Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals

Abstract The stability of ferroelectric domain patterns at the nanoscale has been a topic of much interest for many years. We investigated the relaxation of the polarized state created by application of a local electric field using a conductive tip of a scanning probe microscope for the model uniaxi...

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Main Authors: V. Ya. Shur, V. A. Shikhova, D. O. Alikin, V. A. Lebedev, L. I. Ivleva, J. Dec, D. C. Lupascu, V. V. Shvartsman
Format: Article
Language:English
Published: Nature Portfolio 2017-03-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-017-00172-1
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author V. Ya. Shur
V. A. Shikhova
D. O. Alikin
V. A. Lebedev
L. I. Ivleva
J. Dec
D. C. Lupascu
V. V. Shvartsman
author_facet V. Ya. Shur
V. A. Shikhova
D. O. Alikin
V. A. Lebedev
L. I. Ivleva
J. Dec
D. C. Lupascu
V. V. Shvartsman
author_sort V. Ya. Shur
collection DOAJ
description Abstract The stability of ferroelectric domain patterns at the nanoscale has been a topic of much interest for many years. We investigated the relaxation of the polarized state created by application of a local electric field using a conductive tip of a scanning probe microscope for the model uniaxial relaxor system SrxBa1−xNb2O6 (SBN) in its pure and Ce-doped form. The temporal relaxation of the induced PFM contrast was measured at various temperatures. The average value of the induced contrast decreases during heating for all investigated crystals. Below the freezing temperature the induced state remains stable after an initial relaxation. Above the freezing temperature the induced state is unstable and gradually decays with time. The stability of the induced state is strongly affected by the measuring conditions, so continuous scanning results in a faster decay of the poled domain. The obtained effects are attributed to a decrease of the induced polarization and backswitching of the polarized area under the action of the depolarization field.
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spelling doaj.art-9af5ca9f695042069fa89a41739792132022-12-21T22:56:12ZengNature PortfolioScientific Reports2045-23222017-03-01711710.1038/s41598-017-00172-1Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single CrystalsV. Ya. Shur0V. A. Shikhova1D. O. Alikin2V. A. Lebedev3L. I. Ivleva4J. Dec5D. C. Lupascu6V. V. Shvartsman7School of Natural Sciences and Mathematics, Ural Federal UniversitySchool of Natural Sciences and Mathematics, Ural Federal UniversitySchool of Natural Sciences and Mathematics, Ural Federal UniversityFaculty of Materials Science, Lomonosov Moscow State UniversityProkhorov General Physics Institute, Russian Academy of SciencesInstitute of Materials Science, University of SilesiaInstitute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-EssenInstitute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-EssenAbstract The stability of ferroelectric domain patterns at the nanoscale has been a topic of much interest for many years. We investigated the relaxation of the polarized state created by application of a local electric field using a conductive tip of a scanning probe microscope for the model uniaxial relaxor system SrxBa1−xNb2O6 (SBN) in its pure and Ce-doped form. The temporal relaxation of the induced PFM contrast was measured at various temperatures. The average value of the induced contrast decreases during heating for all investigated crystals. Below the freezing temperature the induced state remains stable after an initial relaxation. Above the freezing temperature the induced state is unstable and gradually decays with time. The stability of the induced state is strongly affected by the measuring conditions, so continuous scanning results in a faster decay of the poled domain. The obtained effects are attributed to a decrease of the induced polarization and backswitching of the polarized area under the action of the depolarization field.https://doi.org/10.1038/s41598-017-00172-1
spellingShingle V. Ya. Shur
V. A. Shikhova
D. O. Alikin
V. A. Lebedev
L. I. Ivleva
J. Dec
D. C. Lupascu
V. V. Shvartsman
Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
Scientific Reports
title Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
title_full Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
title_fullStr Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
title_full_unstemmed Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
title_short Temperature Effect on the Stability of the Polarized State Created by Local Electric Fields in Strontium Barium Niobate Single Crystals
title_sort temperature effect on the stability of the polarized state created by local electric fields in strontium barium niobate single crystals
url https://doi.org/10.1038/s41598-017-00172-1
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