Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures

An accurate estimate of the ferroelectric polarization in ferroelectric-dielectric stacks is important from a materials science perspective, and it is also crucial for the development of ferroelectric based electron devices. This paper revisits the theory and application of the PUND technique in Met...

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Main Authors: Mattia Segatto, Riccardo Fontanini, Francesco Driussi, Daniel Lizzit, David Esseni
Format: Article
Language:English
Published: IEEE 2022-01-01
Series:IEEE Journal of the Electron Devices Society
Subjects:
Online Access:https://ieeexplore.ieee.org/document/9754361/
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author Mattia Segatto
Riccardo Fontanini
Francesco Driussi
Daniel Lizzit
David Esseni
author_facet Mattia Segatto
Riccardo Fontanini
Francesco Driussi
Daniel Lizzit
David Esseni
author_sort Mattia Segatto
collection DOAJ
description An accurate estimate of the ferroelectric polarization in ferroelectric-dielectric stacks is important from a materials science perspective, and it is also crucial for the development of ferroelectric based electron devices. This paper revisits the theory and application of the PUND technique in Metal-Ferroelectric-Dielectric-Metal (MFDM) structures by using analytical derivations and numerical simulations. In an MFDM structure the results of the PUND technique may largely differ from the polarization actually switched in the stack, which in turn is different from the remnant polarization of the underlying ferroelectric. The main hindrances that prevent PUND measurements from providing a good estimate of the polarization switching in MFDM stacks are thus discussed. The inspection of the involved physical quantities, not always accessible in experiments, provides a useful insight about the main sources of the errors in the PUND technique, and clarifies the delicate interplay between the depolarization field and the charge injection and trapping in MFDM stacks with a thin dielectric layer.
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spelling doaj.art-a306f22c7ffc44e4b50cf6dfde8d42f32022-12-22T00:46:01ZengIEEEIEEE Journal of the Electron Devices Society2168-67342022-01-011032433310.1109/JEDS.2022.31646529754361Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric HeterostructuresMattia Segatto0https://orcid.org/0000-0002-0091-1862Riccardo Fontanini1https://orcid.org/0000-0002-4246-946XFrancesco Driussi2https://orcid.org/0000-0003-2175-6977Daniel Lizzit3https://orcid.org/0000-0002-5243-5888David Esseni4https://orcid.org/0000-0002-3468-5197Department of DPIA, University of Udine, Udine, ItalyDepartment of DPIA, University of Udine, Udine, ItalyDepartment of DPIA, University of Udine, Udine, ItalyDepartment of DPIA, University of Udine, Udine, ItalyDepartment of DPIA, University of Udine, Udine, ItalyAn accurate estimate of the ferroelectric polarization in ferroelectric-dielectric stacks is important from a materials science perspective, and it is also crucial for the development of ferroelectric based electron devices. This paper revisits the theory and application of the PUND technique in Metal-Ferroelectric-Dielectric-Metal (MFDM) structures by using analytical derivations and numerical simulations. In an MFDM structure the results of the PUND technique may largely differ from the polarization actually switched in the stack, which in turn is different from the remnant polarization of the underlying ferroelectric. The main hindrances that prevent PUND measurements from providing a good estimate of the polarization switching in MFDM stacks are thus discussed. The inspection of the involved physical quantities, not always accessible in experiments, provides a useful insight about the main sources of the errors in the PUND technique, and clarifies the delicate interplay between the depolarization field and the charge injection and trapping in MFDM stacks with a thin dielectric layer.https://ieeexplore.ieee.org/document/9754361/HZOferroelectricMFDMdielectricPUNDdepolarization
spellingShingle Mattia Segatto
Riccardo Fontanini
Francesco Driussi
Daniel Lizzit
David Esseni
Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
IEEE Journal of the Electron Devices Society
HZO
ferroelectric
MFDM
dielectric
PUND
depolarization
title Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
title_full Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
title_fullStr Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
title_full_unstemmed Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
title_short Limitations to Electrical Probing of Spontaneous Polarization in Ferroelectric-Dielectric Heterostructures
title_sort limitations to electrical probing of spontaneous polarization in ferroelectric dielectric heterostructures
topic HZO
ferroelectric
MFDM
dielectric
PUND
depolarization
url https://ieeexplore.ieee.org/document/9754361/
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AT riccardofontanini limitationstoelectricalprobingofspontaneouspolarizationinferroelectricdielectricheterostructures
AT francescodriussi limitationstoelectricalprobingofspontaneouspolarizationinferroelectricdielectricheterostructures
AT daniellizzit limitationstoelectricalprobingofspontaneouspolarizationinferroelectricdielectricheterostructures
AT davidesseni limitationstoelectricalprobingofspontaneouspolarizationinferroelectricdielectricheterostructures