Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures

Twisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré he...

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Main Authors: Dominik Kiese, Finn Lasse Buessen, Ciarán Hickey, Simon Trebst, Michael M. Scherer
Format: Article
Language:English
Published: American Physical Society 2020-03-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.013370
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author Dominik Kiese
Finn Lasse Buessen
Ciarán Hickey
Simon Trebst
Michael M. Scherer
author_facet Dominik Kiese
Finn Lasse Buessen
Ciarán Hickey
Simon Trebst
Michael M. Scherer
author_sort Dominik Kiese
collection DOAJ
description Twisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré heterostructures, derived in the strong-coupling limit at integer filling, generically leads to spin-valley Heisenberg models. Here we explore the emergence and stability of spin-liquid behavior in an SU(2)^{spin}⊗SU(2)^{valley} Heisenberg model upon inclusion of Hund's-induced and longer-ranged exchange couplings, employing a pseudofermion functional renormalization group approach. We consider two lattice geometries, triangular and honeycomb (relevant to different moiré heterostructures), and find, for both cases, an extended parameter regime surrounding the SU(4) symmetric point where no long-range order occurs, indicating a stable realm of quantum spin-liquid behavior. For large Hund's coupling, we identify the adjacent magnetic orders, with both antiferromagnetic and ferromagnetic ground states emerging in the separate spin and valley degrees of freedom. For both lattice geometries the inclusion of longer-ranged exchange couplings is found to have both stabilizing and destabilizing effects on the spin-liquid regime depending on the sign of the additional couplings.
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spelling doaj.art-9d9eebfa3c684584825ae219486a1ac82024-04-12T16:52:10ZengAmerican Physical SocietyPhysical Review Research2643-15642020-03-012101337010.1103/PhysRevResearch.2.013370Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructuresDominik KieseFinn Lasse BuessenCiarán HickeySimon TrebstMichael M. SchererTwisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré heterostructures, derived in the strong-coupling limit at integer filling, generically leads to spin-valley Heisenberg models. Here we explore the emergence and stability of spin-liquid behavior in an SU(2)^{spin}⊗SU(2)^{valley} Heisenberg model upon inclusion of Hund's-induced and longer-ranged exchange couplings, employing a pseudofermion functional renormalization group approach. We consider two lattice geometries, triangular and honeycomb (relevant to different moiré heterostructures), and find, for both cases, an extended parameter regime surrounding the SU(4) symmetric point where no long-range order occurs, indicating a stable realm of quantum spin-liquid behavior. For large Hund's coupling, we identify the adjacent magnetic orders, with both antiferromagnetic and ferromagnetic ground states emerging in the separate spin and valley degrees of freedom. For both lattice geometries the inclusion of longer-ranged exchange couplings is found to have both stabilizing and destabilizing effects on the spin-liquid regime depending on the sign of the additional couplings.http://doi.org/10.1103/PhysRevResearch.2.013370
spellingShingle Dominik Kiese
Finn Lasse Buessen
Ciarán Hickey
Simon Trebst
Michael M. Scherer
Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
Physical Review Research
title Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
title_full Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
title_fullStr Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
title_full_unstemmed Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
title_short Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures
title_sort emergence and stability of spin valley entangled quantum liquids in moire heterostructures
url http://doi.org/10.1103/PhysRevResearch.2.013370
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