Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells

Abstract Large-area polydimethylsiloxane (PDMS) films with variably sized moth-eye structures were fabricated to improve the efficiency of perovskite solar cells. An approach that incorporated photolithography, bilayer PDMS deposition and replication was used in the fabrication process. By simply at...

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Main Authors: Min-cheol Kim, Segeun Jang, Jiwoo Choi, Seong Min Kang, Mansoo Choi
Format: Article
Language:English
Published: SpringerOpen 2019-06-01
Series:Nano-Micro Letters
Subjects:
Online Access:http://link.springer.com/article/10.1007/s40820-019-0284-y
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author Min-cheol Kim
Segeun Jang
Jiwoo Choi
Seong Min Kang
Mansoo Choi
author_facet Min-cheol Kim
Segeun Jang
Jiwoo Choi
Seong Min Kang
Mansoo Choi
author_sort Min-cheol Kim
collection DOAJ
description Abstract Large-area polydimethylsiloxane (PDMS) films with variably sized moth-eye structures were fabricated to improve the efficiency of perovskite solar cells. An approach that incorporated photolithography, bilayer PDMS deposition and replication was used in the fabrication process. By simply attaching the moth-eye PDMS films to the transparent substrates of perovskite solar cells, the optical properties of the devices could be tuned by changing the size of the moth-eye structures. The device with 300-nm moth-eye PDMS films greatly enhanced power conversion efficiency of ~ 21% due to the antireflective effect of the moth-eye structure. Furthermore, beautiful coloration was observed on the 1000-nm moth-eye PDMS films through optical interference caused by the diffraction grating effect. Our results imply that moth-eye PDMS films can greatly enhance the efficiency of perovskite solar cells and building-integrated photovoltaics.
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spelling doaj.art-9ca61fa9b3ef48638c7cfe4741161c7d2022-12-22T03:50:17ZengSpringerOpenNano-Micro Letters2311-67062150-55512019-06-0111111010.1007/s40820-019-0284-yMoth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar CellsMin-cheol Kim0Segeun Jang1Jiwoo Choi2Seong Min Kang3Mansoo Choi4Global Frontier Center for Multiscale Energy Systems, Seoul National UniversityDepartment of Mechanical Engineering, Hanbat National UniversityGlobal Frontier Center for Multiscale Energy Systems, Seoul National UniversityDepartment of Mechanical Engineering, Chungnam National UniversityGlobal Frontier Center for Multiscale Energy Systems, Seoul National UniversityAbstract Large-area polydimethylsiloxane (PDMS) films with variably sized moth-eye structures were fabricated to improve the efficiency of perovskite solar cells. An approach that incorporated photolithography, bilayer PDMS deposition and replication was used in the fabrication process. By simply attaching the moth-eye PDMS films to the transparent substrates of perovskite solar cells, the optical properties of the devices could be tuned by changing the size of the moth-eye structures. The device with 300-nm moth-eye PDMS films greatly enhanced power conversion efficiency of ~ 21% due to the antireflective effect of the moth-eye structure. Furthermore, beautiful coloration was observed on the 1000-nm moth-eye PDMS films through optical interference caused by the diffraction grating effect. Our results imply that moth-eye PDMS films can greatly enhance the efficiency of perovskite solar cells and building-integrated photovoltaics.http://link.springer.com/article/10.1007/s40820-019-0284-yPolydimethylsiloxane filmsMoth-eyePhotolithographyPerovskite solar cellsPhotovoltaic
spellingShingle Min-cheol Kim
Segeun Jang
Jiwoo Choi
Seong Min Kang
Mansoo Choi
Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
Nano-Micro Letters
Polydimethylsiloxane films
Moth-eye
Photolithography
Perovskite solar cells
Photovoltaic
title Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
title_full Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
title_fullStr Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
title_full_unstemmed Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
title_short Moth-eye Structured Polydimethylsiloxane Films for High-Efficiency Perovskite Solar Cells
title_sort moth eye structured polydimethylsiloxane films for high efficiency perovskite solar cells
topic Polydimethylsiloxane films
Moth-eye
Photolithography
Perovskite solar cells
Photovoltaic
url http://link.springer.com/article/10.1007/s40820-019-0284-y
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AT segeunjang motheyestructuredpolydimethylsiloxanefilmsforhighefficiencyperovskitesolarcells
AT jiwoochoi motheyestructuredpolydimethylsiloxanefilmsforhighefficiencyperovskitesolarcells
AT seongminkang motheyestructuredpolydimethylsiloxanefilmsforhighefficiencyperovskitesolarcells
AT mansoochoi motheyestructuredpolydimethylsiloxanefilmsforhighefficiencyperovskitesolarcells