A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films

Energy-efficient computing paradigms beyond conventional von-Neumann architecture, such as neuromorphic computing, require novel devices that enable information storage at nanoscale in an analogue way and in-memory computing. Memristive devices with long-/short-term synaptic plasticity are expected...

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Main Author: Jong-Gul Yoon
Format: Article
Language:English
Published: MDPI AG 2020-08-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/13/17/3680
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author Jong-Gul Yoon
author_facet Jong-Gul Yoon
author_sort Jong-Gul Yoon
collection DOAJ
description Energy-efficient computing paradigms beyond conventional von-Neumann architecture, such as neuromorphic computing, require novel devices that enable information storage at nanoscale in an analogue way and in-memory computing. Memristive devices with long-/short-term synaptic plasticity are expected to provide a more capable neuromorphic system compared to traditional Si-based complementary metal-oxide-semiconductor circuits. Here, compositionally graded oxide films of Al-doped Mg<i><sub>x</sub></i>Zn<sub>1−<i>x</i></sub>O (<i>g</i>-Al:MgZnO) are studied to fabricate a memristive device, in which the composition of the film changes continuously through the film thickness. Compositional grading in the films should give rise to asymmetry of Schottky barrier heights at the film-electrode interfaces. The <i>g</i>-Al:MgZnO films are grown by using aerosol-assisted chemical vapor deposition. The current-voltage (<i>I-V</i>) and capacitance-voltage (<i>C-V</i>) characteristics of the films show self-rectifying memristive behaviors which are dependent on maximum applied voltage and repeated application of electrical pulses. Endurance and retention performance tests of the device show stable bipolar resistance switching (BRS) with a short-term memory effect. The short-term memory effects are ascribed to the thermally activated release of the trapped electrons near/at the <i>g</i>-Al:MgZnO film-electrode interface of the device. The volatile resistive switching can be used as a potential selector device in a crossbar memory array and a short-term synapse in neuromorphic computing.
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spelling doaj.art-a27d311659c34badbcfacced0b354b072023-11-20T10:47:45ZengMDPI AGMaterials1996-19442020-08-011317368010.3390/ma13173680A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded FilmsJong-Gul Yoon0Department of Physics and Electronic Materials Engineering, University of Suwon, Gyeonggi-do 18323, KoreaEnergy-efficient computing paradigms beyond conventional von-Neumann architecture, such as neuromorphic computing, require novel devices that enable information storage at nanoscale in an analogue way and in-memory computing. Memristive devices with long-/short-term synaptic plasticity are expected to provide a more capable neuromorphic system compared to traditional Si-based complementary metal-oxide-semiconductor circuits. Here, compositionally graded oxide films of Al-doped Mg<i><sub>x</sub></i>Zn<sub>1−<i>x</i></sub>O (<i>g</i>-Al:MgZnO) are studied to fabricate a memristive device, in which the composition of the film changes continuously through the film thickness. Compositional grading in the films should give rise to asymmetry of Schottky barrier heights at the film-electrode interfaces. The <i>g</i>-Al:MgZnO films are grown by using aerosol-assisted chemical vapor deposition. The current-voltage (<i>I-V</i>) and capacitance-voltage (<i>C-V</i>) characteristics of the films show self-rectifying memristive behaviors which are dependent on maximum applied voltage and repeated application of electrical pulses. Endurance and retention performance tests of the device show stable bipolar resistance switching (BRS) with a short-term memory effect. The short-term memory effects are ascribed to the thermally activated release of the trapped electrons near/at the <i>g</i>-Al:MgZnO film-electrode interface of the device. The volatile resistive switching can be used as a potential selector device in a crossbar memory array and a short-term synapse in neuromorphic computing.https://www.mdpi.com/1996-1944/13/17/3680compositionally graded oxide filmself-rectifying bipolar resistance switchingaerosol-assisted chemical depositionshort-term memoryZnO-based memristor
spellingShingle Jong-Gul Yoon
A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
Materials
compositionally graded oxide film
self-rectifying bipolar resistance switching
aerosol-assisted chemical deposition
short-term memory
ZnO-based memristor
title A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
title_full A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
title_fullStr A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
title_full_unstemmed A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
title_short A New Approach to the Fabrication of Memristive Neuromorphic Devices: Compositionally Graded Films
title_sort new approach to the fabrication of memristive neuromorphic devices compositionally graded films
topic compositionally graded oxide film
self-rectifying bipolar resistance switching
aerosol-assisted chemical deposition
short-term memory
ZnO-based memristor
url https://www.mdpi.com/1996-1944/13/17/3680
work_keys_str_mv AT jonggulyoon anewapproachtothefabricationofmemristiveneuromorphicdevicescompositionallygradedfilms
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