Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing

Control over the microstructure and properties of alloys produced via additive manufacturing (AM) is a key barrier that limits widespread industrial adoption. Herein we demonstrate that liquid metal jetting (LMJ), an emerging metal-AM technique, can address this need by controlling the microstructur...

Full description

Bibliographic Details
Main Authors: Kellen D. Traxel, Eric S. Elton, Amelia M. Petersen, Chinthaka M. Silva, Aurélien Perron, Jason R. Jeffries, Andrew J. Pascall
Format: Article
Language:English
Published: Elsevier 2024-01-01
Series:Materials & Design
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S0264127523009607
_version_ 1827375619080454144
author Kellen D. Traxel
Eric S. Elton
Amelia M. Petersen
Chinthaka M. Silva
Aurélien Perron
Jason R. Jeffries
Andrew J. Pascall
author_facet Kellen D. Traxel
Eric S. Elton
Amelia M. Petersen
Chinthaka M. Silva
Aurélien Perron
Jason R. Jeffries
Andrew J. Pascall
author_sort Kellen D. Traxel
collection DOAJ
description Control over the microstructure and properties of alloys produced via additive manufacturing (AM) is a key barrier that limits widespread industrial adoption. Herein we demonstrate that liquid metal jetting (LMJ), an emerging metal-AM technique, can address this need by controlling the microstructure evolution during printing of bronze alloy C95400 (Cu-Al-Fe-Mn). We probed several solid-state phase transformations upon cooling by printing single-tracks onto a heated baseplate ranging from 50 °C to 600 °C surface temperature, which led to significant variation in the α-Cu and δ-Fe phase distribution, grain morphology, and chemical distribution within the deposited single-tracks. The printed microstructures exhibited as much as 80% difference in α-Cu grain size and nearly 30 % difference in α-Cu phase fraction due to baseplate temperature variation, indicating a wide range of available microstructures and properties achievable. Greater than 92% dense multi-layer samples were fabricated with fine grain structure and 27–34% higher hardness values compared to the barstock in the as-printed condition, demonstrating the applicability of this printing approach for multi-layer part fabrication. Our results highlight a unique microstructure tailoring capability for metal-AM parts that can be leveraged by manufacturers and end-users of AM technologies.
first_indexed 2024-03-08T11:54:38Z
format Article
id doaj.art-a1deb8f678ec4942b30d3a61bb71026c
institution Directory Open Access Journal
issn 0264-1275
language English
last_indexed 2024-03-08T11:54:38Z
publishDate 2024-01-01
publisher Elsevier
record_format Article
series Materials & Design
spelling doaj.art-a1deb8f678ec4942b30d3a61bb71026c2024-01-24T05:16:16ZengElsevierMaterials & Design0264-12752024-01-01237112544Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturingKellen D. Traxel0Eric S. Elton1Amelia M. Petersen2Chinthaka M. Silva3Aurélien Perron4Jason R. Jeffries5Andrew J. Pascall6Lawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United States; Corresponding author.Lawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United StatesLawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United StatesPacific Northwest National Laboratory, 02 Battelle Boulevard Richland, WA 99354, United StatesLawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United StatesLawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United StatesLawrence Livermore National Laboratory, 7000 East Ave, Livermore, CA 94550, United StatesControl over the microstructure and properties of alloys produced via additive manufacturing (AM) is a key barrier that limits widespread industrial adoption. Herein we demonstrate that liquid metal jetting (LMJ), an emerging metal-AM technique, can address this need by controlling the microstructure evolution during printing of bronze alloy C95400 (Cu-Al-Fe-Mn). We probed several solid-state phase transformations upon cooling by printing single-tracks onto a heated baseplate ranging from 50 °C to 600 °C surface temperature, which led to significant variation in the α-Cu and δ-Fe phase distribution, grain morphology, and chemical distribution within the deposited single-tracks. The printed microstructures exhibited as much as 80% difference in α-Cu grain size and nearly 30 % difference in α-Cu phase fraction due to baseplate temperature variation, indicating a wide range of available microstructures and properties achievable. Greater than 92% dense multi-layer samples were fabricated with fine grain structure and 27–34% higher hardness values compared to the barstock in the as-printed condition, demonstrating the applicability of this printing approach for multi-layer part fabrication. Our results highlight a unique microstructure tailoring capability for metal-AM parts that can be leveraged by manufacturers and end-users of AM technologies.http://www.sciencedirect.com/science/article/pii/S0264127523009607Additive manufacturingLiquid metal jettingAluminum bronzeMicrostructurePhase transformations
spellingShingle Kellen D. Traxel
Eric S. Elton
Amelia M. Petersen
Chinthaka M. Silva
Aurélien Perron
Jason R. Jeffries
Andrew J. Pascall
Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
Materials & Design
Additive manufacturing
Liquid metal jetting
Aluminum bronze
Microstructure
Phase transformations
title Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
title_full Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
title_fullStr Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
title_full_unstemmed Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
title_short Processing and microstructure of a Cu-Al-Fe-Mn alloy via droplet-on-demand additive manufacturing
title_sort processing and microstructure of a cu al fe mn alloy via droplet on demand additive manufacturing
topic Additive manufacturing
Liquid metal jetting
Aluminum bronze
Microstructure
Phase transformations
url http://www.sciencedirect.com/science/article/pii/S0264127523009607
work_keys_str_mv AT kellendtraxel processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT ericselton processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT ameliampetersen processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT chinthakamsilva processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT aurelienperron processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT jasonrjeffries processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing
AT andrewjpascall processingandmicrostructureofacualfemnalloyviadropletondemandadditivemanufacturing