Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City

Consideration of the relationship between residential floor level and concentration of traffic-related airborne pollutants may predict individual residential exposure among inner city dwellers more accurately. Our objective was to characterize the vertical gradient of residential levels of polycycli...

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Main Authors: Rachel L. Miller, Frederica P. Perera, David Camann, Patrick L. Kinney, Robin Whyatt, Beizhan Yan, Steven N. Chillrud, Kyung Hwa Jung, Kerlly Bernabé, Kathleen Moors
Format: Article
Language:English
Published: MDPI AG 2011-05-01
Series:Atmosphere
Subjects:
Online Access:http://www.mdpi.com/2073-4433/2/2/96/
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author Rachel L. Miller
Frederica P. Perera
David Camann
Patrick L. Kinney
Robin Whyatt
Beizhan Yan
Steven N. Chillrud
Kyung Hwa Jung
Kerlly Bernabé
Kathleen Moors
author_facet Rachel L. Miller
Frederica P. Perera
David Camann
Patrick L. Kinney
Robin Whyatt
Beizhan Yan
Steven N. Chillrud
Kyung Hwa Jung
Kerlly Bernabé
Kathleen Moors
author_sort Rachel L. Miller
collection DOAJ
description Consideration of the relationship between residential floor level and concentration of traffic-related airborne pollutants may predict individual residential exposure among inner city dwellers more accurately. Our objective was to characterize the vertical gradient of residential levels of polycyclic aromatic hydrocarbons (PAH; dichotomized into Σ8PAHsemivolatile (MW 178–206), and Σ8PAHnonvolatile (MW 228–278), black carbon (BC), PM2.5 (particulate matter) by floor level (FL), season and building type. We hypothesize that PAH, BC and PM2.5 concentrations may decrease with higher FL and the vertical gradients of these compounds would be affected by heating season and building type. PAH, BC and PM2.5 were measured over a two-week period outdoor and indoor of the residences of a cohort of 5–6 year old children (n = 339) living in New York City’s Northern Manhattan and the Bronx. Airborne-pollutant levels were analyzed by three categorized FL groups (0–2nd, 3rd–5th, and 6th–32nd FL) and two building types (low-rise versus high-rise apartment building). Indoor Σ8PAHnonvolatile and BC levels declined with increasing FL. During the nonheating season, the median outdoor Σ8PAHnonvolatile, but not Σ8PAHsemivolatile, level at 6th–2nd FL was 1.5–2 times lower than levels measured at lower FL. Similarly, outdoor and indoor BC concentrations at 6th–32nd FL were significantly lower than those at lower FL only during the nonheating season (p < 0.05). In addition, living in a low-rise building was associated significantly with higher levels of Σ8PAHnonvolatile and BC. These results suggest that young inner city children may be exposed to varying levels of air pollutants depending on their FL, season, and building type.
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spelling doaj.art-a24ee7eacbd3484caa9c0459f9c776602022-12-21T20:37:05ZengMDPI AGAtmosphere2073-44332011-05-01229610910.3390/atmos2020096Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York CityRachel L. MillerFrederica P. PereraDavid CamannPatrick L. KinneyRobin WhyattBeizhan YanSteven N. ChillrudKyung Hwa JungKerlly BernabéKathleen MoorsConsideration of the relationship between residential floor level and concentration of traffic-related airborne pollutants may predict individual residential exposure among inner city dwellers more accurately. Our objective was to characterize the vertical gradient of residential levels of polycyclic aromatic hydrocarbons (PAH; dichotomized into Σ8PAHsemivolatile (MW 178–206), and Σ8PAHnonvolatile (MW 228–278), black carbon (BC), PM2.5 (particulate matter) by floor level (FL), season and building type. We hypothesize that PAH, BC and PM2.5 concentrations may decrease with higher FL and the vertical gradients of these compounds would be affected by heating season and building type. PAH, BC and PM2.5 were measured over a two-week period outdoor and indoor of the residences of a cohort of 5–6 year old children (n = 339) living in New York City’s Northern Manhattan and the Bronx. Airborne-pollutant levels were analyzed by three categorized FL groups (0–2nd, 3rd–5th, and 6th–32nd FL) and two building types (low-rise versus high-rise apartment building). Indoor Σ8PAHnonvolatile and BC levels declined with increasing FL. During the nonheating season, the median outdoor Σ8PAHnonvolatile, but not Σ8PAHsemivolatile, level at 6th–2nd FL was 1.5–2 times lower than levels measured at lower FL. Similarly, outdoor and indoor BC concentrations at 6th–32nd FL were significantly lower than those at lower FL only during the nonheating season (p < 0.05). In addition, living in a low-rise building was associated significantly with higher levels of Σ8PAHnonvolatile and BC. These results suggest that young inner city children may be exposed to varying levels of air pollutants depending on their FL, season, and building type.http://www.mdpi.com/2073-4433/2/2/96/vertical gradientfloor level (FL)building typeheating seasontraffic-related air pollutionpolycyclic aromatic hydrocarbons (PAHs)outdoor and indoor
spellingShingle Rachel L. Miller
Frederica P. Perera
David Camann
Patrick L. Kinney
Robin Whyatt
Beizhan Yan
Steven N. Chillrud
Kyung Hwa Jung
Kerlly Bernabé
Kathleen Moors
Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
Atmosphere
vertical gradient
floor level (FL)
building type
heating season
traffic-related air pollution
polycyclic aromatic hydrocarbons (PAHs)
outdoor and indoor
title Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
title_full Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
title_fullStr Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
title_full_unstemmed Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
title_short Effects of Floor Level and Building Type on Residential Levels of Outdoor and Indoor Polycyclic Aromatic Hydrocarbons, Black Carbon, and Particulate Matter in New York City
title_sort effects of floor level and building type on residential levels of outdoor and indoor polycyclic aromatic hydrocarbons black carbon and particulate matter in new york city
topic vertical gradient
floor level (FL)
building type
heating season
traffic-related air pollution
polycyclic aromatic hydrocarbons (PAHs)
outdoor and indoor
url http://www.mdpi.com/2073-4433/2/2/96/
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