Measurement of field-free molecular alignment by balanced weak field polarization technique

We demonstrate the measurement of field-free molecular alignment of air can be realized by combining the weak field polarization technique (WFPT) with a balanced detection system. The measured signal is proportional to the alignment parameter. Periodic revival structures of the transient alignment a...

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Bibliographic Details
Main Authors: Peng Peng, Ya Bai, Na Li, Peng Liu
Format: Article
Language:English
Published: AIP Publishing LLC 2015-12-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/1.4937476
Description
Summary:We demonstrate the measurement of field-free molecular alignment of air can be realized by combining the weak field polarization technique (WFPT) with a balanced detection system. The measured signal is proportional to the alignment parameter. Periodic revival structures of the transient alignment and permanent alignment between revivals can be detected clearly by a single measurement with high sensitivity. Fourier transform spectrum of the measured signal agrees well with the calculation result and provides information of the populations of different J states in the rotational wave packet.
ISSN:2158-3226