Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management

Serious pollution of multiple chemicals in irregulated e-waste recycling sites (IR-sites) were extensively investigated. However, little is known about the pollution in regulated sites. This study investigated the occurrence of 21 polybrominated diphenyl ethers (PBDEs) and 10 metals in a regulated s...

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Main Authors: Hongmin Yin, Jiayi Ma, Zhidong Li, Yonghong Li, Tong Meng, Zhenwu Tang
Format: Article
Language:English
Published: MDPI AG 2021-04-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/26/8/2169
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author Hongmin Yin
Jiayi Ma
Zhidong Li
Yonghong Li
Tong Meng
Zhenwu Tang
author_facet Hongmin Yin
Jiayi Ma
Zhidong Li
Yonghong Li
Tong Meng
Zhenwu Tang
author_sort Hongmin Yin
collection DOAJ
description Serious pollution of multiple chemicals in irregulated e-waste recycling sites (IR-sites) were extensively investigated. However, little is known about the pollution in regulated sites. This study investigated the occurrence of 21 polybrominated diphenyl ethers (PBDEs) and 10 metals in a regulated site, in Eastern China. The concentrations of PBDEs and Cd, Cu, Pb, Sb, and Zn in soils and sediments were 1–4 and 1–3 orders of magnitude lower than those reported in the IR-sites, respectively. However, these were generally comparable to those in the urban and industrial areas. In general, a moderate pollution of PBDEs and metals was present in the vegetables in this area. A health risk assessment model was used to calculate human exposure to metals in soils. The summed non-carcinogenic risks of metals and PBDEs in the investigated soils were 1.59–3.27 and 0.25–0.51 for children and adults, respectively. Arsenic contributed to 47% of the total risks and As risks in 71.4% of the total soil samples exceeded the acceptable level. These results suggested that the pollution from e-waste recycling could be substantially decreased by the regulated activities, relative to poorly controlled operations, but arsenic pollution from the regulated cycling should be further controlled.
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spelling doaj.art-a37f12eab2094eb6b2efc6a283198d9c2023-11-21T14:52:18ZengMDPI AGMolecules1420-30492021-04-01268216910.3390/molecules26082169Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk ManagementHongmin Yin0Jiayi Ma1Zhidong Li2Yonghong Li3Tong Meng4Zhenwu Tang5College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, ChinaCollege of Life and Environmental Sciences, Minzu University of China, Beijing 100081, ChinaCangzhou Ecology and Environment Bureau, Cangzhou 061000, ChinaCollege of Life and Environmental Sciences, Minzu University of China, Beijing 100081, ChinaCollege of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, ChinaCollege of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, ChinaSerious pollution of multiple chemicals in irregulated e-waste recycling sites (IR-sites) were extensively investigated. However, little is known about the pollution in regulated sites. This study investigated the occurrence of 21 polybrominated diphenyl ethers (PBDEs) and 10 metals in a regulated site, in Eastern China. The concentrations of PBDEs and Cd, Cu, Pb, Sb, and Zn in soils and sediments were 1–4 and 1–3 orders of magnitude lower than those reported in the IR-sites, respectively. However, these were generally comparable to those in the urban and industrial areas. In general, a moderate pollution of PBDEs and metals was present in the vegetables in this area. A health risk assessment model was used to calculate human exposure to metals in soils. The summed non-carcinogenic risks of metals and PBDEs in the investigated soils were 1.59–3.27 and 0.25–0.51 for children and adults, respectively. Arsenic contributed to 47% of the total risks and As risks in 71.4% of the total soil samples exceeded the acceptable level. These results suggested that the pollution from e-waste recycling could be substantially decreased by the regulated activities, relative to poorly controlled operations, but arsenic pollution from the regulated cycling should be further controlled.https://www.mdpi.com/1420-3049/26/8/2169regulated e-waste recyclingpolybrominated diphenyl ethers (PBDEs)heavy metalsenvironmental mediavegetablerisks
spellingShingle Hongmin Yin
Jiayi Ma
Zhidong Li
Yonghong Li
Tong Meng
Zhenwu Tang
Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
Molecules
regulated e-waste recycling
polybrominated diphenyl ethers (PBDEs)
heavy metals
environmental media
vegetable
risks
title Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
title_full Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
title_fullStr Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
title_full_unstemmed Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
title_short Polybrominated Diphenyl Ethers and Heavy Metals in a Regulated E-Waste Recycling Site, Eastern China: Implications for Risk Management
title_sort polybrominated diphenyl ethers and heavy metals in a regulated e waste recycling site eastern china implications for risk management
topic regulated e-waste recycling
polybrominated diphenyl ethers (PBDEs)
heavy metals
environmental media
vegetable
risks
url https://www.mdpi.com/1420-3049/26/8/2169
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