Molecular design of recyclable thermosetting polyimide and its composite with excellent mechanical and tribological properties

Abstract Recyclability of thermosetting polymers and their composites is a challenge for alleviating environmental pollution and resource waste. In this study, solvent-recyclable thermosetting polyimide (PI) and its composite were successfully synthesized. The tensile strength, elongation at break,...

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Bibliographic Details
Main Authors: Xiaoyue Wang, Zenghui Yang, Tingmei Wang, Qihua Wang, Xinrui Zhang, Song Li
Format: Article
Language:English
Published: SpringerOpen 2023-12-01
Series:Friction
Subjects:
Online Access:https://doi.org/10.1007/s40544-023-0770-6
Description
Summary:Abstract Recyclability of thermosetting polymers and their composites is a challenge for alleviating environmental pollution and resource waste. In this study, solvent-recyclable thermosetting polyimide (PI) and its composite were successfully synthesized. The tensile strength, elongation at break, and Young’s modulus of PI are 108.70 ± 7.29 MPa, 19.35% ± 3.89%, and 2336.42 ± 128.00 MPa, respectively. The addition of reduced graphene oxide (RGO) not only enhances the mechanical properties of PI but also endows it with excellent tribological properties. The PI illustrates a high recycling efficiency of 94.15%, but the recycled composite exhibits inferior mechanical properties. The recycling and utilization of PI and its composite are realized through imine bonds (–C=N), which provides new guidance for solving the problem of environmental pollution and resource waste and is potential application in the field of sustainable tribology.
ISSN:2223-7690
2223-7704