Multimode polariton effects on molecular energy transport and spectral fluctuations
Optical microcavities affect chemical processes via strong light-matter interactions, but the extent to which chemistry can be controlled with these materials remains unclear. Here, the author employs microscopic simulations of multimode photonic wire under strong coupling with a disordered molecula...
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| Format: | Article |
| Language: | English |
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Nature Portfolio
2022-04-01
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| Series: | Communications Chemistry |
| Online Access: | https://doi.org/10.1038/s42004-022-00660-0 |
| _version_ | 1811290469499404288 |
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| author | Raphael F. Ribeiro |
| author_facet | Raphael F. Ribeiro |
| author_sort | Raphael F. Ribeiro |
| collection | DOAJ |
| description | Optical microcavities affect chemical processes via strong light-matter interactions, but the extent to which chemistry can be controlled with these materials remains unclear. Here, the author employs microscopic simulations of multimode photonic wire under strong coupling with a disordered molecular ensemble to investigate the influence of the cavity resonator on the local molecular density of states and excited-state diffusion. |
| first_indexed | 2024-04-13T04:13:25Z |
| format | Article |
| id | doaj.art-a017f2a9d786423baf1517671b7da457 |
| institution | Directory Open Access Journal |
| issn | 2399-3669 |
| language | English |
| last_indexed | 2024-04-13T04:13:25Z |
| publishDate | 2022-04-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Communications Chemistry |
| spelling | doaj.art-a017f2a9d786423baf1517671b7da4572022-12-22T03:03:03ZengNature PortfolioCommunications Chemistry2399-36692022-04-015111010.1038/s42004-022-00660-0Multimode polariton effects on molecular energy transport and spectral fluctuationsRaphael F. Ribeiro0Department of Chemistry and Cherry Emerson Center for Scientific Computation, Emory UniversityOptical microcavities affect chemical processes via strong light-matter interactions, but the extent to which chemistry can be controlled with these materials remains unclear. Here, the author employs microscopic simulations of multimode photonic wire under strong coupling with a disordered molecular ensemble to investigate the influence of the cavity resonator on the local molecular density of states and excited-state diffusion.https://doi.org/10.1038/s42004-022-00660-0 |
| spellingShingle | Raphael F. Ribeiro Multimode polariton effects on molecular energy transport and spectral fluctuations Communications Chemistry |
| title | Multimode polariton effects on molecular energy transport and spectral fluctuations |
| title_full | Multimode polariton effects on molecular energy transport and spectral fluctuations |
| title_fullStr | Multimode polariton effects on molecular energy transport and spectral fluctuations |
| title_full_unstemmed | Multimode polariton effects on molecular energy transport and spectral fluctuations |
| title_short | Multimode polariton effects on molecular energy transport and spectral fluctuations |
| title_sort | multimode polariton effects on molecular energy transport and spectral fluctuations |
| url | https://doi.org/10.1038/s42004-022-00660-0 |
| work_keys_str_mv | AT raphaelfribeiro multimodepolaritoneffectsonmolecularenergytransportandspectralfluctuations |