The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses
Single bubble sonoluminescence (SBSL) is the phenomenon of synchronous light emission due to the violent collapse of a single spherical bubble in a liquid, driven by an ultrasonic field. During the bubble collapse, matter inside the bubble reaches extreme conditions of several gigapascals and temper...
Main Authors: | , , , , , , , , , , , , , , , |
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IOP Publishing
2024-01-01
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Series: | New Journal of Physics |
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Online Access: | https://doi.org/10.1088/1367-2630/ad295b |
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author | Hannes P Hoeppe Markus Osterhoff Atiyeh Aghel Maleki Juan M Rosselló Malte Vassholz Johannes Hagemann Thea Engler Daniel Schwarz Angel Rodriguez-Fernandez Ulrike Boesenberg Johannes Möller Roman Shayduk Jörg Hallmann Anders Madsen Robert Mettin Tim Salditt |
author_facet | Hannes P Hoeppe Markus Osterhoff Atiyeh Aghel Maleki Juan M Rosselló Malte Vassholz Johannes Hagemann Thea Engler Daniel Schwarz Angel Rodriguez-Fernandez Ulrike Boesenberg Johannes Möller Roman Shayduk Jörg Hallmann Anders Madsen Robert Mettin Tim Salditt |
author_sort | Hannes P Hoeppe |
collection | DOAJ |
description | Single bubble sonoluminescence (SBSL) is the phenomenon of synchronous light emission due to the violent collapse of a single spherical bubble in a liquid, driven by an ultrasonic field. During the bubble collapse, matter inside the bubble reaches extreme conditions of several gigapascals and temperatures on the order of 10000 K, leading to picosecond flashes of visible light. To this day, details regarding the energy focusing mechanism rely on simulations due to the fast dynamics of the bubble collapse and spatial scales below the optical resolution limit. In this work we present phase-contrast holographic imaging with single x-ray free-electron laser (XFEL) pulses of a SBSL cavitation bubble in water. X-rays probe the electron density structure and by that provide a uniquely new view on the bubble interior and its collapse dynamics. The involved fast time-scales are accessed by sub-100 fs XFEL pulses and a custom synchronization scheme for the bubble oscillator. We find that during the whole oscillation cycle the bubble’s density profile can be well described by a simple step-like structure, with the radius R following the dynamics of the Gilmore model. The quantitatively measured internal density and width of the boundary layer exhibit a large variance. Smallest reconstructed bubble sizes reach down to $R\simeq0.8\,\mu \mathrm{m}$ , and are consistent with spherical symmetry. While we here achieved a spatial resolution of a few 100 nm, the visibility of the bubble and its internal structure is limited by the total x-ray phase shift which can be scaled with experimental parameters. |
first_indexed | 2024-03-07T15:38:50Z |
format | Article |
id | doaj.art-9bb35900bebd452f880b6d1be6ad92b7 |
institution | Directory Open Access Journal |
issn | 1367-2630 |
language | English |
last_indexed | 2024-03-07T15:38:50Z |
publishDate | 2024-01-01 |
publisher | IOP Publishing |
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series | New Journal of Physics |
spelling | doaj.art-9bb35900bebd452f880b6d1be6ad92b72024-03-05T09:16:05ZengIOP PublishingNew Journal of Physics1367-26302024-01-0126303300210.1088/1367-2630/ad295bThe collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulsesHannes P Hoeppe0https://orcid.org/0000-0002-4341-5121Markus Osterhoff1https://orcid.org/0000-0002-7865-515XAtiyeh Aghel Maleki2https://orcid.org/0009-0001-8771-1707Juan M Rosselló3https://orcid.org/0000-0001-7005-9452Malte Vassholz4https://orcid.org/0000-0002-0368-8782Johannes Hagemann5https://orcid.org/0000-0003-2768-9496Thea Engler6https://orcid.org/0009-0006-8183-3603Daniel Schwarz7Angel Rodriguez-Fernandez8https://orcid.org/0000-0003-0587-5263Ulrike Boesenberg9https://orcid.org/0000-0002-1195-6329Johannes Möller10https://orcid.org/0000-0001-8363-9077Roman Shayduk11https://orcid.org/0000-0002-3577-8918Jörg Hallmann12https://orcid.org/0000-0002-1996-397XAnders Madsen13https://orcid.org/0000-0001-6594-1029Robert Mettin14https://orcid.org/0000-0003-1780-5131Tim Salditt15https://orcid.org/0000-0003-4636-0813Institut für Röntgenphysik, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanyInstitut für Röntgenphysik, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanyDrittes Physikalisches Institut, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanyDrittes Physikalisches Institut, Georg-August-Universität Göttingen , D-37077 Göttingen, Germany; Faculty of Mechanical Engineering, University of Ljubljana , SVN-1000 Ljubljana, SloveniaInstitut für Röntgenphysik, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanyHelmholtz Imaging Platform, Deutsches Elektronen-Synchrotron DESY , D-22607 Hamburg, Germany; CXNS—Center for X-ray and Nano Science, Deutsches Elektronen-Synchrotron DESY , D-22607 Hamburg, GermanyHelmholtz Imaging Platform, Deutsches Elektronen-Synchrotron DESY , D-22607 Hamburg, Germany; CXNS—Center for X-ray and Nano Science, Deutsches Elektronen-Synchrotron DESY , D-22607 Hamburg, GermanyCXNS—Center for X-ray and Nano Science, Deutsches Elektronen-Synchrotron DESY , D-22607 Hamburg, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyEuropean X-ray Free-Electron Laser Facility , D-22869 Schenefeld, GermanyDrittes Physikalisches Institut, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanyInstitut für Röntgenphysik, Georg-August-Universität Göttingen , D-37077 Göttingen, GermanySingle bubble sonoluminescence (SBSL) is the phenomenon of synchronous light emission due to the violent collapse of a single spherical bubble in a liquid, driven by an ultrasonic field. During the bubble collapse, matter inside the bubble reaches extreme conditions of several gigapascals and temperatures on the order of 10000 K, leading to picosecond flashes of visible light. To this day, details regarding the energy focusing mechanism rely on simulations due to the fast dynamics of the bubble collapse and spatial scales below the optical resolution limit. In this work we present phase-contrast holographic imaging with single x-ray free-electron laser (XFEL) pulses of a SBSL cavitation bubble in water. X-rays probe the electron density structure and by that provide a uniquely new view on the bubble interior and its collapse dynamics. The involved fast time-scales are accessed by sub-100 fs XFEL pulses and a custom synchronization scheme for the bubble oscillator. We find that during the whole oscillation cycle the bubble’s density profile can be well described by a simple step-like structure, with the radius R following the dynamics of the Gilmore model. The quantitatively measured internal density and width of the boundary layer exhibit a large variance. Smallest reconstructed bubble sizes reach down to $R\simeq0.8\,\mu \mathrm{m}$ , and are consistent with spherical symmetry. While we here achieved a spatial resolution of a few 100 nm, the visibility of the bubble and its internal structure is limited by the total x-ray phase shift which can be scaled with experimental parameters.https://doi.org/10.1088/1367-2630/ad295bx-ray holographysingle-bubble sonoluminescencebubble collapse dynamicsacoustic trapsingle-pulse imagingx-ray free-electron laser |
spellingShingle | Hannes P Hoeppe Markus Osterhoff Atiyeh Aghel Maleki Juan M Rosselló Malte Vassholz Johannes Hagemann Thea Engler Daniel Schwarz Angel Rodriguez-Fernandez Ulrike Boesenberg Johannes Möller Roman Shayduk Jörg Hallmann Anders Madsen Robert Mettin Tim Salditt The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses New Journal of Physics x-ray holography single-bubble sonoluminescence bubble collapse dynamics acoustic trap single-pulse imaging x-ray free-electron laser |
title | The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses |
title_full | The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses |
title_fullStr | The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses |
title_full_unstemmed | The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses |
title_short | The collapse of a sonoluminescent cavitation bubble imaged with X-ray free-electron laser pulses |
title_sort | collapse of a sonoluminescent cavitation bubble imaged with x ray free electron laser pulses |
topic | x-ray holography single-bubble sonoluminescence bubble collapse dynamics acoustic trap single-pulse imaging x-ray free-electron laser |
url | https://doi.org/10.1088/1367-2630/ad295b |
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