Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water
Abstract A wide range of chemicals was measured in different types of drinking water and urine samples through target and non-target screening (NTS) to estimate human exposure. Tap water samples collected from 42 locations in Barcelona (August–October/2020, May/2021), tap water filtered with domesti...
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Format: | Article |
Language: | English |
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Nature Portfolio
2023-03-01
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Series: | npj Clean Water |
Online Access: | https://doi.org/10.1038/s41545-023-00236-y |
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author | Dora Cserbik Paula E. Redondo-Hasselerharm Maria J. Farré Josep Sanchís Arantxa Bartolomé Alexandra Paraian Eva María Herrera Josep Caixach Cristina M. Villanueva Cintia Flores |
author_facet | Dora Cserbik Paula E. Redondo-Hasselerharm Maria J. Farré Josep Sanchís Arantxa Bartolomé Alexandra Paraian Eva María Herrera Josep Caixach Cristina M. Villanueva Cintia Flores |
author_sort | Dora Cserbik |
collection | DOAJ |
description | Abstract A wide range of chemicals was measured in different types of drinking water and urine samples through target and non-target screening (NTS) to estimate human exposure. Tap water samples collected from 42 locations in Barcelona (August–October/2020, May/2021), tap water filtered with domestic activated carbon filters (AC, N = 6) and reverse osmosis (RO, N = 5), commercial bottled water (N = 10), and urine (N = 39) samples were included. 35 per- and polyfluoroalkyl substances (PFAS), bisphenol A, and nonylphenol were analyzed using LC–MS/MS and GC–MS/MS, and NTS using LC–HRMS. 9 PFAS were detected in unfiltered tap water of first sampling (79% samples, median = 30 ng/L), 6 in the second (69%, median = 9.8 ng/L), and 5 in 13% urine samples. NTS tentatively identified pharmaceuticals and other industrial chemicals in drinking water. PFAS were removed by RO and not by AC filters. Findings provide valuable information for exposure science and water quality monitoring of emerging drinking water contaminants. |
first_indexed | 2024-04-09T23:12:12Z |
format | Article |
id | doaj.art-a12f28e0f5014de3bd57cd57b48f603d |
institution | Directory Open Access Journal |
issn | 2059-7037 |
language | English |
last_indexed | 2024-04-09T23:12:12Z |
publishDate | 2023-03-01 |
publisher | Nature Portfolio |
record_format | Article |
series | npj Clean Water |
spelling | doaj.art-a12f28e0f5014de3bd57cd57b48f603d2023-03-22T10:18:29ZengNature Portfolionpj Clean Water2059-70372023-03-016111010.1038/s41545-023-00236-yHuman exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking waterDora Cserbik0Paula E. Redondo-Hasselerharm1Maria J. Farré2Josep Sanchís3Arantxa Bartolomé4Alexandra Paraian5Eva María Herrera6Josep Caixach7Cristina M. Villanueva8Cintia Flores9ISGlobalISGlobalCatalan Institute for Water Research, ICRACatalan Institute for Water Research, ICRAMass Spectrometry Laboratory/Organic Pollutants, Institute of Environmental Assessment and Water Research, IDAEA-CSICMass Spectrometry Laboratory/Organic Pollutants, Institute of Environmental Assessment and Water Research, IDAEA-CSICMass Spectrometry Laboratory/Organic Pollutants, Institute of Environmental Assessment and Water Research, IDAEA-CSICMass Spectrometry Laboratory/Organic Pollutants, Institute of Environmental Assessment and Water Research, IDAEA-CSICISGlobalMass Spectrometry Laboratory/Organic Pollutants, Institute of Environmental Assessment and Water Research, IDAEA-CSICAbstract A wide range of chemicals was measured in different types of drinking water and urine samples through target and non-target screening (NTS) to estimate human exposure. Tap water samples collected from 42 locations in Barcelona (August–October/2020, May/2021), tap water filtered with domestic activated carbon filters (AC, N = 6) and reverse osmosis (RO, N = 5), commercial bottled water (N = 10), and urine (N = 39) samples were included. 35 per- and polyfluoroalkyl substances (PFAS), bisphenol A, and nonylphenol were analyzed using LC–MS/MS and GC–MS/MS, and NTS using LC–HRMS. 9 PFAS were detected in unfiltered tap water of first sampling (79% samples, median = 30 ng/L), 6 in the second (69%, median = 9.8 ng/L), and 5 in 13% urine samples. NTS tentatively identified pharmaceuticals and other industrial chemicals in drinking water. PFAS were removed by RO and not by AC filters. Findings provide valuable information for exposure science and water quality monitoring of emerging drinking water contaminants.https://doi.org/10.1038/s41545-023-00236-y |
spellingShingle | Dora Cserbik Paula E. Redondo-Hasselerharm Maria J. Farré Josep Sanchís Arantxa Bartolomé Alexandra Paraian Eva María Herrera Josep Caixach Cristina M. Villanueva Cintia Flores Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water npj Clean Water |
title | Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water |
title_full | Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water |
title_fullStr | Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water |
title_full_unstemmed | Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water |
title_short | Human exposure to per- and polyfluoroalkyl substances and other emerging contaminants in drinking water |
title_sort | human exposure to per and polyfluoroalkyl substances and other emerging contaminants in drinking water |
url | https://doi.org/10.1038/s41545-023-00236-y |
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