Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers

Because electromagnetic (EM) pollution of the environment is becoming such a pervasive issue, highly efficient solutions for EM protection are being keenly sought for. Our approach provides new avenues to simple, compact, and efficient broadband microwave absorbers designed to cancel EM interference...

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Main Authors: Yann Danlée, Francisco Mederos-Henry, Sophie Hermans, Christian Bailly, Isabelle Huynen
Format: Article
Language:English
Published: Frontiers Media S.A. 2020-07-01
Series:Frontiers in Materials
Subjects:
Online Access:https://www.frontiersin.org/article/10.3389/fmats.2020.00214/full
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author Yann Danlée
Yann Danlée
Francisco Mederos-Henry
Sophie Hermans
Christian Bailly
Isabelle Huynen
author_facet Yann Danlée
Yann Danlée
Francisco Mederos-Henry
Sophie Hermans
Christian Bailly
Isabelle Huynen
author_sort Yann Danlée
collection DOAJ
description Because electromagnetic (EM) pollution of the environment is becoming such a pervasive issue, highly efficient solutions for EM protection are being keenly sought for. Our approach provides new avenues to simple, compact, and efficient broadband microwave absorbers designed to cancel EM interferences in the microwave range. The paper demonstrates the potential of a clever organization of nanoscale inclusions (carbon nanotubes, graphene, magnetic metallic nanowires or nanoparticles) in polymer matrices for controlling the propagation of microwaves over a wide range of wavelengths (10−3-10−1 m), focusing on broadband absorption. Controlled architectures of polymer composites loaded with various nanofillers, and in particular layered stacks of composite films enable optimization of the absorption bandwidth while preserving the compactness of the structure. First, various carbon-based and metallic nanofillers are synthesized. Next, nanofillers are dispersed in a polymer matrix thanks to melt polymer processing and dispersion techniques. The absorption characteristics of resulting thin composite slabs are first characterized. Various combinations of superposed slabs are then investigated and modeled in order to optimize the absorption of the resulting multilayers. As innovative approach, the performances of the investigated structures are finally compared with the help of a new figure of merit combining the maximum absorption and its bandwidth.
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spelling doaj.art-9e246bd4e5ad4b1bbd3bd4e96205192a2022-12-21T23:59:00ZengFrontiers Media S.A.Frontiers in Materials2296-80162020-07-01710.3389/fmats.2020.00214544389Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic NanofillersYann Danlée0Yann Danlée1Francisco Mederos-Henry2Sophie Hermans3Christian Bailly4Isabelle Huynen5BSMA Division, Institute IMCN, Université Catholique de Louvain (UCLouvain), Louvain-la-Neuve, BelgiumELEN Division, Institute ICTEAM, UCLouvain, Louvain-la-Neuve, BelgiumMOST Division, Institute IMCN, UCLouvain, Louvain-la-Neuve, BelgiumMOST Division, Institute IMCN, UCLouvain, Louvain-la-Neuve, BelgiumBSMA Division, Institute IMCN, Université Catholique de Louvain (UCLouvain), Louvain-la-Neuve, BelgiumELEN Division, Institute ICTEAM, UCLouvain, Louvain-la-Neuve, BelgiumBecause electromagnetic (EM) pollution of the environment is becoming such a pervasive issue, highly efficient solutions for EM protection are being keenly sought for. Our approach provides new avenues to simple, compact, and efficient broadband microwave absorbers designed to cancel EM interferences in the microwave range. The paper demonstrates the potential of a clever organization of nanoscale inclusions (carbon nanotubes, graphene, magnetic metallic nanowires or nanoparticles) in polymer matrices for controlling the propagation of microwaves over a wide range of wavelengths (10−3-10−1 m), focusing on broadband absorption. Controlled architectures of polymer composites loaded with various nanofillers, and in particular layered stacks of composite films enable optimization of the absorption bandwidth while preserving the compactness of the structure. First, various carbon-based and metallic nanofillers are synthesized. Next, nanofillers are dispersed in a polymer matrix thanks to melt polymer processing and dispersion techniques. The absorption characteristics of resulting thin composite slabs are first characterized. Various combinations of superposed slabs are then investigated and modeled in order to optimize the absorption of the resulting multilayers. As innovative approach, the performances of the investigated structures are finally compared with the help of a new figure of merit combining the maximum absorption and its bandwidth.https://www.frontiersin.org/article/10.3389/fmats.2020.00214/fullmicrowave absorptioncarbon nanotubesmetallic nanowiresnanocompositegradient structure
spellingShingle Yann Danlée
Yann Danlée
Francisco Mederos-Henry
Sophie Hermans
Christian Bailly
Isabelle Huynen
Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
Frontiers in Materials
microwave absorption
carbon nanotubes
metallic nanowires
nanocomposite
gradient structure
title Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
title_full Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
title_fullStr Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
title_full_unstemmed Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
title_short Ranking Broadband Microwave Absorption Performance of Multilayered Polymer Nanocomposites Containing Carbon and Metallic Nanofillers
title_sort ranking broadband microwave absorption performance of multilayered polymer nanocomposites containing carbon and metallic nanofillers
topic microwave absorption
carbon nanotubes
metallic nanowires
nanocomposite
gradient structure
url https://www.frontiersin.org/article/10.3389/fmats.2020.00214/full
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