refractive indexphotothermal effectphotoacoustic effectfinite element method
spellingShingle Zhiying Xia
Bin Ni
Ruijie Hou
Yang Zhang
Lianping Hou
Jamie Jiangmin Hou
John H. Marsh
Xuefeng Liu
Jichuan Xiong
Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
Applied Sciences
refractive index
photothermal effect
photoacoustic effect
finite element method
title Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
title_full Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
title_fullStr Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
title_full_unstemmed Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
title_short Temporal Evolution of Refractive Index Induced by Short Laser Pulses Accounting for Both Photoacoustic and Photothermal Effects
title_sort temporal evolution of refractive index induced by short laser pulses accounting for both photoacoustic and photothermal effects
topic refractive index
photothermal effect
photoacoustic effect
finite element method
url https://www.mdpi.com/2076-3417/12/12/6256
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