Modeling and characterization of stochastic resistive switching in single Ag2S nanowires

Abstract Chalcogenide resistive switches (RS), such as Ag2S, change resistance due to the growth of metallic filaments between electrodes along the electric field gradient. Therefore, they are candidates for neuromorphic and volatile memory applications. This work analyzed the RS of individual Ag2S...

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Main Authors: Nikolay Frick, Mahshid Hosseini, Damien Guilbaud, Ming Gao, Thomas H. LaBean
Format: Article
Language:English
Published: Nature Portfolio 2022-04-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-022-09893-4
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author Nikolay Frick
Mahshid Hosseini
Damien Guilbaud
Ming Gao
Thomas H. LaBean
author_facet Nikolay Frick
Mahshid Hosseini
Damien Guilbaud
Ming Gao
Thomas H. LaBean
author_sort Nikolay Frick
collection DOAJ
description Abstract Chalcogenide resistive switches (RS), such as Ag2S, change resistance due to the growth of metallic filaments between electrodes along the electric field gradient. Therefore, they are candidates for neuromorphic and volatile memory applications. This work analyzed the RS of individual Ag2S nanowires (NWs) and extended the basic RS model to reproduce experimental observations. The work models resistivity of the device as a percolation of the conductive filaments. It also addressed continuous fluctuations of the resistivity with a stochastic change in volume fractions of the filaments in the device. As a result, these fluctuations cause unpredictable patterns in current-voltage characteristics and include a spontaneous change in resistance of the device during the linear sweep that conventional memristor models with constant resistivity cannot represent. The parameters of the presented stochastic model of a single Ag2S NW were fitted to the experimental data and reproduced key features of RS in the physical devices. Moreover, the model suggested a non-core shell structure of the Ag2S NWs. The outcome of this work is aimed to aid in simulating large self-assembled memristive networks and help to extend existing RS models.
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spelling doaj.art-a0a9cfcf32184f288d46dc40f0fdb7e42022-12-22T02:08:05ZengNature PortfolioScientific Reports2045-23222022-04-0112111010.1038/s41598-022-09893-4Modeling and characterization of stochastic resistive switching in single Ag2S nanowiresNikolay Frick0Mahshid Hosseini1Damien Guilbaud2Ming Gao3Thomas H. LaBean4NC State University, Materials Science and EngineeringNC State University, Materials Science and EngineeringNC State University, Biomedical EngineeringNC State University, Materials Science and EngineeringNC State University, Materials Science and EngineeringAbstract Chalcogenide resistive switches (RS), such as Ag2S, change resistance due to the growth of metallic filaments between electrodes along the electric field gradient. Therefore, they are candidates for neuromorphic and volatile memory applications. This work analyzed the RS of individual Ag2S nanowires (NWs) and extended the basic RS model to reproduce experimental observations. The work models resistivity of the device as a percolation of the conductive filaments. It also addressed continuous fluctuations of the resistivity with a stochastic change in volume fractions of the filaments in the device. As a result, these fluctuations cause unpredictable patterns in current-voltage characteristics and include a spontaneous change in resistance of the device during the linear sweep that conventional memristor models with constant resistivity cannot represent. The parameters of the presented stochastic model of a single Ag2S NW were fitted to the experimental data and reproduced key features of RS in the physical devices. Moreover, the model suggested a non-core shell structure of the Ag2S NWs. The outcome of this work is aimed to aid in simulating large self-assembled memristive networks and help to extend existing RS models.https://doi.org/10.1038/s41598-022-09893-4
spellingShingle Nikolay Frick
Mahshid Hosseini
Damien Guilbaud
Ming Gao
Thomas H. LaBean
Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
Scientific Reports
title Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
title_full Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
title_fullStr Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
title_full_unstemmed Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
title_short Modeling and characterization of stochastic resistive switching in single Ag2S nanowires
title_sort modeling and characterization of stochastic resistive switching in single ag2s nanowires
url https://doi.org/10.1038/s41598-022-09893-4
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