Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid

Recently, various environmental-friendly materials have been investigated and developed, especially composites of polylactic acid (PLA) and plant fibers. This paper investigates the effects of pulp fiber (PF) and epoxidized Tung oil (ETO) content on the properties of biocomposites, based on polylact...

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Main Authors: Van Khoi Nguyen, Thanh Tung Nguyen, Thu Ha Pham Thi, Thu Trang Pham
Format: Article
Language:English
Published: MDPI AG 2020-05-01
Series:Journal of Composites Science
Subjects:
Online Access:https://www.mdpi.com/2504-477X/4/2/56
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author Van Khoi Nguyen
Thanh Tung Nguyen
Thu Ha Pham Thi
Thu Trang Pham
author_facet Van Khoi Nguyen
Thanh Tung Nguyen
Thu Ha Pham Thi
Thu Trang Pham
author_sort Van Khoi Nguyen
collection DOAJ
description Recently, various environmental-friendly materials have been investigated and developed, especially composites of polylactic acid (PLA) and plant fibers. This paper investigates the effects of pulp fiber (PF) and epoxidized Tung oil (ETO) content on the properties of biocomposites, based on polylactic acid. The bleached pulp fiber reinforced PLA (PLA/PF) composites with 10–50 wt% fiber contents and 0–15% epoxidized Tung oil contents (with a certain number of fiber) were prepared in an internal mixer (Plastograph<sup>®</sup> EC) at 150 °C. The mechanical properties of PLA/PF composites were improved significantly. The pulp fiber reinforced PLA composites, with the fiber content of 30 wt%, were found to have the highest mechanical properties. The tensile and flexural properties of PLA/Tung oil-soaked-pulp fiber composites were higher than those of PLA/Tung oil unsoaked pulp fiber composites. In addition, the degradation temperature of PLA-based composites decreased after adding more pulp fiber. The pulp fibers were well-dispersed in the PLA matrix with the content up to 30 wt%. The interaction between pulp fiber and PLA matrix improved by the addition of epoxidized Tung oil. Epoxidized Tung oil also improved tensile and flexural strength of composite materials when it was added with a number of below 10% of fiber.
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spelling doaj.art-9ea3243bec8c4103acba935878091e122023-11-20T00:56:49ZengMDPI AGJournal of Composites Science2504-477X2020-05-01425610.3390/jcs4020056Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic AcidVan Khoi Nguyen0Thanh Tung Nguyen1Thu Ha Pham Thi2Thu Trang Pham3Institute of Chemistry, VAST, 18 Hoang Quoc Viet, Cau Giay, Ha Noi 122300, VietnamInstitute of Chemistry, VAST, 18 Hoang Quoc Viet, Cau Giay, Ha Noi 122300, VietnamInstitute of Chemistry, VAST, 18 Hoang Quoc Viet, Cau Giay, Ha Noi 122300, VietnamInstitute of Chemistry, VAST, 18 Hoang Quoc Viet, Cau Giay, Ha Noi 122300, VietnamRecently, various environmental-friendly materials have been investigated and developed, especially composites of polylactic acid (PLA) and plant fibers. This paper investigates the effects of pulp fiber (PF) and epoxidized Tung oil (ETO) content on the properties of biocomposites, based on polylactic acid. The bleached pulp fiber reinforced PLA (PLA/PF) composites with 10–50 wt% fiber contents and 0–15% epoxidized Tung oil contents (with a certain number of fiber) were prepared in an internal mixer (Plastograph<sup>®</sup> EC) at 150 °C. The mechanical properties of PLA/PF composites were improved significantly. The pulp fiber reinforced PLA composites, with the fiber content of 30 wt%, were found to have the highest mechanical properties. The tensile and flexural properties of PLA/Tung oil-soaked-pulp fiber composites were higher than those of PLA/Tung oil unsoaked pulp fiber composites. In addition, the degradation temperature of PLA-based composites decreased after adding more pulp fiber. The pulp fibers were well-dispersed in the PLA matrix with the content up to 30 wt%. The interaction between pulp fiber and PLA matrix improved by the addition of epoxidized Tung oil. Epoxidized Tung oil also improved tensile and flexural strength of composite materials when it was added with a number of below 10% of fiber.https://www.mdpi.com/2504-477X/4/2/56poly (lactic acid)pulp fibernatural fiber reinforced compositesepoxidized Tung oil
spellingShingle Van Khoi Nguyen
Thanh Tung Nguyen
Thu Ha Pham Thi
Thu Trang Pham
Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
Journal of Composites Science
poly (lactic acid)
pulp fiber
natural fiber reinforced composites
epoxidized Tung oil
title Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
title_full Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
title_fullStr Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
title_full_unstemmed Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
title_short Effects of Pulp Fiber and Epoxidized Tung Oil Content on the Properties of Biocomposites Based on Polylactic Acid
title_sort effects of pulp fiber and epoxidized tung oil content on the properties of biocomposites based on polylactic acid
topic poly (lactic acid)
pulp fiber
natural fiber reinforced composites
epoxidized Tung oil
url https://www.mdpi.com/2504-477X/4/2/56
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