The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys

Experimental studies into the forced magnetostriction, magnetization, and temperature dependence of permeability in Ni<sub>2</sub>MnIn and Ni<sub>2</sub>MnSn ferromagnetic Heusler alloys were performed according to the spin fluctuation theory of itinerant ferromagnetism propo...

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Main Authors: Takuo Sakon, Junya Yamazaki, Takumi Komori, Takeshi Kanomata, Yasuo Narumi, Masayuki Hagiwara, Hiroyuki Nojiri, Yoshiya Adachi
Format: Article
Language:English
Published: MDPI AG 2020-04-01
Series:Materials
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Online Access:https://www.mdpi.com/1996-1944/13/9/2017
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author Takuo Sakon
Junya Yamazaki
Takumi Komori
Takeshi Kanomata
Yasuo Narumi
Masayuki Hagiwara
Hiroyuki Nojiri
Yoshiya Adachi
author_facet Takuo Sakon
Junya Yamazaki
Takumi Komori
Takeshi Kanomata
Yasuo Narumi
Masayuki Hagiwara
Hiroyuki Nojiri
Yoshiya Adachi
author_sort Takuo Sakon
collection DOAJ
description Experimental studies into the forced magnetostriction, magnetization, and temperature dependence of permeability in Ni<sub>2</sub>MnIn and Ni<sub>2</sub>MnSn ferromagnetic Heusler alloys were performed according to the spin fluctuation theory of itinerant ferromagnetism proposed by Takahashi. We investigated the magnetic field (<i>H</i>) dependence of magnetization (<i>M</i>) at the Curie temperature <i>T</i><sub>C</sub>, and at <i>T</i> = 4.2 K, which concerns the ground state of the ferromagnetic state. The <i>M</i>-<i>H</i> result at <i>T</i><sub>C</sub> was analyzed by means of the <i>H</i> versus <i>M</i><sup>5</sup> dependence. At 4.2 K, it was investigated by means of an Arrott plot (<i>H</i>/<i>M</i> vs. <i>M</i><sup>2</sup>) according to Takahashi’s theory. As for Ni<sub>2</sub>MnIn and Ni<sub>2</sub>MnSn, the spin fluctuation parameters in <i>k</i>-space (momentum space, <i>T</i><sub>A</sub>) and that in energy space (frequency space, <i>T</i><sub>0</sub>) obtained at <i>T</i><sub>C</sub> and 4.2 K were almost the same. The average values obtained at <i>T</i><sub>C</sub> and 4.2 K were <i>T</i><sub>A</sub> = 342 K, <i>T</i><sub>0</sub> = 276 K for Ni<sub>2</sub>MnIn and <i>T</i><sub>A</sub> = 447 K, <i>T</i><sub>0</sub> = 279 K for Ni<sub>2</sub>MnSn, respectively. The forced magnetostriction at <i>T</i><sub>C</sub> was also investigated. The forced linear magnetostriction (Δ<i>L</i>/<i>L</i>) and the forced volume magnetostriction (Δ<i>V</i>/<i>V</i>) were proportional to <i>M</i><sup>4</sup>, which followed Takahashi’s theory. We compared the forced volume magnetostriction Δ<i>V</i>/<i>V</i> and mechanical parameter, bulk modulus <i>K</i>. Δ<i>V</i>/<i>V</i> is inversely proportional to <i>K</i>. We also discuss the spin polarization of Ni<sub>2</sub>MnIn and other magnetic Heusler alloys. The <i>p</i><sub>C</sub>/<i>p</i><sub>S</sub> of Ni<sub>2</sub>MnIn was 0.860. This is comparable with that of Co<sub>2</sub>MnGa, which is a famous half-metallic alloy.
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spelling doaj.art-a073e5b384444b1183c6ddb62166724a2023-11-19T22:42:27ZengMDPI AGMaterials1996-19442020-04-01139201710.3390/ma13092017The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler AlloysTakuo Sakon0Junya Yamazaki1Takumi Komori2Takeshi Kanomata3Yasuo Narumi4Masayuki Hagiwara5Hiroyuki Nojiri6Yoshiya Adachi7Department of Mechanical and Systems Engineering, Faculty of Science and Technology, Ryukoku University, Otsu 520-2194, Shiga, JapanDepartment of Mechanical and Systems Engineering, Faculty of Science and Technology, Ryukoku University, Otsu 520-2194, Shiga, JapanDepartment of Mechanical and Systems Engineering, Faculty of Science and Technology, Ryukoku University, Otsu 520-2194, Shiga, JapanResearch Institute for Engineering and Technology, Tohoku Gakuin University, Tagajo 985-8537, Miyagi, JapanCenter for Advanced High Magnetic Field Science, Graduate School of Science, Osaka University, 1-1 Machikaneyama, Toyonaka 560-0043, Osaka, JapanCenter for Advanced High Magnetic Field Science, Graduate School of Science, Osaka University, 1-1 Machikaneyama, Toyonaka 560-0043, Osaka, JapanInstitute for Materials Research, Tohoku University, Sendai 980-8577, Miyagi, JapanGraduate School of Science and Engineering, Yamagata University, Yonezawa 992-8510, Yamagata, JapanExperimental studies into the forced magnetostriction, magnetization, and temperature dependence of permeability in Ni<sub>2</sub>MnIn and Ni<sub>2</sub>MnSn ferromagnetic Heusler alloys were performed according to the spin fluctuation theory of itinerant ferromagnetism proposed by Takahashi. We investigated the magnetic field (<i>H</i>) dependence of magnetization (<i>M</i>) at the Curie temperature <i>T</i><sub>C</sub>, and at <i>T</i> = 4.2 K, which concerns the ground state of the ferromagnetic state. The <i>M</i>-<i>H</i> result at <i>T</i><sub>C</sub> was analyzed by means of the <i>H</i> versus <i>M</i><sup>5</sup> dependence. At 4.2 K, it was investigated by means of an Arrott plot (<i>H</i>/<i>M</i> vs. <i>M</i><sup>2</sup>) according to Takahashi’s theory. As for Ni<sub>2</sub>MnIn and Ni<sub>2</sub>MnSn, the spin fluctuation parameters in <i>k</i>-space (momentum space, <i>T</i><sub>A</sub>) and that in energy space (frequency space, <i>T</i><sub>0</sub>) obtained at <i>T</i><sub>C</sub> and 4.2 K were almost the same. The average values obtained at <i>T</i><sub>C</sub> and 4.2 K were <i>T</i><sub>A</sub> = 342 K, <i>T</i><sub>0</sub> = 276 K for Ni<sub>2</sub>MnIn and <i>T</i><sub>A</sub> = 447 K, <i>T</i><sub>0</sub> = 279 K for Ni<sub>2</sub>MnSn, respectively. The forced magnetostriction at <i>T</i><sub>C</sub> was also investigated. The forced linear magnetostriction (Δ<i>L</i>/<i>L</i>) and the forced volume magnetostriction (Δ<i>V</i>/<i>V</i>) were proportional to <i>M</i><sup>4</sup>, which followed Takahashi’s theory. We compared the forced volume magnetostriction Δ<i>V</i>/<i>V</i> and mechanical parameter, bulk modulus <i>K</i>. Δ<i>V</i>/<i>V</i> is inversely proportional to <i>K</i>. We also discuss the spin polarization of Ni<sub>2</sub>MnIn and other magnetic Heusler alloys. The <i>p</i><sub>C</sub>/<i>p</i><sub>S</sub> of Ni<sub>2</sub>MnIn was 0.860. This is comparable with that of Co<sub>2</sub>MnGa, which is a famous half-metallic alloy.https://www.mdpi.com/1996-1944/13/9/2017ferromagnetic Heusler alloymagnetostrictionmagnetizationitinerant ferromagnetismspin polarization
spellingShingle Takuo Sakon
Junya Yamazaki
Takumi Komori
Takeshi Kanomata
Yasuo Narumi
Masayuki Hagiwara
Hiroyuki Nojiri
Yoshiya Adachi
The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
Materials
ferromagnetic Heusler alloy
magnetostriction
magnetization
itinerant ferromagnetism
spin polarization
title The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
title_full The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
title_fullStr The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
title_full_unstemmed The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
title_short The Forced Magnetostrictions and Magnetic Properties of Ni<sub>2</sub>MnX (X = In, Sn) Ferromagnetic Heusler Alloys
title_sort forced magnetostrictions and magnetic properties of ni sub 2 sub mnx x in sn ferromagnetic heusler alloys
topic ferromagnetic Heusler alloy
magnetostriction
magnetization
itinerant ferromagnetism
spin polarization
url https://www.mdpi.com/1996-1944/13/9/2017
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