Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations

<p>Volcanic eruptions eject large amounts of ash and trace gases such as sulfur dioxide (SO<span class="inline-formula"><sub>2</sub></span>) into the atmosphere. A significant difficulty in mitigating the impact of volcanic SO<span class="inline-formul...

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Main Authors: M.-E. Koukouli, K. Michailidis, P. Hedelt, I. A. Taylor, A. Inness, L. Clarisse, D. Balis, D. Efremenko, D. Loyola, R. G. Grainger, C. Retscher
Format: Article
Language:English
Published: Copernicus Publications 2022-04-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/22/5665/2022/acp-22-5665-2022.pdf
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author M.-E. Koukouli
K. Michailidis
P. Hedelt
I. A. Taylor
A. Inness
L. Clarisse
D. Balis
D. Efremenko
D. Loyola
R. G. Grainger
C. Retscher
author_facet M.-E. Koukouli
K. Michailidis
P. Hedelt
I. A. Taylor
A. Inness
L. Clarisse
D. Balis
D. Efremenko
D. Loyola
R. G. Grainger
C. Retscher
author_sort M.-E. Koukouli
collection DOAJ
description <p>Volcanic eruptions eject large amounts of ash and trace gases such as sulfur dioxide (SO<span class="inline-formula"><sub>2</sub></span>) into the atmosphere. A significant difficulty in mitigating the impact of volcanic SO<span class="inline-formula"><sub>2</sub></span> clouds on air traffic safety is that these gas emissions can be rapidly transported over long distances. The use of space-borne instruments enables the global monitoring of volcanic SO<span class="inline-formula"><sub>2</sub></span> emissions in an economical and risk-free manner. Within the European Space Agency (ESA) Sentinel-5p<span class="inline-formula">+</span> Innovation project, the S5P SO<span class="inline-formula"><sub>2</sub></span> layer height (S5P<span class="inline-formula">+</span>I: SO2LH) activities led to the improvements of the retrieval algorithm and generation of the corresponding near real-time S5P SO<span class="inline-formula"><sub>2</sub></span> LH products. These are currently operationally provided, in near real-time, by the German Aerospace Center (DLR) within the framework of the Innovative Products for Analyses of Atmospheric Composition (INPULS) project. The main aim of this paper is to present its extensive verification, accomplished within the S5P<span class="inline-formula">+</span>I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements from the IASI/Metop and CALIOP/CALIPSO instruments as well as assess its impact on the forecasts provided by the Copernicus Atmospheric Monitoring Service (CAMS). The mean difference between S5P and IASI observations for the Raikoke 2019, the Nishinoshima 2020 and the La Soufrière-St Vincent 2021 eruptive periods is <span class="inline-formula">∼</span> 0.5 <span class="inline-formula">±</span> 3 km, while for the Taal 2020 eruption, a larger difference was found, between 3 <span class="inline-formula">±</span> 3 km and 4 <span class="inline-formula">±</span> 3 km. The comparison of the daily mean SO<span class="inline-formula"><sub>2</sub></span> LH further demonstrates the capabilities of this near real-time product, with slopes between 0.8 and 1 and correlation coefficients ranging between 0.6 and 0.8. Comparisons between the S5P SO<span class="inline-formula"><sub>2</sub></span> LH and the CALIOP/CALIPSO ash plumes revealed an expected bias at <span class="inline-formula">−</span>2.5 <span class="inline-formula">±</span> 2 km, considering that the injected SO<span class="inline-formula"><sub>2</sub></span> and ash plume locations do not always coincide over an eruption. Furthermore, the CAMS assimilation of the S5P SO<span class="inline-formula"><sub>2</sub></span> LH product led to much improved model output against the non-assimilated IASI LH, with a mean difference of 1.5 <span class="inline-formula">±</span> 2 km, compared to the original CAMS analysis, and improved the geographical spread of the Raikoke volcanic plume following the eruptive days.</p>
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spelling doaj.art-9d2fdf005ac94020b12faff2fbf5b6872022-12-22T00:13:38ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242022-04-01225665568310.5194/acp-22-5665-2022Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observationsM.-E. Koukouli0K. Michailidis1P. Hedelt2I. A. Taylor3A. Inness4L. Clarisse5D. Balis6D. Efremenko7D. Loyola8R. G. Grainger9C. Retscher10Laboratory of Atmospheric Physics, Aristotle University of Thessaloniki, Thessaloniki, GreeceLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, Thessaloniki, GreeceGerman Aerospace Center (DLR), Remote Sensing Technology Institute, Oberpfaffenhofen, GermanyCOMET, Sub-department of Atmospheric, Oceanic and Planetary Physics, University of Oxford, Oxford, UKEuropean Centre for Medium-Range Weather Forecasts (ECMWF), Reading, UKUniversité Libre de Bruxelles (ULB), Spectroscopy, Quantum Chemistry and Atmospheric Remote Sensing (SQUARES), Brussels, BelgiumLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, Thessaloniki, GreeceGerman Aerospace Center (DLR), Remote Sensing Technology Institute, Oberpfaffenhofen, GermanyGerman Aerospace Center (DLR), Remote Sensing Technology Institute, Oberpfaffenhofen, GermanyCOMET, Sub-department of Atmospheric, Oceanic and Planetary Physics, University of Oxford, Oxford, UKEuropean Space Agency, ESRIN, Frascati, Rome, Italy<p>Volcanic eruptions eject large amounts of ash and trace gases such as sulfur dioxide (SO<span class="inline-formula"><sub>2</sub></span>) into the atmosphere. A significant difficulty in mitigating the impact of volcanic SO<span class="inline-formula"><sub>2</sub></span> clouds on air traffic safety is that these gas emissions can be rapidly transported over long distances. The use of space-borne instruments enables the global monitoring of volcanic SO<span class="inline-formula"><sub>2</sub></span> emissions in an economical and risk-free manner. Within the European Space Agency (ESA) Sentinel-5p<span class="inline-formula">+</span> Innovation project, the S5P SO<span class="inline-formula"><sub>2</sub></span> layer height (S5P<span class="inline-formula">+</span>I: SO2LH) activities led to the improvements of the retrieval algorithm and generation of the corresponding near real-time S5P SO<span class="inline-formula"><sub>2</sub></span> LH products. These are currently operationally provided, in near real-time, by the German Aerospace Center (DLR) within the framework of the Innovative Products for Analyses of Atmospheric Composition (INPULS) project. The main aim of this paper is to present its extensive verification, accomplished within the S5P<span class="inline-formula">+</span>I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements from the IASI/Metop and CALIOP/CALIPSO instruments as well as assess its impact on the forecasts provided by the Copernicus Atmospheric Monitoring Service (CAMS). The mean difference between S5P and IASI observations for the Raikoke 2019, the Nishinoshima 2020 and the La Soufrière-St Vincent 2021 eruptive periods is <span class="inline-formula">∼</span> 0.5 <span class="inline-formula">±</span> 3 km, while for the Taal 2020 eruption, a larger difference was found, between 3 <span class="inline-formula">±</span> 3 km and 4 <span class="inline-formula">±</span> 3 km. The comparison of the daily mean SO<span class="inline-formula"><sub>2</sub></span> LH further demonstrates the capabilities of this near real-time product, with slopes between 0.8 and 1 and correlation coefficients ranging between 0.6 and 0.8. Comparisons between the S5P SO<span class="inline-formula"><sub>2</sub></span> LH and the CALIOP/CALIPSO ash plumes revealed an expected bias at <span class="inline-formula">−</span>2.5 <span class="inline-formula">±</span> 2 km, considering that the injected SO<span class="inline-formula"><sub>2</sub></span> and ash plume locations do not always coincide over an eruption. Furthermore, the CAMS assimilation of the S5P SO<span class="inline-formula"><sub>2</sub></span> LH product led to much improved model output against the non-assimilated IASI LH, with a mean difference of 1.5 <span class="inline-formula">±</span> 2 km, compared to the original CAMS analysis, and improved the geographical spread of the Raikoke volcanic plume following the eruptive days.</p>https://acp.copernicus.org/articles/22/5665/2022/acp-22-5665-2022.pdf
spellingShingle M.-E. Koukouli
K. Michailidis
P. Hedelt
I. A. Taylor
A. Inness
L. Clarisse
D. Balis
D. Efremenko
D. Loyola
R. G. Grainger
C. Retscher
Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
Atmospheric Chemistry and Physics
title Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
title_full Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
title_fullStr Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
title_full_unstemmed Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
title_short Volcanic SO<sub>2</sub> layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
title_sort volcanic so sub 2 sub layer height by tropomi s5p evaluation against iasi metop and caliop calipso observations
url https://acp.copernicus.org/articles/22/5665/2022/acp-22-5665-2022.pdf
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