Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate

Active particles have been regarded as the key models to mimic and understand the complex systems of nature. Although chemical and field-powered active particles have received wide attentions, light-programmed actuation with long-range interaction and high throughput remains elusive. Here, we utiliz...

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Main Authors: Fangfang Deng, Juntao Chen, Junxiang Xiang, Yong Li, Yan Qiao, Ze Liu, Tao Ding
Format: Article
Language:English
Published: American Association for the Advancement of Science (AAAS) 2023-01-01
Series:Research
Online Access:https://spj.science.org/doi/10.34133/research.0020
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author Fangfang Deng
Juntao Chen
Junxiang Xiang
Yong Li
Yan Qiao
Ze Liu
Tao Ding
author_facet Fangfang Deng
Juntao Chen
Junxiang Xiang
Yong Li
Yan Qiao
Ze Liu
Tao Ding
author_sort Fangfang Deng
collection DOAJ
description Active particles have been regarded as the key models to mimic and understand the complex systems of nature. Although chemical and field-powered active particles have received wide attentions, light-programmed actuation with long-range interaction and high throughput remains elusive. Here, we utilize photothermal active plasmonic substrate made of porous anodic aluminum oxide filled with Au nanoparticles and poly(N-isopropylacrylamide) (PNIPAM) to optically oscillate silica beads with robust reversibility. The thermal gradient generated by the laser beam incurs the phase change of PNIPAM, producing gradient of surface forces and large volume changes within the complex system. The dynamic evolution of phase change and water diffusion in PNIPAM films result in bistate locomotion of silica beads, which can be programmed by modulating the laser beam. This light-programmed bistate colloidal actuation provides promising opportunity to control and mimic the natural complex systems.
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spelling doaj.art-9c7aeb968c714faf9d5ee428b2e835d52024-03-03T06:58:43ZengAmerican Association for the Advancement of Science (AAAS)Research2639-52742023-01-01610.34133/research.0020Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic SubstrateFangfang Deng0Juntao Chen1Junxiang Xiang2Yong Li3Yan Qiao4Ze Liu5Tao Ding6Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education of China, School of Physics and Technology, Wuhan University, Wuhan 430072, China.Department of Engineering Mechanics, School of Civil Engineering, Wuhan University, Wuhan, Hubei 430072, China.Department of Engineering Mechanics, School of Civil Engineering, Wuhan University, Wuhan, Hubei 430072, China.Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education of China, School of Physics and Technology, Wuhan University, Wuhan 430072, China.Beijing National Laboratory for Molecular Sciences (BNLMS), Laboratory of Polymer Physics and Chemistry, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China.Department of Engineering Mechanics, School of Civil Engineering, Wuhan University, Wuhan, Hubei 430072, China.Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education of China, School of Physics and Technology, Wuhan University, Wuhan 430072, China.Active particles have been regarded as the key models to mimic and understand the complex systems of nature. Although chemical and field-powered active particles have received wide attentions, light-programmed actuation with long-range interaction and high throughput remains elusive. Here, we utilize photothermal active plasmonic substrate made of porous anodic aluminum oxide filled with Au nanoparticles and poly(N-isopropylacrylamide) (PNIPAM) to optically oscillate silica beads with robust reversibility. The thermal gradient generated by the laser beam incurs the phase change of PNIPAM, producing gradient of surface forces and large volume changes within the complex system. The dynamic evolution of phase change and water diffusion in PNIPAM films result in bistate locomotion of silica beads, which can be programmed by modulating the laser beam. This light-programmed bistate colloidal actuation provides promising opportunity to control and mimic the natural complex systems.https://spj.science.org/doi/10.34133/research.0020
spellingShingle Fangfang Deng
Juntao Chen
Junxiang Xiang
Yong Li
Yan Qiao
Ze Liu
Tao Ding
Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
Research
title Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
title_full Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
title_fullStr Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
title_full_unstemmed Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
title_short Light-Programmed Bistate Colloidal Actuation Based on Photothermal Active Plasmonic Substrate
title_sort light programmed bistate colloidal actuation based on photothermal active plasmonic substrate
url https://spj.science.org/doi/10.34133/research.0020
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AT yanqiao lightprogrammedbistatecolloidalactuationbasedonphotothermalactiveplasmonicsubstrate
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