Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide

Natural fibre biopolymer composites with both fibres and matrix being derived from biomaterials are increasingly used in demanding applications, such as sensing, packaging, building, and transport, and require good electrical, thermal, and flame retardant properties. Herein, an investigation of the...

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Main Authors: Yilin He, Shuying Wu, Anthony Chun Yin Yuen, Feng Huang, Cyrille Boyer, Chun H. Wang, Jin Zhang
Format: Article
Language:English
Published: MDPI AG 2022-09-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/14/19/3946
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author Yilin He
Shuying Wu
Anthony Chun Yin Yuen
Feng Huang
Cyrille Boyer
Chun H. Wang
Jin Zhang
author_facet Yilin He
Shuying Wu
Anthony Chun Yin Yuen
Feng Huang
Cyrille Boyer
Chun H. Wang
Jin Zhang
author_sort Yilin He
collection DOAJ
description Natural fibre biopolymer composites with both fibres and matrix being derived from biomaterials are increasingly used in demanding applications, such as sensing, packaging, building, and transport, and require good electrical, thermal, and flame retardant properties. Herein, an investigation of the effectiveness of functionalising nonwoven cotton/poly(lactic acid) (PLA) fibre mats with graphene oxide nanosheets has been reported by using a facile dip-coating method followed by thermal reduction for enhancing the electric, thermal, and abrasion-resistance properties. The manufacturing processes for preparing biocomposites and introducing functionality are readily scalable. Experimental results reveal that with the addition of less than 0.5 wt% graphene nanoplatelets, the biocomposites showed significant improvements in abrasion resistance, electrical conductivity, thermal conductivity, and diffusivity. Furthermore, the composite shows excellent piezo-resistivity to act as strain sensors with a gauge factor of 2.59 at strains up to 1%.
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spelling doaj.art-9e8966d073eb46c8a1436b3e0e9b5af92023-11-23T21:31:39ZengMDPI AGPolymers2073-43602022-09-011419394610.3390/polym14193946Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene OxideYilin He0Shuying Wu1Anthony Chun Yin Yuen2Feng Huang3Cyrille Boyer4Chun H. Wang5Jin Zhang6School of Mechanical and Manufacturing Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaSchool of Engineering, Macquarie University, Sydney, NSW 2109, AustraliaSchool of Mechanical and Manufacturing Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaSchool of Mechanical and Manufacturing Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaSchool of Chemical Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaSchool of Mechanical and Manufacturing Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaSchool of Mechanical and Manufacturing Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaNatural fibre biopolymer composites with both fibres and matrix being derived from biomaterials are increasingly used in demanding applications, such as sensing, packaging, building, and transport, and require good electrical, thermal, and flame retardant properties. Herein, an investigation of the effectiveness of functionalising nonwoven cotton/poly(lactic acid) (PLA) fibre mats with graphene oxide nanosheets has been reported by using a facile dip-coating method followed by thermal reduction for enhancing the electric, thermal, and abrasion-resistance properties. The manufacturing processes for preparing biocomposites and introducing functionality are readily scalable. Experimental results reveal that with the addition of less than 0.5 wt% graphene nanoplatelets, the biocomposites showed significant improvements in abrasion resistance, electrical conductivity, thermal conductivity, and diffusivity. Furthermore, the composite shows excellent piezo-resistivity to act as strain sensors with a gauge factor of 2.59 at strains up to 1%.https://www.mdpi.com/2073-4360/14/19/3946biocompositephysical propertiesmicrostructural analysiscompression moulding
spellingShingle Yilin He
Shuying Wu
Anthony Chun Yin Yuen
Feng Huang
Cyrille Boyer
Chun H. Wang
Jin Zhang
Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
Polymers
biocomposite
physical properties
microstructural analysis
compression moulding
title Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
title_full Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
title_fullStr Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
title_full_unstemmed Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
title_short Scalable Manufacturing Process and Multifunctional Performance of Cotton Fibre-Reinforced Poly(Lactic Acid) (PLA) Bio-Composites Coated by Graphene Oxide
title_sort scalable manufacturing process and multifunctional performance of cotton fibre reinforced poly lactic acid pla bio composites coated by graphene oxide
topic biocomposite
physical properties
microstructural analysis
compression moulding
url https://www.mdpi.com/2073-4360/14/19/3946
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