Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells

Manipulation of the performance of the random lasers from dye-doped nematic liquid crystals with TiN nanoparticles in non-oriented cells is studied. The experimental results show that the introduction of TiN nanoparticles into dye-doped nematic liquid crystals significantly reduces the threshold of...

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Main Authors: Yuan Wan, Luogen Deng
Format: Article
Language:English
Published: MDPI AG 2019-12-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/10/1/199
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author Yuan Wan
Luogen Deng
author_facet Yuan Wan
Luogen Deng
author_sort Yuan Wan
collection DOAJ
description Manipulation of the performance of the random lasers from dye-doped nematic liquid crystals with TiN nanoparticles in non-oriented cells is studied. The experimental results show that the introduction of TiN nanoparticles into dye-doped nematic liquid crystals significantly reduces the threshold of random lasing due to the localized surface plasmon resonance of TiN nanoparticles. The emission spectrum of random lasers can be controlled by the shape of the pump spot. The threshold of random lasers increases with the decrease of the length of pump stripe. In order to obtain the emission spectrum with fine discrete sharp peaks, the narrow pump stripe is more effective than the circular pump spot. When the pump area is more like a circle, the emission spectrum is more like an amplified spontaneous emission. The underlying mechanisms of these phenomena are discussed in detail. This study provides a promising platform for designing the high-quality and low-threshold random lasers which can be controlled by the shape of the pump spot.
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spelling doaj.art-9c36653a9c214ec5a4e6f6b72dcf1e4b2022-12-22T03:41:19ZengMDPI AGApplied Sciences2076-34172019-12-0110119910.3390/app10010199app10010199Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented CellsYuan Wan0Luogen Deng1School of Physics, Beijing Institute of Technology, Beijing 100081, ChinaSchool of Physics, Beijing Institute of Technology, Beijing 100081, ChinaManipulation of the performance of the random lasers from dye-doped nematic liquid crystals with TiN nanoparticles in non-oriented cells is studied. The experimental results show that the introduction of TiN nanoparticles into dye-doped nematic liquid crystals significantly reduces the threshold of random lasing due to the localized surface plasmon resonance of TiN nanoparticles. The emission spectrum of random lasers can be controlled by the shape of the pump spot. The threshold of random lasers increases with the decrease of the length of pump stripe. In order to obtain the emission spectrum with fine discrete sharp peaks, the narrow pump stripe is more effective than the circular pump spot. When the pump area is more like a circle, the emission spectrum is more like an amplified spontaneous emission. The underlying mechanisms of these phenomena are discussed in detail. This study provides a promising platform for designing the high-quality and low-threshold random lasers which can be controlled by the shape of the pump spot.https://www.mdpi.com/2076-3417/10/1/199random laserstin nanoparticleslocalized surface plasmon resonancemultiple scattering
spellingShingle Yuan Wan
Luogen Deng
Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
Applied Sciences
random lasers
tin nanoparticles
localized surface plasmon resonance
multiple scattering
title Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
title_full Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
title_fullStr Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
title_full_unstemmed Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
title_short Pump-Controlled Plasmonic Random Lasers from Dye-Doped Nematic Liquid Crystals with TiN Nanoparticles in Non-Oriented Cells
title_sort pump controlled plasmonic random lasers from dye doped nematic liquid crystals with tin nanoparticles in non oriented cells
topic random lasers
tin nanoparticles
localized surface plasmon resonance
multiple scattering
url https://www.mdpi.com/2076-3417/10/1/199
work_keys_str_mv AT yuanwan pumpcontrolledplasmonicrandomlasersfromdyedopednematicliquidcrystalswithtinnanoparticlesinnonorientedcells
AT luogendeng pumpcontrolledplasmonicrandomlasersfromdyedopednematicliquidcrystalswithtinnanoparticlesinnonorientedcells